Cargando…
On the adsorption and reactivity of element 114, flerovium
Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas...
Autores principales: | , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Frontiers Media S.A.
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9453156/ https://www.ncbi.nlm.nih.gov/pubmed/36092655 http://dx.doi.org/10.3389/fchem.2022.976635 |
_version_ | 1784785081916719104 |
---|---|
author | Yakushev, A. Lens, L. Düllmann, Ch. E. Khuyagbaatar, J. Jäger, E. Krier, J. Runke, J. Albers, H. M. Asai, M. Block, M. Despotopulos, J. Di Nitto, A. Eberhardt, K. Forsberg, U. Golubev, P. Götz, M. Götz, S. Haba, H. Harkness-Brennan, L. Herzberg, R.-D. Heßberger, F. P. Hinde, D. Hübner, A. Judson, D. Kindler, B. Komori, Y. Konki, J. Kratz, J.V. Kurz, N. Laatiaoui, M. Lahiri, S. Lommel, B. Maiti, M. Mistry, A. K. Mokry, Ch. Moody, K. J. Nagame, Y. Omtvedt, J. P. Papadakis, P. Pershina, V. Rudolph, D. Samiento, L.G. Sato, T.K. Schädel, M. Scharrer, P. Schausten, B. Shaughnessy, D. A. Steiner, J. Thörle-Pospiech, P. Toyoshima, A. Trautmann, N. Tsukada, K. Uusitalo, J. Voss, K.-O. Ward, A. Wegrzecki, M. Wiehl, N. Williams, E. Yakusheva, V. |
author_facet | Yakushev, A. Lens, L. Düllmann, Ch. E. Khuyagbaatar, J. Jäger, E. Krier, J. Runke, J. Albers, H. M. Asai, M. Block, M. Despotopulos, J. Di Nitto, A. Eberhardt, K. Forsberg, U. Golubev, P. Götz, M. Götz, S. Haba, H. Harkness-Brennan, L. Herzberg, R.-D. Heßberger, F. P. Hinde, D. Hübner, A. Judson, D. Kindler, B. Komori, Y. Konki, J. Kratz, J.V. Kurz, N. Laatiaoui, M. Lahiri, S. Lommel, B. Maiti, M. Mistry, A. K. Mokry, Ch. Moody, K. J. Nagame, Y. Omtvedt, J. P. Papadakis, P. Pershina, V. Rudolph, D. Samiento, L.G. Sato, T.K. Schädel, M. Scharrer, P. Schausten, B. Shaughnessy, D. A. Steiner, J. Thörle-Pospiech, P. Toyoshima, A. Trautmann, N. Tsukada, K. Uusitalo, J. Voss, K.-O. Ward, A. Wegrzecki, M. Wiehl, N. Williams, E. Yakusheva, V. |
author_sort | Yakushev, A. |
collection | PubMed |
description | Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn. |
format | Online Article Text |
id | pubmed-9453156 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Frontiers Media S.A. |
record_format | MEDLINE/PubMed |
spelling | pubmed-94531562022-09-09 On the adsorption and reactivity of element 114, flerovium Yakushev, A. Lens, L. Düllmann, Ch. E. Khuyagbaatar, J. Jäger, E. Krier, J. Runke, J. Albers, H. M. Asai, M. Block, M. Despotopulos, J. Di Nitto, A. Eberhardt, K. Forsberg, U. Golubev, P. Götz, M. Götz, S. Haba, H. Harkness-Brennan, L. Herzberg, R.-D. Heßberger, F. P. Hinde, D. Hübner, A. Judson, D. Kindler, B. Komori, Y. Konki, J. Kratz, J.V. Kurz, N. Laatiaoui, M. Lahiri, S. Lommel, B. Maiti, M. Mistry, A. K. Mokry, Ch. Moody, K. J. Nagame, Y. Omtvedt, J. P. Papadakis, P. Pershina, V. Rudolph, D. Samiento, L.G. Sato, T.K. Schädel, M. Scharrer, P. Schausten, B. Shaughnessy, D. A. Steiner, J. Thörle-Pospiech, P. Toyoshima, A. Trautmann, N. Tsukada, K. Uusitalo, J. Voss, K.-O. Ward, A. Wegrzecki, M. Wiehl, N. Williams, E. Yakusheva, V. Front Chem Chemistry Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn. Frontiers Media S.A. 2022-08-25 /pmc/articles/PMC9453156/ /pubmed/36092655 http://dx.doi.org/10.3389/fchem.2022.976635 Text en Copyright © 2022 Yakushev, Lens, Düllmann, Khuyagbaatar, Jäger, Krier, Runke, Albers, Asai, Block, Despotopulos, Di Nitto, Eberhardt, Forsberg, Golubev, Götz, Götz, Haba, Harkness-Brennan, Herzberg, Heßberger, Hinde, Hübner, Judson, Kindler, Komori, Konki, Kratz, Kurz, Laatiaoui, Lahiri, Lommel, Maiti, Mistry, Mokry, Moody, Nagame, Omtvedt, Papadakis, Pershina, Rudolph, Samiento, Sato, Schädel, Scharrer, Schausten, Shaughnessy, Steiner, Thörle-Pospiech, Toyoshima, Trautmann, Tsukada, Uusitalo, Voss, Ward, Wegrzecki, Wiehl, Williams and Yakusheva. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms. |
spellingShingle | Chemistry Yakushev, A. Lens, L. Düllmann, Ch. E. Khuyagbaatar, J. Jäger, E. Krier, J. Runke, J. Albers, H. M. Asai, M. Block, M. Despotopulos, J. Di Nitto, A. Eberhardt, K. Forsberg, U. Golubev, P. Götz, M. Götz, S. Haba, H. Harkness-Brennan, L. Herzberg, R.-D. Heßberger, F. P. Hinde, D. Hübner, A. Judson, D. Kindler, B. Komori, Y. Konki, J. Kratz, J.V. Kurz, N. Laatiaoui, M. Lahiri, S. Lommel, B. Maiti, M. Mistry, A. K. Mokry, Ch. Moody, K. J. Nagame, Y. Omtvedt, J. P. Papadakis, P. Pershina, V. Rudolph, D. Samiento, L.G. Sato, T.K. Schädel, M. Scharrer, P. Schausten, B. Shaughnessy, D. A. Steiner, J. Thörle-Pospiech, P. Toyoshima, A. Trautmann, N. Tsukada, K. Uusitalo, J. Voss, K.-O. Ward, A. Wegrzecki, M. Wiehl, N. Williams, E. Yakusheva, V. On the adsorption and reactivity of element 114, flerovium |
