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On the adsorption and reactivity of element 114, flerovium

Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas...

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Autores principales: Yakushev, A., Lens, L., Düllmann, Ch. E., Khuyagbaatar, J., Jäger, E., Krier, J., Runke, J., Albers, H. M., Asai, M., Block, M., Despotopulos, J., Di Nitto, A., Eberhardt, K., Forsberg, U., Golubev, P., Götz, M., Götz, S., Haba, H., Harkness-Brennan, L., Herzberg, R.-D., Heßberger, F. P., Hinde, D., Hübner, A., Judson, D., Kindler, B., Komori, Y., Konki, J., Kratz, J.V., Kurz, N., Laatiaoui, M., Lahiri, S., Lommel, B., Maiti, M., Mistry, A. K., Mokry, Ch., Moody, K. J., Nagame, Y., Omtvedt, J. P., Papadakis, P., Pershina, V., Rudolph, D., Samiento, L.G., Sato, T.K., Schädel, M., Scharrer, P., Schausten, B., Shaughnessy, D. A., Steiner, J., Thörle-Pospiech, P., Toyoshima, A., Trautmann, N., Tsukada, K., Uusitalo, J., Voss, K.-O., Ward, A., Wegrzecki, M., Wiehl, N., Williams, E., Yakusheva, V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9453156/
https://www.ncbi.nlm.nih.gov/pubmed/36092655
http://dx.doi.org/10.3389/fchem.2022.976635
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author Yakushev, A.
Lens, L.
Düllmann, Ch. E.
Khuyagbaatar, J.
Jäger, E.
Krier, J.
Runke, J.
Albers, H. M.
Asai, M.
Block, M.
Despotopulos, J.
Di Nitto, A.
Eberhardt, K.
Forsberg, U.
Golubev, P.
Götz, M.
Götz, S.
Haba, H.
Harkness-Brennan, L.
Herzberg, R.-D.
Heßberger, F. P.
Hinde, D.
Hübner, A.
Judson, D.
Kindler, B.
Komori, Y.
Konki, J.
Kratz, J.V.
Kurz, N.
Laatiaoui, M.
Lahiri, S.
Lommel, B.
Maiti, M.
Mistry, A. K.
Mokry, Ch.
Moody, K. J.
Nagame, Y.
Omtvedt, J. P.
Papadakis, P.
Pershina, V.
Rudolph, D.
Samiento, L.G.
Sato, T.K.
Schädel, M.
Scharrer, P.
Schausten, B.
Shaughnessy, D. A.
Steiner, J.
Thörle-Pospiech, P.
Toyoshima, A.
Trautmann, N.
Tsukada, K.
Uusitalo, J.
Voss, K.-O.
Ward, A.
Wegrzecki, M.
Wiehl, N.
Williams, E.
Yakusheva, V.
author_facet Yakushev, A.
Lens, L.
Düllmann, Ch. E.
Khuyagbaatar, J.
Jäger, E.
Krier, J.
Runke, J.
Albers, H. M.
Asai, M.
Block, M.
Despotopulos, J.
Di Nitto, A.
Eberhardt, K.
Forsberg, U.
Golubev, P.
Götz, M.
Götz, S.
Haba, H.
Harkness-Brennan, L.
Herzberg, R.-D.
Heßberger, F. P.
Hinde, D.
Hübner, A.
Judson, D.
Kindler, B.
Komori, Y.
Konki, J.
Kratz, J.V.
Kurz, N.
Laatiaoui, M.
Lahiri, S.
Lommel, B.
Maiti, M.
Mistry, A. K.
Mokry, Ch.
Moody, K. J.
Nagame, Y.
Omtvedt, J. P.
Papadakis, P.
Pershina, V.
Rudolph, D.
Samiento, L.G.
Sato, T.K.
Schädel, M.
Scharrer, P.
Schausten, B.
Shaughnessy, D. A.
Steiner, J.
Thörle-Pospiech, P.
Toyoshima, A.
Trautmann, N.
Tsukada, K.
Uusitalo, J.
Voss, K.-O.
Ward, A.
Wegrzecki, M.
Wiehl, N.
Williams, E.
Yakusheva, V.
author_sort Yakushev, A.
collection PubMed
description Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn.
