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Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector

Influence on photocurrent sensitivity of hydrothermally synthesized electrochemically active graphene quantum dots on conjugated polymer utilized for a novel single-layer device has been performed. Fabrications of high-performance ultraviolet photodetector by depositing the polypyrrole-graphene quan...

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Autores principales: Vandana, Molahalli, Devendrappa, Hundekal, Padova, Paola De, Hegde, Gurumurthy
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9502816/
https://www.ncbi.nlm.nih.gov/pubmed/36144964
http://dx.doi.org/10.3390/nano12183175
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author Vandana, Molahalli
Devendrappa, Hundekal
Padova, Paola De
Hegde, Gurumurthy
author_facet Vandana, Molahalli
Devendrappa, Hundekal
Padova, Paola De
Hegde, Gurumurthy
author_sort Vandana, Molahalli
collection PubMed
description Influence on photocurrent sensitivity of hydrothermally synthesized electrochemically active graphene quantum dots on conjugated polymer utilized for a novel single-layer device has been performed. Fabrications of high-performance ultraviolet photodetector by depositing the polypyrrole-graphene quantum dots (PPy-GQDs) active layer of the ITO electrode were exposed to an Ultraviolet (UV) source with 265 and 355 nm wavelengths for about 200 s, and we examined the time-dependent photoresponse. The excellent performance of GQDs was exploited as a light absorber, acting as an electron donor to improve the carrier concentration. PGC4 exhibits high photoresponsivity up to the 2.33 µA/W at 6 V bias and the photocurrent changes from 2.9 to 18 µA. The electrochemical measurement was studied using an electrochemical workstation. The cyclic voltammetry (CV) results show that the hysteresis loop is optically tunable with a UV light source with 265 and 355 nm at 0.1 to 0.5 V/s. The photocurrent response in PPy-GQDs devices may be applicable to optoelectronics devices.
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spelling pubmed-95028162022-09-24 Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector Vandana, Molahalli Devendrappa, Hundekal Padova, Paola De Hegde, Gurumurthy Nanomaterials (Basel) Article Influence on photocurrent sensitivity of hydrothermally synthesized electrochemically active graphene quantum dots on conjugated polymer utilized for a novel single-layer device has been performed. Fabrications of high-performance ultraviolet photodetector by depositing the polypyrrole-graphene quantum dots (PPy-GQDs) active layer of the ITO electrode were exposed to an Ultraviolet (UV) source with 265 and 355 nm wavelengths for about 200 s, and we examined the time-dependent photoresponse. The excellent performance of GQDs was exploited as a light absorber, acting as an electron donor to improve the carrier concentration. PGC4 exhibits high photoresponsivity up to the 2.33 µA/W at 6 V bias and the photocurrent changes from 2.9 to 18 µA. The electrochemical measurement was studied using an electrochemical workstation. The cyclic voltammetry (CV) results show that the hysteresis loop is optically tunable with a UV light source with 265 and 355 nm at 0.1 to 0.5 V/s. The photocurrent response in PPy-GQDs devices may be applicable to optoelectronics devices. MDPI 2022-09-13 /pmc/articles/PMC9502816/ /pubmed/36144964 http://dx.doi.org/10.3390/nano12183175 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Vandana, Molahalli
Devendrappa, Hundekal
Padova, Paola De
Hegde, Gurumurthy
Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector
title Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector
title_full Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector
title_fullStr Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector
title_full_unstemmed Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector
title_short Polymer Nanocomposite Graphene Quantum Dots for High-Efficiency Ultraviolet Photodetector
title_sort polymer nanocomposite graphene quantum dots for high-efficiency ultraviolet photodetector
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9502816/
https://www.ncbi.nlm.nih.gov/pubmed/36144964
http://dx.doi.org/10.3390/nano12183175
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