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Phonon drag thermal Hall effect in metallic strontium titanate
SrTiO(3), a quantum paralectric, displays a detectable phonon thermal Hall effect (THE). Here, we show that the amplitude of the THE is extremely sensitive to stoichiometry. It drastically decreases upon substitution of a tiny fraction of Sr atoms with Ca, which stabilizes the ferroelectric order. I...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
National Academy of Sciences
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9436374/ https://www.ncbi.nlm.nih.gov/pubmed/35994652 http://dx.doi.org/10.1073/pnas.2201975119 |
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author | Jiang, Shan Li, Xiaokang Fauqué, Benoît Behnia, Kamran |
author_facet | Jiang, Shan Li, Xiaokang Fauqué, Benoît Behnia, Kamran |
author_sort | Jiang, Shan |
collection | PubMed |
description | SrTiO(3), a quantum paralectric, displays a detectable phonon thermal Hall effect (THE). Here, we show that the amplitude of the THE is extremely sensitive to stoichiometry. It drastically decreases upon substitution of a tiny fraction of Sr atoms with Ca, which stabilizes the ferroelectric order. It drastically increases by an even lower density of oxygen vacancies, which turn the system to a dilute metal. The enhancement in the metallic state exceeds by far the sum of the electronic and the phononic contributions. We explain this observation as an outcome of three features: 1) Heat is mostly transported by phonons; 2) the electronic Hall angle is extremely large; and 3) there is substantial momentum exchange between electrons and phonons. Starting from Herring’s picture of phonon drag, we arrive to a quantitative account of the enhanced THE. Thus, phonon drag, hitherto detected as an amplifier of thermoelectric coefficients, can generate a purely thermal transverse response in a dilute metal with a large Hall angle. Our results reveal a hitherto-unknown consequence of momentum-conserving collisions between electrons and phonons. |
format | Online Article Text |
id | pubmed-9436374 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | National Academy of Sciences |
record_format | MEDLINE/PubMed |
spelling | pubmed-94363742023-02-22 Phonon drag thermal Hall effect in metallic strontium titanate Jiang, Shan Li, Xiaokang Fauqué, Benoît Behnia, Kamran Proc Natl Acad Sci U S A Physical Sciences SrTiO(3), a quantum paralectric, displays a detectable phonon thermal Hall effect (THE). Here, we show that the amplitude of the THE is extremely sensitive to stoichiometry. It drastically decreases upon substitution of a tiny fraction of Sr atoms with Ca, which stabilizes the ferroelectric order. It drastically increases by an even lower density of oxygen vacancies, which turn the system to a dilute metal. The enhancement in the metallic state exceeds by far the sum of the electronic and the phononic contributions. We explain this observation as an outcome of three features: 1) Heat is mostly transported by phonons; 2) the electronic Hall angle is extremely large; and 3) there is substantial momentum exchange between electrons and phonons. Starting from Herring’s picture of phonon drag, we arrive to a quantitative account of the enhanced THE. Thus, phonon drag, hitherto detected as an amplifier of thermoelectric coefficients, can generate a purely thermal transverse response in a dilute metal with a large Hall angle. Our results reveal a hitherto-unknown consequence of momentum-conserving collisions between electrons and phonons. National Academy of Sciences 2022-08-22 2022-08-30 /pmc/articles/PMC9436374/ /pubmed/35994652 http://dx.doi.org/10.1073/pnas.2201975119 Text en Copyright © 2022 the Author(s). Published by PNAS. https://creativecommons.org/licenses/by-nc-nd/4.0/This article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND) (https://creativecommons.org/licenses/by-nc-nd/4.0/) . |
spellingShingle | Physical Sciences Jiang, Shan Li, Xiaokang Fauqué, Benoît Behnia, Kamran Phonon drag thermal Hall effect in metallic strontium titanate |
title | Phonon drag thermal Hall effect in metallic strontium titanate |
title_full | Phonon drag thermal Hall effect in metallic strontium titanate |
title_fullStr | Phonon drag thermal Hall effect in metallic strontium titanate |
title_full_unstemmed | Phonon drag thermal Hall effect in metallic strontium titanate |
title_short | Phonon drag thermal Hall effect in metallic strontium titanate |
title_sort | phonon drag thermal hall effect in metallic strontium titanate |
topic | Physical Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9436374/ https://www.ncbi.nlm.nih.gov/pubmed/35994652 http://dx.doi.org/10.1073/pnas.2201975119 |
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