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Observation of Bose-Einstein condensates of excitons in a bulk semiconductor

An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appeari...

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Autores principales: Morita, Yusuke, Yoshioka, Kosuke, Kuwata-Gonokami, Makoto
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9474864/
https://www.ncbi.nlm.nih.gov/pubmed/36104375
http://dx.doi.org/10.1038/s41467-022-33103-4
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author Morita, Yusuke
Yoshioka, Kosuke
Kuwata-Gonokami, Makoto
author_facet Morita, Yusuke
Yoshioka, Kosuke
Kuwata-Gonokami, Makoto
author_sort Morita, Yusuke
collection PubMed
description An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appearing in a trapped gas of 1s paraexcitons in bulk Cu(2)O below 400 mK, by directly visualizing the exciton cloud in real space using mid-infrared induced absorption imaging that we realized in a dilution refrigerator. Our study shows that the paraexciton condensate is undetectable by conventional luminescence spectroscopy. We find an unconventionally small condensate fraction of 0.016 with the spatial profile of the condensate well described by mean-field theory. Our discovery of this new type of BEC in the purely matter-like exciton system interacting with a cold phonon bath could pave the way for the classification of its long-range order, and for essential understanding of quantum statistical mechanics of non-equilibrium open systems.
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spelling pubmed-94748642022-09-16 Observation of Bose-Einstein condensates of excitons in a bulk semiconductor Morita, Yusuke Yoshioka, Kosuke Kuwata-Gonokami, Makoto Nat Commun Article An unambiguous observation of the Bose-Einstein condensation (BEC) of excitons in a photoexcited bulk semiconductor and elucidation of its inherent nature have been longstanding problems in condensed matter physics. Here, we observe the quantum phase transition and a Bose-Einstein condensate appearing in a trapped gas of 1s paraexcitons in bulk Cu(2)O below 400 mK, by directly visualizing the exciton cloud in real space using mid-infrared induced absorption imaging that we realized in a dilution refrigerator. Our study shows that the paraexciton condensate is undetectable by conventional luminescence spectroscopy. We find an unconventionally small condensate fraction of 0.016 with the spatial profile of the condensate well described by mean-field theory. Our discovery of this new type of BEC in the purely matter-like exciton system interacting with a cold phonon bath could pave the way for the classification of its long-range order, and for essential understanding of quantum statistical mechanics of non-equilibrium open systems. Nature Publishing Group UK 2022-09-14 /pmc/articles/PMC9474864/ /pubmed/36104375 http://dx.doi.org/10.1038/s41467-022-33103-4 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Morita, Yusuke
Yoshioka, Kosuke
Kuwata-Gonokami, Makoto
Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
title Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
title_full Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
title_fullStr Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
title_full_unstemmed Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
title_short Observation of Bose-Einstein condensates of excitons in a bulk semiconductor
title_sort observation of bose-einstein condensates of excitons in a bulk semiconductor
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9474864/
https://www.ncbi.nlm.nih.gov/pubmed/36104375
http://dx.doi.org/10.1038/s41467-022-33103-4
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