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Tropopause‐Level NO(x) in the Asian Summer Monsoon
Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO(2), NO, and NO(x) in the UTLS ASM anticyclone from satellite measurements. Observations of NO(2) from the Optic...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
John Wiley and Sons Inc.
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9539711/ https://www.ncbi.nlm.nih.gov/pubmed/36246737 http://dx.doi.org/10.1029/2022GL099848 |
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author | Dubé, Kimberlee Randel, William Bourassa, Adam Degenstein, Doug |
author_facet | Dubé, Kimberlee Randel, William Bourassa, Adam Degenstein, Doug |
author_sort | Dubé, Kimberlee |
collection | PubMed |
description | Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO(2), NO, and NO(x) in the UTLS ASM anticyclone from satellite measurements. Observations of NO(2) from the Optical Spectrograph and InfraRed Imager System, the Atmospheric Chemistry Experiment ‐ Fourier Transform Spectrometer (ACE‐FTS), and the Stratospheric Aerosol and Gas Experiment III on the International Space Station are considered. The PRATMO photochemical box model is used to quantify the NO(x) photochemistry, and to derive the NO(x) concentration using OSIRIS NO(2) and O(3) observations. The satellite data show a relative minimum in NO(2) over the ASM in the summer months, while the corresponding NO and NO(x) anomalies are elevated, mainly due to low O(3) and cold temperatures within the ASM. The observations within the ASM show reasonable agreement to simulations from the Whole Atmosphere Community Climate Model. |
format | Online Article Text |
id | pubmed-9539711 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | John Wiley and Sons Inc. |
record_format | MEDLINE/PubMed |
spelling | pubmed-95397112022-10-14 Tropopause‐Level NO(x) in the Asian Summer Monsoon Dubé, Kimberlee Randel, William Bourassa, Adam Degenstein, Doug Geophys Res Lett Research Letter Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO(2), NO, and NO(x) in the UTLS ASM anticyclone from satellite measurements. Observations of NO(2) from the Optical Spectrograph and InfraRed Imager System, the Atmospheric Chemistry Experiment ‐ Fourier Transform Spectrometer (ACE‐FTS), and the Stratospheric Aerosol and Gas Experiment III on the International Space Station are considered. The PRATMO photochemical box model is used to quantify the NO(x) photochemistry, and to derive the NO(x) concentration using OSIRIS NO(2) and O(3) observations. The satellite data show a relative minimum in NO(2) over the ASM in the summer months, while the corresponding NO and NO(x) anomalies are elevated, mainly due to low O(3) and cold temperatures within the ASM. The observations within the ASM show reasonable agreement to simulations from the Whole Atmosphere Community Climate Model. John Wiley and Sons Inc. 2022-09-14 2022-09-28 /pmc/articles/PMC9539711/ /pubmed/36246737 http://dx.doi.org/10.1029/2022GL099848 Text en © 2022 The Authors. https://creativecommons.org/licenses/by-nc/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc/4.0/ (https://creativecommons.org/licenses/by-nc/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes. |
spellingShingle | Research Letter Dubé, Kimberlee Randel, William Bourassa, Adam Degenstein, Doug Tropopause‐Level NO(x) in the Asian Summer Monsoon |
title | Tropopause‐Level NO(x) in the Asian Summer Monsoon |
title_full | Tropopause‐Level NO(x) in the Asian Summer Monsoon |
title_fullStr | Tropopause‐Level NO(x) in the Asian Summer Monsoon |
title_full_unstemmed | Tropopause‐Level NO(x) in the Asian Summer Monsoon |
title_short | Tropopause‐Level NO(x) in the Asian Summer Monsoon |
title_sort | tropopause‐level no(x) in the asian summer monsoon |
topic | Research Letter |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9539711/ https://www.ncbi.nlm.nih.gov/pubmed/36246737 http://dx.doi.org/10.1029/2022GL099848 |
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