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Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot
A theoretical investigation on neutral excitons confined to a mono-layer (ML) semiconductor transition metal dichalcogenide (TMDC) materials under the influence of elliptically deformed gate induced confining potential is presented. It has been shown that the anisotropy of the confinement induces th...
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Formato: | Online Artículo Texto |
Lenguaje: | English |
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Nature Publishing Group UK
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9427995/ https://www.ncbi.nlm.nih.gov/pubmed/36042272 http://dx.doi.org/10.1038/s41598-022-19119-2 |
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author | Poszwa, A. |
author_facet | Poszwa, A. |
author_sort | Poszwa, A. |
collection | PubMed |
description | A theoretical investigation on neutral excitons confined to a mono-layer (ML) semiconductor transition metal dichalcogenide (TMDC) materials under the influence of elliptically deformed gate induced confining potential is presented. It has been shown that the anisotropy of the confinement induces the anisotropy of linear response of the system on in-plane external electric field. The linear response is expressed in terms of principal moments of the static dipole polarizability tensor. In this manner the direction-dependent polarizability of the system can be fully controlled by tuning the parameters of gate-induced confining potential. The components of the polarizability tensor are determined using finite-field method based on the exact diagonalization of the electron-hole Hamiltonian including confining potential, Coulomb electron-hole interaction and an external electric field, within effective mass approximation, close to the K-points of the first Brillouin zone of a single-layer MX[Formula: see text] material. The useful scaling relations for energies and dipole polarizabilities as functions of material parameters have been found. The influence of the anisotropy of the confining potential on correlated behavior of charge distribution inside the neutral system has also been demonstrated. |
format | Online Article Text |
id | pubmed-9427995 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-94279952022-09-01 Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot Poszwa, A. Sci Rep Article A theoretical investigation on neutral excitons confined to a mono-layer (ML) semiconductor transition metal dichalcogenide (TMDC) materials under the influence of elliptically deformed gate induced confining potential is presented. It has been shown that the anisotropy of the confinement induces the anisotropy of linear response of the system on in-plane external electric field. The linear response is expressed in terms of principal moments of the static dipole polarizability tensor. In this manner the direction-dependent polarizability of the system can be fully controlled by tuning the parameters of gate-induced confining potential. The components of the polarizability tensor are determined using finite-field method based on the exact diagonalization of the electron-hole Hamiltonian including confining potential, Coulomb electron-hole interaction and an external electric field, within effective mass approximation, close to the K-points of the first Brillouin zone of a single-layer MX[Formula: see text] material. The useful scaling relations for energies and dipole polarizabilities as functions of material parameters have been found. The influence of the anisotropy of the confining potential on correlated behavior of charge distribution inside the neutral system has also been demonstrated. Nature Publishing Group UK 2022-08-30 /pmc/articles/PMC9427995/ /pubmed/36042272 http://dx.doi.org/10.1038/s41598-022-19119-2 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Poszwa, A. Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot |
title | Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot |
title_full | Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot |
title_fullStr | Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot |
title_full_unstemmed | Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot |
title_short | Geometry-modulated dipole polarizability of the two-dimensional Mott-Wannier excitons in gate-defined anisotropic quantum dot |
title_sort | geometry-modulated dipole polarizability of the two-dimensional mott-wannier excitons in gate-defined anisotropic quantum dot |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9427995/ https://www.ncbi.nlm.nih.gov/pubmed/36042272 http://dx.doi.org/10.1038/s41598-022-19119-2 |
work_keys_str_mv | AT poszwaa geometrymodulateddipolepolarizabilityofthetwodimensionalmottwannierexcitonsingatedefinedanisotropicquantumdot |