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Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction

Owning to their distinctive electronic structure, rare-earth-based catalysts exhibit good performance in the oxygen reduction reaction (ORR) and can replace commercial Pt/C. In this study, CeO(2)-modified N-doped C-based materials were synthesized using salt template and high-temperature calcination...

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Autores principales: Wen, Xin, Chang, Ying, Jia, Jingchun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9457935/
https://www.ncbi.nlm.nih.gov/pubmed/36080094
http://dx.doi.org/10.3390/nano12173057
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author Wen, Xin
Chang, Ying
Jia, Jingchun
author_facet Wen, Xin
Chang, Ying
Jia, Jingchun
author_sort Wen, Xin
collection PubMed
description Owning to their distinctive electronic structure, rare-earth-based catalysts exhibit good performance in the oxygen reduction reaction (ORR) and can replace commercial Pt/C. In this study, CeO(2)-modified N-doped C-based materials were synthesized using salt template and high-temperature calcination methods, and the synthesis conditions were optimized. The successful synthesis of CeO(2)–CN–800 was confirmed through a series of characterization methods and electrochemical tests. The test results show that the material has the peak onset potential of 0.90 V and the half-wave potential of 0.84 V, and has good durability and methanol resistance. The material demonstrates good ORR catalytic performance and can be used in Zn–air batteries. Moreover, it is an excellent catalyst for new energy equipment.
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spelling pubmed-94579352022-09-09 Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction Wen, Xin Chang, Ying Jia, Jingchun Nanomaterials (Basel) Article Owning to their distinctive electronic structure, rare-earth-based catalysts exhibit good performance in the oxygen reduction reaction (ORR) and can replace commercial Pt/C. In this study, CeO(2)-modified N-doped C-based materials were synthesized using salt template and high-temperature calcination methods, and the synthesis conditions were optimized. The successful synthesis of CeO(2)–CN–800 was confirmed through a series of characterization methods and electrochemical tests. The test results show that the material has the peak onset potential of 0.90 V and the half-wave potential of 0.84 V, and has good durability and methanol resistance. The material demonstrates good ORR catalytic performance and can be used in Zn–air batteries. Moreover, it is an excellent catalyst for new energy equipment. MDPI 2022-09-02 /pmc/articles/PMC9457935/ /pubmed/36080094 http://dx.doi.org/10.3390/nano12173057 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Wen, Xin
Chang, Ying
Jia, Jingchun
Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction
title Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction
title_full Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction
title_fullStr Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction
title_full_unstemmed Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction
title_short Evaluating the Growth of Ceria-Modified N-Doped Carbon-Based Materials and Their Performance in the Oxygen Reduction Reaction
title_sort evaluating the growth of ceria-modified n-doped carbon-based materials and their performance in the oxygen reduction reaction
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9457935/
https://www.ncbi.nlm.nih.gov/pubmed/36080094
http://dx.doi.org/10.3390/nano12173057
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