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Tropopause‐Level NO(x) in the Asian Summer Monsoon

Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO(2), NO, and NO(x) in the UTLS ASM anticyclone from satellite measurements. Observations of NO(2) from the Optic...

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Autores principales: Dubé, Kimberlee, Randel, William, Bourassa, Adam, Degenstein, Doug
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9539711/
https://www.ncbi.nlm.nih.gov/pubmed/36246737
http://dx.doi.org/10.1029/2022GL099848
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author Dubé, Kimberlee
Randel, William
Bourassa, Adam
Degenstein, Doug
author_facet Dubé, Kimberlee
Randel, William
Bourassa, Adam
Degenstein, Doug
author_sort Dubé, Kimberlee
collection PubMed
description Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO(2), NO, and NO(x) in the UTLS ASM anticyclone from satellite measurements. Observations of NO(2) from the Optical Spectrograph and InfraRed Imager System, the Atmospheric Chemistry Experiment ‐ Fourier Transform Spectrometer (ACE‐FTS), and the Stratospheric Aerosol and Gas Experiment III on the International Space Station are considered. The PRATMO photochemical box model is used to quantify the NO(x) photochemistry, and to derive the NO(x) concentration using OSIRIS NO(2) and O(3) observations. The satellite data show a relative minimum in NO(2) over the ASM in the summer months, while the corresponding NO and NO(x) anomalies are elevated, mainly due to low O(3) and cold temperatures within the ASM. The observations within the ASM show reasonable agreement to simulations from the Whole Atmosphere Community Climate Model.
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spelling pubmed-95397112022-10-14 Tropopause‐Level NO(x) in the Asian Summer Monsoon Dubé, Kimberlee Randel, William Bourassa, Adam Degenstein, Doug Geophys Res Lett Research Letter Deep convection within the Asian summer monsoon (ASM) transports surface level air into the upper troposphere‐lower stratosphere (UTLS). This work aims to understand the distribution of NO(2), NO, and NO(x) in the UTLS ASM anticyclone from satellite measurements. Observations of NO(2) from the Optical Spectrograph and InfraRed Imager System, the Atmospheric Chemistry Experiment ‐ Fourier Transform Spectrometer (ACE‐FTS), and the Stratospheric Aerosol and Gas Experiment III on the International Space Station are considered. The PRATMO photochemical box model is used to quantify the NO(x) photochemistry, and to derive the NO(x) concentration using OSIRIS NO(2) and O(3) observations. The satellite data show a relative minimum in NO(2) over the ASM in the summer months, while the corresponding NO and NO(x) anomalies are elevated, mainly due to low O(3) and cold temperatures within the ASM. The observations within the ASM show reasonable agreement to simulations from the Whole Atmosphere Community Climate Model. John Wiley and Sons Inc. 2022-09-14 2022-09-28 /pmc/articles/PMC9539711/ /pubmed/36246737 http://dx.doi.org/10.1029/2022GL099848 Text en © 2022 The Authors. https://creativecommons.org/licenses/by-nc/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc/4.0/ (https://creativecommons.org/licenses/by-nc/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes.
spellingShingle Research Letter
Dubé, Kimberlee
Randel, William
Bourassa, Adam
Degenstein, Doug
Tropopause‐Level NO(x) in the Asian Summer Monsoon
title Tropopause‐Level NO(x) in the Asian Summer Monsoon
title_full Tropopause‐Level NO(x) in the Asian Summer Monsoon
title_fullStr Tropopause‐Level NO(x) in the Asian Summer Monsoon
title_full_unstemmed Tropopause‐Level NO(x) in the Asian Summer Monsoon
title_short Tropopause‐Level NO(x) in the Asian Summer Monsoon
title_sort tropopause‐level no(x) in the asian summer monsoon
topic Research Letter
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9539711/
https://www.ncbi.nlm.nih.gov/pubmed/36246737
http://dx.doi.org/10.1029/2022GL099848
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