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Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes

The artificial photocatalytic degradation of organic pollutants has emerged as a promising approach to purifying the water environment. The core issue of this ongoing research is to construct efficient but easily recyclable photocatalysts without quadratic harm. Here, we report an eco-friendly photo...

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Autores principales: Shen, Hancheng, Zhang, Weiwei, Guo, Chunyun, Zhu, Jing, Cui, Junjie, Xue, Zhonghua, Chen, Peirong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9504825/
https://www.ncbi.nlm.nih.gov/pubmed/36144916
http://dx.doi.org/10.3390/nano12183130
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author Shen, Hancheng
Zhang, Weiwei
Guo, Chunyun
Zhu, Jing
Cui, Junjie
Xue, Zhonghua
Chen, Peirong
author_facet Shen, Hancheng
Zhang, Weiwei
Guo, Chunyun
Zhu, Jing
Cui, Junjie
Xue, Zhonghua
Chen, Peirong
author_sort Shen, Hancheng
collection PubMed
description The artificial photocatalytic degradation of organic pollutants has emerged as a promising approach to purifying the water environment. The core issue of this ongoing research is to construct efficient but easily recyclable photocatalysts without quadratic harm. Here, we report an eco-friendly photocatalyst with in situ generated TiO(2) quantum dots (TQDs) on natural cotton cellulose (CC) by a simple one-step hydrothermal method. The porous fine structure and abundant hydroxyl groups control the shape growth and improve the stability of nanoparticles, making natural CC suitable for TQDs. The TQDs/CC photocatalyst was synthesized without the chemical modification of the TQDs. FE-SEM and TEM results showed that 5–6 nm TQDs are uniformly decorated on the CC surface. The long-term stability in photocatalytic activity and structure of more than ten cycles directly demonstrates the stability of CC on TQDs. With larger CC sizes, TQDs are easier to recycle. The TQDs/CC photocatalysts show impressive potential in the photocatalytic degradation of anionic methyl orange (MO) dyes and cationic rhodamine B (RhB) dyes.
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spelling pubmed-95048252022-09-24 Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes Shen, Hancheng Zhang, Weiwei Guo, Chunyun Zhu, Jing Cui, Junjie Xue, Zhonghua Chen, Peirong Nanomaterials (Basel) Article The artificial photocatalytic degradation of organic pollutants has emerged as a promising approach to purifying the water environment. The core issue of this ongoing research is to construct efficient but easily recyclable photocatalysts without quadratic harm. Here, we report an eco-friendly photocatalyst with in situ generated TiO(2) quantum dots (TQDs) on natural cotton cellulose (CC) by a simple one-step hydrothermal method. The porous fine structure and abundant hydroxyl groups control the shape growth and improve the stability of nanoparticles, making natural CC suitable for TQDs. The TQDs/CC photocatalyst was synthesized without the chemical modification of the TQDs. FE-SEM and TEM results showed that 5–6 nm TQDs are uniformly decorated on the CC surface. The long-term stability in photocatalytic activity and structure of more than ten cycles directly demonstrates the stability of CC on TQDs. With larger CC sizes, TQDs are easier to recycle. The TQDs/CC photocatalysts show impressive potential in the photocatalytic degradation of anionic methyl orange (MO) dyes and cationic rhodamine B (RhB) dyes. MDPI 2022-09-09 /pmc/articles/PMC9504825/ /pubmed/36144916 http://dx.doi.org/10.3390/nano12183130 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Shen, Hancheng
Zhang, Weiwei
Guo, Chunyun
Zhu, Jing
Cui, Junjie
Xue, Zhonghua
Chen, Peirong
Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
title Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
title_full Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
title_fullStr Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
title_full_unstemmed Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
title_short Natural Cotton Cellulose-Supported TiO(2) Quantum Dots for the Highly Efficient Photocatalytic Degradation of Dyes
title_sort natural cotton cellulose-supported tio(2) quantum dots for the highly efficient photocatalytic degradation of dyes
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9504825/
https://www.ncbi.nlm.nih.gov/pubmed/36144916
http://dx.doi.org/10.3390/nano12183130
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