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A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons

[Image: see text] Long-lived indirect excitons (IXs) exhibit a rich phase diagram, including a Bose–Einstein condensate (BEC), a Wigner crystal, and other exotic phases. Recent experiments have hinted at a “classical” liquid of IXs above the BEC transition. To uncover the nature of this phase, we us...

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Autores principales: Wrona, Paul R., Rabani, Eran, Geissler, Phillip L.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9527805/
https://www.ncbi.nlm.nih.gov/pubmed/36069715
http://dx.doi.org/10.1021/acsnano.2c06947
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author Wrona, Paul R.
Rabani, Eran
Geissler, Phillip L.
author_facet Wrona, Paul R.
Rabani, Eran
Geissler, Phillip L.
author_sort Wrona, Paul R.
collection PubMed
description [Image: see text] Long-lived indirect excitons (IXs) exhibit a rich phase diagram, including a Bose–Einstein condensate (BEC), a Wigner crystal, and other exotic phases. Recent experiments have hinted at a “classical” liquid of IXs above the BEC transition. To uncover the nature of this phase, we use a broad range of theoretical tools and find no evidence of a driving force toward classical condensation. Instead, we attribute the condensed phase to a quantum electron–hole liquid (EHL), first proposed by Keldysh for direct excitons. Taking into account the association of free carriers into bound excitons, we study the phase equilibrium between a gas of excitons, a gas of free carriers, and an EHL for a wide range of electron–hole separations, temperatures, densities, and mass ratios. Our results agree reasonably well with recent measurements of GaAs/AlGaAs coupled quantum wells.
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spelling pubmed-95278052022-10-04 A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons Wrona, Paul R. Rabani, Eran Geissler, Phillip L. ACS Nano [Image: see text] Long-lived indirect excitons (IXs) exhibit a rich phase diagram, including a Bose–Einstein condensate (BEC), a Wigner crystal, and other exotic phases. Recent experiments have hinted at a “classical” liquid of IXs above the BEC transition. To uncover the nature of this phase, we use a broad range of theoretical tools and find no evidence of a driving force toward classical condensation. Instead, we attribute the condensed phase to a quantum electron–hole liquid (EHL), first proposed by Keldysh for direct excitons. Taking into account the association of free carriers into bound excitons, we study the phase equilibrium between a gas of excitons, a gas of free carriers, and an EHL for a wide range of electron–hole separations, temperatures, densities, and mass ratios. Our results agree reasonably well with recent measurements of GaAs/AlGaAs coupled quantum wells. American Chemical Society 2022-09-07 2022-09-27 /pmc/articles/PMC9527805/ /pubmed/36069715 http://dx.doi.org/10.1021/acsnano.2c06947 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Wrona, Paul R.
Rabani, Eran
Geissler, Phillip L.
A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons
title A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons
title_full A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons
title_fullStr A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons
title_full_unstemmed A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons
title_short A Pair of 2D Quantum Liquids: Investigating the Phase Behavior of Indirect Excitons
title_sort pair of 2d quantum liquids: investigating the phase behavior of indirect excitons
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9527805/
https://www.ncbi.nlm.nih.gov/pubmed/36069715
http://dx.doi.org/10.1021/acsnano.2c06947
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