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Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere

The spontaneous emission of a fluorophore is altered by the surrounding electromagnetic field. Therefore, the radiation of the fluorophore can be engineered by inter-coupling with the nanoscale plasmons. This work proposes a nanoscale hemisphere structure that enhances the electric field and further...

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Detalles Bibliográficos
Autores principales: Lv, Jiangtao, Chang, Minghui, Gu, Qiongchan, Ying, Yu, Si, Guangyuan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9459785/
https://www.ncbi.nlm.nih.gov/pubmed/36080107
http://dx.doi.org/10.3390/nano12173070
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author Lv, Jiangtao
Chang, Minghui
Gu, Qiongchan
Ying, Yu
Si, Guangyuan
author_facet Lv, Jiangtao
Chang, Minghui
Gu, Qiongchan
Ying, Yu
Si, Guangyuan
author_sort Lv, Jiangtao
collection PubMed
description The spontaneous emission of a fluorophore is altered by the surrounding electromagnetic field. Therefore, the radiation of the fluorophore can be engineered by inter-coupling with the nanoscale plasmons. This work proposes a nanoscale hemisphere structure that enhances the electric field and further modulates its effects on fluorophores by adjusting the radius of the hemisphere. A full-wave simulation is carried out using the finite element method, and the radiation characteristics of the nanoscale hemisphere are studied in detail. Compared with free space, the structure has generated significant enhancement exceeding 30. Through curve fitting, the relationship between the enhanced peak wavelength and the radius of the hemisphere is obtained.
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spelling pubmed-94597852022-09-10 Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere Lv, Jiangtao Chang, Minghui Gu, Qiongchan Ying, Yu Si, Guangyuan Nanomaterials (Basel) Article The spontaneous emission of a fluorophore is altered by the surrounding electromagnetic field. Therefore, the radiation of the fluorophore can be engineered by inter-coupling with the nanoscale plasmons. This work proposes a nanoscale hemisphere structure that enhances the electric field and further modulates its effects on fluorophores by adjusting the radius of the hemisphere. A full-wave simulation is carried out using the finite element method, and the radiation characteristics of the nanoscale hemisphere are studied in detail. Compared with free space, the structure has generated significant enhancement exceeding 30. Through curve fitting, the relationship between the enhanced peak wavelength and the radius of the hemisphere is obtained. MDPI 2022-09-03 /pmc/articles/PMC9459785/ /pubmed/36080107 http://dx.doi.org/10.3390/nano12173070 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Lv, Jiangtao
Chang, Minghui
Gu, Qiongchan
Ying, Yu
Si, Guangyuan
Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere
title Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere
title_full Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere
title_fullStr Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere
title_full_unstemmed Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere
title_short Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere
title_sort plasmon-enhanced fluorescence emission of an electric dipole modulated by a nanoscale silver hemisphere
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9459785/
https://www.ncbi.nlm.nih.gov/pubmed/36080107
http://dx.doi.org/10.3390/nano12173070
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