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spelling pubmed-94531562022-09-09 On the adsorption and reactivity of element 114, flerovium Yakushev, A. Lens, L. Düllmann, Ch. E. Khuyagbaatar, J. Jäger, E. Krier, J. Runke, J. Albers, H. M. Asai, M. Block, M. Despotopulos, J. Di Nitto, A. Eberhardt, K. Forsberg, U. Golubev, P. Götz, M. Götz, S. Haba, H. Harkness-Brennan, L. Herzberg, R.-D. Heßberger, F. P. Hinde, D. Hübner, A. Judson, D. Kindler, B. Komori, Y. Konki, J. Kratz, J.V. Kurz, N. Laatiaoui, M. Lahiri, S. Lommel, B. Maiti, M. Mistry, A. K. Mokry, Ch. Moody, K. J. Nagame, Y. Omtvedt, J. P. Papadakis, P. Pershina, V. Rudolph, D. Samiento, L.G. Sato, T.K. Schädel, M. Scharrer, P. Schausten, B. Shaughnessy, D. A. Steiner, J. Thörle-Pospiech, P. Toyoshima, A. Trautmann, N. Tsukada, K. Uusitalo, J. Voss, K.-O. Ward, A. Wegrzecki, M. Wiehl, N. Williams, E. Yakusheva, V. Front Chem Chemistry Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn. Frontiers Media S.A. 2022-08-25 /pmc/articles/PMC9453156/ /pubmed/36092655 http://dx.doi.org/10.3389/fchem.2022.976635 Text en Copyright © 2022 Yakushev, Lens, Düllmann, Khuyagbaatar, Jäger, Krier, Runke, Albers, Asai, Block, Despotopulos, Di Nitto, Eberhardt, Forsberg, Golubev, Götz, Götz, Haba, Harkness-Brennan, Herzberg, Heßberger, Hinde, Hübner, Judson, Kindler, Komori, Konki, Kratz, Kurz, Laatiaoui, Lahiri, Lommel, Maiti, Mistry, Mokry, Moody, Nagame, Omtvedt, Papadakis, Pershina, Rudolph, Samiento, Sato, Schädel, Scharrer, Schausten, Shaughnessy, Steiner, Thörle-Pospiech, Toyoshima, Trautmann, Tsukada, Uusitalo, Voss, Ward, Wegrzecki, Wiehl, Williams and Yakusheva. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Yakushev, A.
Lens, L.
Düllmann, Ch. E.
Khuyagbaatar, J.
Jäger, E.
Krier, J.
Runke, J.
Albers, H. M.
Asai, M.
Block, M.
Despotopulos, J.
Di Nitto, A.
Eberhardt, K.
Forsberg, U.
Golubev, P.
Götz, M.
Götz, S.
Haba, H.
Harkness-Brennan, L.
Herzberg, R.-D.
Heßberger, F. P.
Hinde, D.
Hübner, A.
Judson, D.
Kindler, B.
Komori, Y.
Konki, J.
Kratz, J.V.
Kurz, N.
Laatiaoui, M.
Lahiri, S.
Lommel, B.
Maiti, M.
Mistry, A. K.
Mokry, Ch.
Moody, K. J.
Nagame, Y.
Omtvedt, J. P.
Papadakis, P.
Pershina, V.
Rudolph, D.
Samiento, L.G.
Sato, T.K.
Schädel, M.
Scharrer, P.
Schausten, B.
Shaughnessy, D. A.
Steiner, J.
Thörle-Pospiech, P.
Toyoshima, A.
Trautmann, N.
Tsukada, K.
Uusitalo, J.
Voss, K.-O.
Ward, A.
Wegrzecki, M.
Wiehl, N.
Williams, E.
Yakusheva, V.
On the adsorption and reactivity of element 114, flerovium
title On the adsorption and reactivity of element 114, flerovium
title_full On the adsorption and reactivity of element 114, flerovium
title_fullStr On the adsorption and reactivity of element 114, flerovium
title_full_unstemmed On the adsorption and reactivity of element 114, flerovium
title_short On the adsorption and reactivity of element 114, flerovium
title_sort on the adsorption and reactivity of element 114, flerovium
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9453156/
https://www.ncbi.nlm.nih.gov/pubmed/36092655
http://dx.doi.org/10.3389/fchem.2022.976635
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