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Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting

[Image: see text] Methane mitigation from the oil and gas (O&G) sector represents a key near-term global climate action opportunity. Recent legislation in the United States requires updating current methane reporting programs for oil and gas facilities with empirical data. While technological ad...

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Autores principales: Wang, Jiayang Lyra, Daniels, William S., Hammerling, Dorit M., Harrison, Matthew, Burmaster, Kaylyn, George, Fiji C., Ravikumar, Arvind P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9583612/
https://www.ncbi.nlm.nih.gov/pubmed/36201663
http://dx.doi.org/10.1021/acs.est.2c06211
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author Wang, Jiayang Lyra
Daniels, William S.
Hammerling, Dorit M.
Harrison, Matthew
Burmaster, Kaylyn
George, Fiji C.
Ravikumar, Arvind P.
author_facet Wang, Jiayang Lyra
Daniels, William S.
Hammerling, Dorit M.
Harrison, Matthew
Burmaster, Kaylyn
George, Fiji C.
Ravikumar, Arvind P.
author_sort Wang, Jiayang Lyra
collection PubMed
description [Image: see text] Methane mitigation from the oil and gas (O&G) sector represents a key near-term global climate action opportunity. Recent legislation in the United States requires updating current methane reporting programs for oil and gas facilities with empirical data. While technological advances have led to improvements in methane emissions measurements and monitoring, the overall effectiveness of mitigation strategies rests on quantifying spatially and temporally varying methane emissions more accurately than the current approaches. In this work, we demonstrate a quantification, monitoring, reporting, and verification framework that pairs snapshot measurements with continuous emissions monitoring systems (CEMS) to reconcile measurements with inventory estimates and account for intermittent emission events. We find that site-level emissions exhibit significant intraday and daily emission variations. Snapshot measurements of methane can span over 3 orders of magnitude and may have limited application in developing annualized inventory estimates at the site level. Consequently, while official inventories underestimate methane emissions on average, emissions at individual facilities can be higher or lower than inventory estimates. Using CEMS, we characterize distributions of frequency and duration of intermittent emission events. Technologies that allow high sampling frequency such as CEMS, paired with a mechanistic understanding of facility-level events, are key to an accurate accounting of short-duration, episodic, and high-volume events that are often missed in snapshot surveys and to scale snapshot measurements to annualized emissions estimates.
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spelling pubmed-95836122022-10-21 Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting Wang, Jiayang Lyra Daniels, William S. Hammerling, Dorit M. Harrison, Matthew Burmaster, Kaylyn George, Fiji C. Ravikumar, Arvind P. Environ Sci Technol [Image: see text] Methane mitigation from the oil and gas (O&G) sector represents a key near-term global climate action opportunity. Recent legislation in the United States requires updating current methane reporting programs for oil and gas facilities with empirical data. While technological advances have led to improvements in methane emissions measurements and monitoring, the overall effectiveness of mitigation strategies rests on quantifying spatially and temporally varying methane emissions more accurately than the current approaches. In this work, we demonstrate a quantification, monitoring, reporting, and verification framework that pairs snapshot measurements with continuous emissions monitoring systems (CEMS) to reconcile measurements with inventory estimates and account for intermittent emission events. We find that site-level emissions exhibit significant intraday and daily emission variations. Snapshot measurements of methane can span over 3 orders of magnitude and may have limited application in developing annualized inventory estimates at the site level. Consequently, while official inventories underestimate methane emissions on average, emissions at individual facilities can be higher or lower than inventory estimates. Using CEMS, we characterize distributions of frequency and duration of intermittent emission events. Technologies that allow high sampling frequency such as CEMS, paired with a mechanistic understanding of facility-level events, are key to an accurate accounting of short-duration, episodic, and high-volume events that are often missed in snapshot surveys and to scale snapshot measurements to annualized emissions estimates. American Chemical Society 2022-10-06 2022-10-18 /pmc/articles/PMC9583612/ /pubmed/36201663 http://dx.doi.org/10.1021/acs.est.2c06211 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Wang, Jiayang Lyra
Daniels, William S.
Hammerling, Dorit M.
Harrison, Matthew
Burmaster, Kaylyn
George, Fiji C.
Ravikumar, Arvind P.
Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting
title Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting
title_full Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting
title_fullStr Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting
title_full_unstemmed Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting
title_short Multiscale Methane Measurements at Oil and Gas Facilities Reveal Necessary Frameworks for Improved Emissions Accounting
title_sort multiscale methane measurements at oil and gas facilities reveal necessary frameworks for improved emissions accounting
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9583612/
https://www.ncbi.nlm.nih.gov/pubmed/36201663
http://dx.doi.org/10.1021/acs.est.2c06211
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