title | On the adsorption and reactivity of element 114, flerovium |
title_full | On the adsorption and reactivity of element 114, flerovium |
title_fullStr | On the adsorption and reactivity of element 114, flerovium |
title_full_unstemmed | On the adsorption and reactivity of element 114, flerovium |
title_short | On the adsorption and reactivity of element 114, flerovium |
title_sort | on the adsorption and reactivity of element 114, flerovium |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9453156/ https://www.ncbi.nlm.nih.gov/pubmed/36092655 http://dx.doi.org/10.3389/fchem.2022.976635 |
work_keys_str_mv | AT yakusheva ontheadsorptionandreactivityofelement114flerovium AT lensl ontheadsorptionandreactivityofelement114flerovium AT dullmannche ontheadsorptionandreactivityofelement114flerovium AT khuyagbaatarj ontheadsorptionandreactivityofelement114flerovium AT jagere ontheadsorptionandreactivityofelement114flerovium AT krierj ontheadsorptionandreactivityofelement114flerovium AT runkej ontheadsorptionandreactivityofelement114flerovium AT albershm ontheadsorptionandreactivityofelement114flerovium AT asaim ontheadsorptionandreactivityofelement114flerovium AT blockm ontheadsorptionandreactivityofelement114flerovium AT despotopulosj ontheadsorptionandreactivityofelement114flerovium AT dinittoa ontheadsorptionandreactivityofelement114flerovium AT eberhardtk ontheadsorptionandreactivityofelement114flerovium AT forsbergu ontheadsorptionandreactivityofelement114flerovium AT golubevp ontheadsorptionandreactivityofelement114flerovium AT gotzm ontheadsorptionandreactivityofelement114flerovium AT gotzs ontheadsorptionandreactivityofelement114flerovium AT habah ontheadsorptionandreactivityofelement114flerovium AT harknessbrennanl ontheadsorptionandreactivityofelement114flerovium AT herzbergrd ontheadsorptionandreactivityofelement114flerovium AT heßbergerfp ontheadsorptionandreactivityofelement114flerovium AT hinded ontheadsorptionandreactivityofelement114flerovium AT hubnera ontheadsorptionandreactivityofelement114flerovium AT judsond ontheadsorptionandreactivityofelement114flerovium AT kindlerb ontheadsorptionandreactivityofelement114flerovium AT komoriy ontheadsorptionandreactivityofelement114flerovium AT konkij ontheadsorptionandreactivityofelement114flerovium AT kratzjv ontheadsorptionandreactivityofelement114flerovium AT kurzn ontheadsorptionandreactivityofelement114flerovium AT laatiaouim ontheadsorptionandreactivityofelement114flerovium AT lahiris ontheadsorptionandreactivityofelement114flerovium AT lommelb ontheadsorptionandreactivityofelement114flerovium AT maitim ontheadsorptionandreactivityofelement114flerovium AT mistryak ontheadsorptionandreactivityofelement114flerovium AT mokrych ontheadsorptionandreactivityofelement114flerovium AT moodykj ontheadsorptionandreactivityofelement114flerovium AT nagamey ontheadsorptionandreactivityofelement114flerovium AT omtvedtjp ontheadsorptionandreactivityofelement114flerovium AT papadakisp ontheadsorptionandreactivityofelement114flerovium AT pershinav ontheadsorptionandreactivityofelement114flerovium AT rudolphd ontheadsorptionandreactivityofelement114flerovium AT samientolg ontheadsorptionandreactivityofelement114flerovium AT satotk ontheadsorptionandreactivityofelement114flerovium AT schadelm ontheadsorptionandreactivityofelement114flerovium AT scharrerp ontheadsorptionandreactivityofelement114flerovium AT schaustenb ontheadsorptionandreactivityofelement114flerovium AT shaughnessyda ontheadsorptionandreactivityofelement114flerovium AT steinerj ontheadsorptionandreactivityofelement114flerovium AT thorlepospiechp ontheadsorptionandreactivityofelement114flerovium AT toyoshimaa ontheadsorptionandreactivityofelement114flerovium AT trautmannn ontheadsorptionandreactivityofelement114flerovium AT tsukadak ontheadsorptionandreactivityofelement114flerovium AT uusitaloj ontheadsorptionandreactivityofelement114flerovium AT vossko ontheadsorptionandreactivityofelement114flerovium AT warda ontheadsorptionandreactivityofelement114flerovium AT wegrzeckim ontheadsorptionandreactivityofelement114flerovium AT wiehln ontheadsorptionandreactivityofelement114flerovium AT williamse ontheadsorptionandreactivityofelement114flerovium AT yakushevav ontheadsorptionandreactivityofelement114flerovium |