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Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters

In light of the emergence of nonclassical effects, a paradigm shift in the conventional macroscopic treatment is required to accurately describe the interaction between light and plasmonic structures with deep-nanometer features. Towards this end, several nonlocal response models, supplemented by ad...

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Autores principales: Kupresak, Mario, Zheng, Xuezhi, Mittra, Raj, Vandenbosch, Guy A. E., Moshchalkov, Victor V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: RSC 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9419619/
https://www.ncbi.nlm.nih.gov/pubmed/36133694
http://dx.doi.org/10.1039/d1na00726b
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author Kupresak, Mario
Zheng, Xuezhi
Mittra, Raj
Vandenbosch, Guy A. E.
Moshchalkov, Victor V.
author_facet Kupresak, Mario
Zheng, Xuezhi
Mittra, Raj
Vandenbosch, Guy A. E.
Moshchalkov, Victor V.
author_sort Kupresak, Mario
collection PubMed
description In light of the emergence of nonclassical effects, a paradigm shift in the conventional macroscopic treatment is required to accurately describe the interaction between light and plasmonic structures with deep-nanometer features. Towards this end, several nonlocal response models, supplemented by additional boundary conditions, have been introduced, investigating the collective motion of the free electron gas in metals. The study of the dipole-excited core–shell nanoparticle has been performed, by employing the following models: the hard-wall hydrodynamic model; the quantum hydrodynamic model; and the generalized nonlocal optical response. The analysis is conducted by investigating the near and far field characteristics of the emitter–nanoparticle system, while considering the emitter outside and inside the studied topology. It is shown that the above models predict striking spectral features, strongly deviating from the results obtained via the classical approach, for both simple and noble constitutive metals.
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spelling pubmed-94196192022-09-20 Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters Kupresak, Mario Zheng, Xuezhi Mittra, Raj Vandenbosch, Guy A. E. Moshchalkov, Victor V. Nanoscale Adv Chemistry In light of the emergence of nonclassical effects, a paradigm shift in the conventional macroscopic treatment is required to accurately describe the interaction between light and plasmonic structures with deep-nanometer features. Towards this end, several nonlocal response models, supplemented by additional boundary conditions, have been introduced, investigating the collective motion of the free electron gas in metals. The study of the dipole-excited core–shell nanoparticle has been performed, by employing the following models: the hard-wall hydrodynamic model; the quantum hydrodynamic model; and the generalized nonlocal optical response. The analysis is conducted by investigating the near and far field characteristics of the emitter–nanoparticle system, while considering the emitter outside and inside the studied topology. It is shown that the above models predict striking spectral features, strongly deviating from the results obtained via the classical approach, for both simple and noble constitutive metals. RSC 2022-04-25 /pmc/articles/PMC9419619/ /pubmed/36133694 http://dx.doi.org/10.1039/d1na00726b Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Kupresak, Mario
Zheng, Xuezhi
Mittra, Raj
Vandenbosch, Guy A. E.
Moshchalkov, Victor V.
Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
title Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
title_full Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
title_fullStr Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
title_full_unstemmed Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
title_short Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
title_sort nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9419619/
https://www.ncbi.nlm.nih.gov/pubmed/36133694
http://dx.doi.org/10.1039/d1na00726b
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