Cargando…

Continuously processing waste lignin into high-value carbon nanotube fibers

High value utilization of renewable biomass materials is of great significance to the sustainable development of human beings. For example, because biomass contains large amounts of carbon, they are ideal candidates for the preparation of carbon nanotube fibers. However, continuous preparation of su...

Descripción completa

Detalles Bibliográficos
Autores principales: Liu, Fuyao, Wang, Qianqian, Zhai, Gongxun, Xiang, Hengxue, Zhou, Jialiang, Jia, Chao, Zhu, Liping, Wu, Qilin, Zhu, Meifang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9525656/
https://www.ncbi.nlm.nih.gov/pubmed/36180457
http://dx.doi.org/10.1038/s41467-022-33496-2
_version_ 1784800728717459456
author Liu, Fuyao
Wang, Qianqian
Zhai, Gongxun
Xiang, Hengxue
Zhou, Jialiang
Jia, Chao
Zhu, Liping
Wu, Qilin
Zhu, Meifang
author_facet Liu, Fuyao
Wang, Qianqian
Zhai, Gongxun
Xiang, Hengxue
Zhou, Jialiang
Jia, Chao
Zhu, Liping
Wu, Qilin
Zhu, Meifang
author_sort Liu, Fuyao
collection PubMed
description High value utilization of renewable biomass materials is of great significance to the sustainable development of human beings. For example, because biomass contains large amounts of carbon, they are ideal candidates for the preparation of carbon nanotube fibers. However, continuous preparation of such fibers using biomass as carbon source remains a huge challenge due to the complex chemical structure of the precursors. Here, we realize continuous preparation of high-performance carbon nanotube fibers from lignin by solvent dispersion, high-temperature pyrolysis, catalytic synthesis, and assembly. The fibers exhibit a tensile strength of 1.33 GPa and an electrical conductivity of 1.19 × 10(5 )S m(−1), superior to that of most biomass-derived carbon materials to date. More importantly, we achieve continuous production rate of 120 m h(−1). Our preparation method is extendable to other biomass materials and will greatly promote the high value application of biomass in a wide range of fields.
format Online
Article
Text
id pubmed-9525656
institution National Center for Biotechnology Information
language English
publishDate 2022
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-95256562022-10-02 Continuously processing waste lignin into high-value carbon nanotube fibers Liu, Fuyao Wang, Qianqian Zhai, Gongxun Xiang, Hengxue Zhou, Jialiang Jia, Chao Zhu, Liping Wu, Qilin Zhu, Meifang Nat Commun Article High value utilization of renewable biomass materials is of great significance to the sustainable development of human beings. For example, because biomass contains large amounts of carbon, they are ideal candidates for the preparation of carbon nanotube fibers. However, continuous preparation of such fibers using biomass as carbon source remains a huge challenge due to the complex chemical structure of the precursors. Here, we realize continuous preparation of high-performance carbon nanotube fibers from lignin by solvent dispersion, high-temperature pyrolysis, catalytic synthesis, and assembly. The fibers exhibit a tensile strength of 1.33 GPa and an electrical conductivity of 1.19 × 10(5 )S m(−1), superior to that of most biomass-derived carbon materials to date. More importantly, we achieve continuous production rate of 120 m h(−1). Our preparation method is extendable to other biomass materials and will greatly promote the high value application of biomass in a wide range of fields. Nature Publishing Group UK 2022-09-30 /pmc/articles/PMC9525656/ /pubmed/36180457 http://dx.doi.org/10.1038/s41467-022-33496-2 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Liu, Fuyao
Wang, Qianqian
Zhai, Gongxun
Xiang, Hengxue
Zhou, Jialiang
Jia, Chao
Zhu, Liping
Wu, Qilin
Zhu, Meifang
Continuously processing waste lignin into high-value carbon nanotube fibers
title Continuously processing waste lignin into high-value carbon nanotube fibers
title_full Continuously processing waste lignin into high-value carbon nanotube fibers
title_fullStr Continuously processing waste lignin into high-value carbon nanotube fibers
title_full_unstemmed Continuously processing waste lignin into high-value carbon nanotube fibers
title_short Continuously processing waste lignin into high-value carbon nanotube fibers
title_sort continuously processing waste lignin into high-value carbon nanotube fibers
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9525656/
https://www.ncbi.nlm.nih.gov/pubmed/36180457
http://dx.doi.org/10.1038/s41467-022-33496-2
work_keys_str_mv AT liufuyao continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT wangqianqian continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT zhaigongxun continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT xianghengxue continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT zhoujialiang continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT jiachao continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT zhuliping continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT wuqilin continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers
AT zhumeifang continuouslyprocessingwasteligninintohighvaluecarbonnanotubefibers