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Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters
In light of the emergence of nonclassical effects, a paradigm shift in the conventional macroscopic treatment is required to accurately describe the interaction between light and plasmonic structures with deep-nanometer features. Towards this end, several nonlocal response models, supplemented by ad...
Autores principales: | , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
RSC
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9419619/ https://www.ncbi.nlm.nih.gov/pubmed/36133694 http://dx.doi.org/10.1039/d1na00726b |
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author | Kupresak, Mario Zheng, Xuezhi Mittra, Raj Vandenbosch, Guy A. E. Moshchalkov, Victor V. |
author_facet | Kupresak, Mario Zheng, Xuezhi Mittra, Raj Vandenbosch, Guy A. E. Moshchalkov, Victor V. |
author_sort | Kupresak, Mario |
collection | PubMed |
description | In light of the emergence of nonclassical effects, a paradigm shift in the conventional macroscopic treatment is required to accurately describe the interaction between light and plasmonic structures with deep-nanometer features. Towards this end, several nonlocal response models, supplemented by additional boundary conditions, have been introduced, investigating the collective motion of the free electron gas in metals. The study of the dipole-excited core–shell nanoparticle has been performed, by employing the following models: the hard-wall hydrodynamic model; the quantum hydrodynamic model; and the generalized nonlocal optical response. The analysis is conducted by investigating the near and far field characteristics of the emitter–nanoparticle system, while considering the emitter outside and inside the studied topology. It is shown that the above models predict striking spectral features, strongly deviating from the results obtained via the classical approach, for both simple and noble constitutive metals. |
format | Online Article Text |
id | pubmed-9419619 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | RSC |
record_format | MEDLINE/PubMed |
spelling | pubmed-94196192022-09-20 Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters Kupresak, Mario Zheng, Xuezhi Mittra, Raj Vandenbosch, Guy A. E. Moshchalkov, Victor V. Nanoscale Adv Chemistry In light of the emergence of nonclassical effects, a paradigm shift in the conventional macroscopic treatment is required to accurately describe the interaction between light and plasmonic structures with deep-nanometer features. Towards this end, several nonlocal response models, supplemented by additional boundary conditions, have been introduced, investigating the collective motion of the free electron gas in metals. The study of the dipole-excited core–shell nanoparticle has been performed, by employing the following models: the hard-wall hydrodynamic model; the quantum hydrodynamic model; and the generalized nonlocal optical response. The analysis is conducted by investigating the near and far field characteristics of the emitter–nanoparticle system, while considering the emitter outside and inside the studied topology. It is shown that the above models predict striking spectral features, strongly deviating from the results obtained via the classical approach, for both simple and noble constitutive metals. RSC 2022-04-25 /pmc/articles/PMC9419619/ /pubmed/36133694 http://dx.doi.org/10.1039/d1na00726b Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Kupresak, Mario Zheng, Xuezhi Mittra, Raj Vandenbosch, Guy A. E. Moshchalkov, Victor V. Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
title | Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
title_full | Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
title_fullStr | Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
title_full_unstemmed | Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
title_short | Nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
title_sort | nonlocal response of plasmonic core–shell nanotopologies excited by dipole emitters |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9419619/ https://www.ncbi.nlm.nih.gov/pubmed/36133694 http://dx.doi.org/10.1039/d1na00726b |
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