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Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride

Emergent color centers with accessible spins hosted by van der Waals materials have attracted substantial interest in recent years due to their significant potential for implementing transformative quantum sensing technologies. Hexagonal boron nitride (hBN) is naturally relevant in this context due...

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Autores principales: Huang, Mengqi, Zhou, Jingcheng, Chen, Di, Lu, Hanyi, McLaughlin, Nathan J., Li, Senlei, Alghamdi, Mohammed, Djugba, Dziga, Shi, Jing, Wang, Hailong, Du, Chunhui Rita
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9470674/
https://www.ncbi.nlm.nih.gov/pubmed/36100604
http://dx.doi.org/10.1038/s41467-022-33016-2
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author Huang, Mengqi
Zhou, Jingcheng
Chen, Di
Lu, Hanyi
McLaughlin, Nathan J.
Li, Senlei
Alghamdi, Mohammed
Djugba, Dziga
Shi, Jing
Wang, Hailong
Du, Chunhui Rita
author_facet Huang, Mengqi
Zhou, Jingcheng
Chen, Di
Lu, Hanyi
McLaughlin, Nathan J.
Li, Senlei
Alghamdi, Mohammed
Djugba, Dziga
Shi, Jing
Wang, Hailong
Du, Chunhui Rita
author_sort Huang, Mengqi
collection PubMed
description Emergent color centers with accessible spins hosted by van der Waals materials have attracted substantial interest in recent years due to their significant potential for implementing transformative quantum sensing technologies. Hexagonal boron nitride (hBN) is naturally relevant in this context due to its remarkable ease of integration into devices consisting of low-dimensional materials. Taking advantage of boron vacancy spin defects in hBN, we report nanoscale quantum imaging of low-dimensional ferromagnetism sustained in Fe(3)GeTe(2)/hBN van der Waals heterostructures. Exploiting spin relaxometry methods, we have further observed spatially varying magnetic fluctuations in the exfoliated Fe(3)GeTe(2) flake, whose magnitude reaches a peak value around the Curie temperature. Our results demonstrate the capability of spin defects in hBN of investigating local magnetic properties of layered materials in an accessible and precise way, which can be extended readily to a broad range of miniaturized van der Waals heterostructure systems.
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spelling pubmed-94706742022-09-15 Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride Huang, Mengqi Zhou, Jingcheng Chen, Di Lu, Hanyi McLaughlin, Nathan J. Li, Senlei Alghamdi, Mohammed Djugba, Dziga Shi, Jing Wang, Hailong Du, Chunhui Rita Nat Commun Article Emergent color centers with accessible spins hosted by van der Waals materials have attracted substantial interest in recent years due to their significant potential for implementing transformative quantum sensing technologies. Hexagonal boron nitride (hBN) is naturally relevant in this context due to its remarkable ease of integration into devices consisting of low-dimensional materials. Taking advantage of boron vacancy spin defects in hBN, we report nanoscale quantum imaging of low-dimensional ferromagnetism sustained in Fe(3)GeTe(2)/hBN van der Waals heterostructures. Exploiting spin relaxometry methods, we have further observed spatially varying magnetic fluctuations in the exfoliated Fe(3)GeTe(2) flake, whose magnitude reaches a peak value around the Curie temperature. Our results demonstrate the capability of spin defects in hBN of investigating local magnetic properties of layered materials in an accessible and precise way, which can be extended readily to a broad range of miniaturized van der Waals heterostructure systems. Nature Publishing Group UK 2022-09-13 /pmc/articles/PMC9470674/ /pubmed/36100604 http://dx.doi.org/10.1038/s41467-022-33016-2 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Huang, Mengqi
Zhou, Jingcheng
Chen, Di
Lu, Hanyi
McLaughlin, Nathan J.
Li, Senlei
Alghamdi, Mohammed
Djugba, Dziga
Shi, Jing
Wang, Hailong
Du, Chunhui Rita
Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride
title Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride
title_full Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride
title_fullStr Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride
title_full_unstemmed Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride
title_short Wide field imaging of van der Waals ferromagnet Fe(3)GeTe(2) by spin defects in hexagonal boron nitride
title_sort wide field imaging of van der waals ferromagnet fe(3)gete(2) by spin defects in hexagonal boron nitride
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9470674/
https://www.ncbi.nlm.nih.gov/pubmed/36100604
http://dx.doi.org/10.1038/s41467-022-33016-2
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