Cargando…
Attosecond dynamics of multi-channel single photon ionization
Photoionization of atoms and molecules is one of the fastest processes in nature. The understanding of the ultrafast temporal dynamics of this process often requires the characterization of the different angular momentum channels over a broad energy range. Using a two-photon interferometry technique...
Autores principales: | , , , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9440915/ https://www.ncbi.nlm.nih.gov/pubmed/36057622 http://dx.doi.org/10.1038/s41467-022-32780-5 |
_version_ | 1784782463454674944 |
---|---|
author | Peschel, Jasper Busto, David Plach, Marius Bertolino, Mattias Hoflund, Maria Maclot, Sylvain Vinbladh, Jimmy Wikmark, Hampus Zapata, Felipe Lindroth, Eva Gisselbrecht, Mathieu Dahlström, Jan Marcus L’Huillier, Anne Eng-Johnsson, Per |
author_facet | Peschel, Jasper Busto, David Plach, Marius Bertolino, Mattias Hoflund, Maria Maclot, Sylvain Vinbladh, Jimmy Wikmark, Hampus Zapata, Felipe Lindroth, Eva Gisselbrecht, Mathieu Dahlström, Jan Marcus L’Huillier, Anne Eng-Johnsson, Per |
author_sort | Peschel, Jasper |
collection | PubMed |
description | Photoionization of atoms and molecules is one of the fastest processes in nature. The understanding of the ultrafast temporal dynamics of this process often requires the characterization of the different angular momentum channels over a broad energy range. Using a two-photon interferometry technique based on extreme ultraviolet and infrared ultrashort pulses, we measure the phase and amplitude of the individual angular momentum channels as a function of kinetic energy in the outer-shell photoionization of neon. This allows us to unravel the influence of channel interference as well as the effect of the short-range, Coulomb and centrifugal potentials, on the dynamics of the photoionization process. |
format | Online Article Text |
id | pubmed-9440915 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-94409152022-09-05 Attosecond dynamics of multi-channel single photon ionization Peschel, Jasper Busto, David Plach, Marius Bertolino, Mattias Hoflund, Maria Maclot, Sylvain Vinbladh, Jimmy Wikmark, Hampus Zapata, Felipe Lindroth, Eva Gisselbrecht, Mathieu Dahlström, Jan Marcus L’Huillier, Anne Eng-Johnsson, Per Nat Commun Article Photoionization of atoms and molecules is one of the fastest processes in nature. The understanding of the ultrafast temporal dynamics of this process often requires the characterization of the different angular momentum channels over a broad energy range. Using a two-photon interferometry technique based on extreme ultraviolet and infrared ultrashort pulses, we measure the phase and amplitude of the individual angular momentum channels as a function of kinetic energy in the outer-shell photoionization of neon. This allows us to unravel the influence of channel interference as well as the effect of the short-range, Coulomb and centrifugal potentials, on the dynamics of the photoionization process. Nature Publishing Group UK 2022-09-03 /pmc/articles/PMC9440915/ /pubmed/36057622 http://dx.doi.org/10.1038/s41467-022-32780-5 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Peschel, Jasper Busto, David Plach, Marius Bertolino, Mattias Hoflund, Maria Maclot, Sylvain Vinbladh, Jimmy Wikmark, Hampus Zapata, Felipe Lindroth, Eva Gisselbrecht, Mathieu Dahlström, Jan Marcus L’Huillier, Anne Eng-Johnsson, Per Attosecond dynamics of multi-channel single photon ionization |
title | Attosecond dynamics of multi-channel single photon ionization |
title_full | Attosecond dynamics of multi-channel single photon ionization |
title_fullStr | Attosecond dynamics of multi-channel single photon ionization |
title_full_unstemmed | Attosecond dynamics of multi-channel single photon ionization |
title_short | Attosecond dynamics of multi-channel single photon ionization |
title_sort | attosecond dynamics of multi-channel single photon ionization |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9440915/ https://www.ncbi.nlm.nih.gov/pubmed/36057622 http://dx.doi.org/10.1038/s41467-022-32780-5 |
work_keys_str_mv | AT pescheljasper attoseconddynamicsofmultichannelsinglephotonionization AT bustodavid attoseconddynamicsofmultichannelsinglephotonionization AT plachmarius attoseconddynamicsofmultichannelsinglephotonionization AT bertolinomattias attoseconddynamicsofmultichannelsinglephotonionization AT hoflundmaria attoseconddynamicsofmultichannelsinglephotonionization AT maclotsylvain attoseconddynamicsofmultichannelsinglephotonionization AT vinbladhjimmy attoseconddynamicsofmultichannelsinglephotonionization AT wikmarkhampus attoseconddynamicsofmultichannelsinglephotonionization AT zapatafelipe attoseconddynamicsofmultichannelsinglephotonionization AT lindrotheva attoseconddynamicsofmultichannelsinglephotonionization AT gisselbrechtmathieu attoseconddynamicsofmultichannelsinglephotonionization AT dahlstromjanmarcus attoseconddynamicsofmultichannelsinglephotonionization AT lhuillieranne attoseconddynamicsofmultichannelsinglephotonionization AT engjohnssonper attoseconddynamicsofmultichannelsinglephotonionization |