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Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
The artificial photocatalytic degradation of organic pollutants has emerged as a promising approach to purifying the water environment. The core issue of this ongoing research is to construct efficient but easily recyclable photocatalysts without quadratic harm. Here, we report an eco-friendly photo...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9504825/ https://www.ncbi.nlm.nih.gov/pubmed/36144916 http://dx.doi.org/10.3390/nano12183130 |
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author | Shen, Hancheng Zhang, Weiwei Guo, Chunyun Zhu, Jing Cui, Junjie Xue, Zhonghua Chen, Peirong |
author_facet | Shen, Hancheng Zhang, Weiwei Guo, Chunyun Zhu, Jing Cui, Junjie Xue, Zhonghua Chen, Peirong |
author_sort | Shen, Hancheng |
collection | PubMed |
description | The artificial photocatalytic degradation of organic pollutants has emerged as a promising approach to purifying the water environment. The core issue of this ongoing research is to construct efficient but easily recyclable photocatalysts without quadratic harm. Here, we report an eco-friendly photocatalyst with in situ generated TiO(2) quantum dots (TQDs) on natural cotton cellulose (CC) by a simple one-step hydrothermal method. The porous fine structure and abundant hydroxyl groups control the shape growth and improve the stability of nanoparticles, making natural CC suitable for TQDs. The TQDs/CC photocatalyst was synthesized without the chemical modification of the TQDs. FE-SEM and TEM results showed that 5–6 nm TQDs are uniformly decorated on the CC surface. The long-term stability in photocatalytic activity and structure of more than ten cycles directly demonstrates the stability of CC on TQDs. With larger CC sizes, TQDs are easier to recycle. The TQDs/CC photocatalysts show impressive potential in the photocatalytic degradation of anionic methyl orange (MO) dyes and cationic rhodamine B (RhB) dyes. |
format | Online Article Text |
id | pubmed-9504825 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-95048252022-09-24 Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes Shen, Hancheng Zhang, Weiwei Guo, Chunyun Zhu, Jing Cui, Junjie Xue, Zhonghua Chen, Peirong Nanomaterials (Basel) Article The artificial photocatalytic degradation of organic pollutants has emerged as a promising approach to purifying the water environment. The core issue of this ongoing research is to construct efficient but easily recyclable photocatalysts without quadratic harm. Here, we report an eco-friendly photocatalyst with in situ generated TiO(2) quantum dots (TQDs) on natural cotton cellulose (CC) by a simple one-step hydrothermal method. The porous fine structure and abundant hydroxyl groups control the shape growth and improve the stability of nanoparticles, making natural CC suitable for TQDs. The TQDs/CC photocatalyst was synthesized without the chemical modification of the TQDs. FE-SEM and TEM results showed that 5–6 nm TQDs are uniformly decorated on the CC surface. The long-term stability in photocatalytic activity and structure of more than ten cycles directly demonstrates the stability of CC on TQDs. With larger CC sizes, TQDs are easier to recycle. The TQDs/CC photocatalysts show impressive potential in the photocatalytic degradation of anionic methyl orange (MO) dyes and cationic rhodamine B (RhB) dyes. MDPI 2022-09-09 /pmc/articles/PMC9504825/ /pubmed/36144916 http://dx.doi.org/10.3390/nano12183130 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Shen, Hancheng Zhang, Weiwei Guo, Chunyun Zhu, Jing Cui, Junjie Xue, Zhonghua Chen, Peirong Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes |
title | Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes |
title_full | Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes |
title_fullStr | Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes |
title_full_unstemmed | Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes |
title_short | Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes |
title_sort | natural cotton cellulose-supported tio(2) quantum dots for the highly efficient photocatalytic degradation of dyes |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9504825/ https://www.ncbi.nlm.nih.gov/pubmed/36144916 http://dx.doi.org/10.3390/nano12183130 |
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