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Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appeari...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9474864/ https://www.ncbi.nlm.nih.gov/pubmed/36104375 http://dx.doi.org/10.1038/s41467-022-33103-4 |
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author | Morita, Yusuke Yoshioka, Kosuke Kuwata-Gonokami, Makoto |
author_facet | Morita, Yusuke Yoshioka, Kosuke Kuwata-Gonokami, Makoto |
author_sort | Morita, Yusuke |
collection | PubMed |
description | An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appearing in a trapped gas of 1s paraexcitons in bulk Cu(2)O below 400 mK, by directly visualizing the exciton cloud in real space using mid-infrared induced absorption imaging that we realized in a dilution refrigerator. Our study shows that the paraexciton condensate is undetectable by conventional luminescence spectroscopy. We find an unconventionally small condensate fraction of 0.016 with the spatial profile of the condensate well described by mean-field theory. Our discovery of this new type of BEC in the purely matter-like exciton system interacting with a cold phonon bath could pave the way for the classification of its long-range order, and for essential understanding of quantum statistical mechanics of non-equilibrium open systems. |
format | Online Article Text |
id | pubmed-9474864 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-94748642022-09-16 Observation of Bose-Einstein condensates of excitons in a bulk semiconductor Morita, Yusuke Yoshioka, Kosuke Kuwata-Gonokami, Makoto Nat Commun Article An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appearing in a trapped gas of 1s paraexcitons in bulk Cu(2)O below 400 mK, by directly visualizing the exciton cloud in real space using mid-infrared induced absorption imaging that we realized in a dilution refrigerator. Our study shows that the paraexciton condensate is undetectable by conventional luminescence spectroscopy. We find an unconventionally small condensate fraction of 0.016 with the spatial profile of the condensate well described by mean-field theory. Our discovery of this new type of BEC in the purely matter-like exciton system interacting with a cold phonon bath could pave the way for the classification of its long-range order, and for essential understanding of quantum statistical mechanics of non-equilibrium open systems. Nature Publishing Group UK 2022-09-14 /pmc/articles/PMC9474864/ /pubmed/36104375 http://dx.doi.org/10.1038/s41467-022-33103-4 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Morita, Yusuke Yoshioka, Kosuke Kuwata-Gonokami, Makoto Observation of Bose-Einstein condensates of excitons in a bulk semiconductor |
title | Observation of Bose-Einstein condensates of excitons in a bulk semiconductor |
title_full | Observation of Bose-Einstein condensates of excitons in a bulk semiconductor |
title_fullStr | Observation of Bose-Einstein condensates of excitons in a bulk semiconductor |
title_full_unstemmed | Observation of Bose-Einstein condensates of excitons in a bulk semiconductor |
title_short | Observation of Bose-Einstein condensates of excitons in a bulk semiconductor |
title_sort | observation of bose-einstein condensates of excitons in a bulk semiconductor |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9474864/ https://www.ncbi.nlm.nih.gov/pubmed/36104375 http://dx.doi.org/10.1038/s41467-022-33103-4 |
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