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Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential

Interlayer excitons (IXs) in MoSe(2)–WSe(2) heterobilayers have generated interest as highly tunable light emitters in transition metal dichalcogenide (TMD) heterostructures. Previous reports of spectrally narrow (<1 meV) photoluminescence (PL) emission lines at low temperature have been attribut...

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Autores principales: Mahdikhanysarvejahany, Fateme, Shanks, Daniel N., Klein, Matthew, Wang, Qian, Koehler, Michael R., Mandrus, David G., Taniguchi, Takashi, Watanabe, Kenji, Monti, Oliver L. A., LeRoy, Brian J., Schaibley, John R.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9468147/
https://www.ncbi.nlm.nih.gov/pubmed/36097165
http://dx.doi.org/10.1038/s41467-022-33082-6
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author Mahdikhanysarvejahany, Fateme
Shanks, Daniel N.
Klein, Matthew
Wang, Qian
Koehler, Michael R.
Mandrus, David G.
Taniguchi, Takashi
Watanabe, Kenji
Monti, Oliver L. A.
LeRoy, Brian J.
Schaibley, John R.
author_facet Mahdikhanysarvejahany, Fateme
Shanks, Daniel N.
Klein, Matthew
Wang, Qian
Koehler, Michael R.
Mandrus, David G.
Taniguchi, Takashi
Watanabe, Kenji
Monti, Oliver L. A.
LeRoy, Brian J.
Schaibley, John R.
author_sort Mahdikhanysarvejahany, Fateme
collection PubMed
description Interlayer excitons (IXs) in MoSe(2)–WSe(2) heterobilayers have generated interest as highly tunable light emitters in transition metal dichalcogenide (TMD) heterostructures. Previous reports of spectrally narrow (<1 meV) photoluminescence (PL) emission lines at low temperature have been attributed to IXs localized by the moiré potential between the TMD layers. We show that spectrally narrow IX PL lines are present even when the moiré potential is suppressed by inserting a bilayer hexagonal boron nitride (hBN) spacer between the TMD layers. We compare the doping, electric field, magnetic field, and temperature dependence of IXs in a directly contacted MoSe(2)–WSe(2) region to those in a region separated by bilayer hBN. The doping, electric field, and temperature dependence of the narrow IX lines are similar for both regions, but their excitonic g-factors have opposite signs, indicating that the origin of narrow IX PL is not the moiré potential.
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spelling pubmed-94681472022-09-14 Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential Mahdikhanysarvejahany, Fateme Shanks, Daniel N. Klein, Matthew Wang, Qian Koehler, Michael R. Mandrus, David G. Taniguchi, Takashi Watanabe, Kenji Monti, Oliver L. A. LeRoy, Brian J. Schaibley, John R. Nat Commun Article Interlayer excitons (IXs) in MoSe(2)–WSe(2) heterobilayers have generated interest as highly tunable light emitters in transition metal dichalcogenide (TMD) heterostructures. Previous reports of spectrally narrow (<1 meV) photoluminescence (PL) emission lines at low temperature have been attributed to IXs localized by the moiré potential between the TMD layers. We show that spectrally narrow IX PL lines are present even when the moiré potential is suppressed by inserting a bilayer hexagonal boron nitride (hBN) spacer between the TMD layers. We compare the doping, electric field, magnetic field, and temperature dependence of IXs in a directly contacted MoSe(2)–WSe(2) region to those in a region separated by bilayer hBN. The doping, electric field, and temperature dependence of the narrow IX lines are similar for both regions, but their excitonic g-factors have opposite signs, indicating that the origin of narrow IX PL is not the moiré potential. Nature Publishing Group UK 2022-09-12 /pmc/articles/PMC9468147/ /pubmed/36097165 http://dx.doi.org/10.1038/s41467-022-33082-6 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Mahdikhanysarvejahany, Fateme
Shanks, Daniel N.
Klein, Matthew
Wang, Qian
Koehler, Michael R.
Mandrus, David G.
Taniguchi, Takashi
Watanabe, Kenji
Monti, Oliver L. A.
LeRoy, Brian J.
Schaibley, John R.
Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential
title Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential
title_full Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential
title_fullStr Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential
title_full_unstemmed Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential
title_short Localized interlayer excitons in MoSe(2)–WSe(2) heterostructures without a moiré potential
title_sort localized interlayer excitons in mose(2)–wse(2) heterostructures without a moiré potential
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9468147/
https://www.ncbi.nlm.nih.gov/pubmed/36097165
http://dx.doi.org/10.1038/s41467-022-33082-6
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