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Probing the Free Energy of Small Water Clusters: Revisiting Classical Nucleation Theory
[Image: see text] By addressing the defects in classical nucleation theory (CNT), we develop an approach for extracting the free energy of small water clusters from nucleation rate experiments without any assumptions about the form of the cluster free energy. For temperatures higher than ∼250 K, the...
Autores principales: | Afzalifar, Ali, Shields, George C., Fowler, Vance R., Ras, Robin H. A. |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9442792/ https://www.ncbi.nlm.nih.gov/pubmed/35993823 http://dx.doi.org/10.1021/acs.jpclett.2c01361 |
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