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The role of incoming flow on crystallization of undercooled liquids with a two-phase layer

Motivated by important applications of crystallization phenomena, we consider a directional solidification process for a binary melt with a two-phase (mushy) layer in the presence of weak melt flow. We consider the steady-state solidification scenario, so that the two-phase layer filled with solid a...

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Autores principales: Alexandrov, Dmitri V., Toropova, Liubov V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9596462/
https://www.ncbi.nlm.nih.gov/pubmed/36284156
http://dx.doi.org/10.1038/s41598-022-22786-w
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author Alexandrov, Dmitri V.
Toropova, Liubov V.
author_facet Alexandrov, Dmitri V.
Toropova, Liubov V.
author_sort Alexandrov, Dmitri V.
collection PubMed
description Motivated by important applications of crystallization phenomena, we consider a directional solidification process for a binary melt with a two-phase (mushy) layer in the presence of weak melt flow. We consider the steady-state solidification scenario, so that the two-phase layer filled with solid and liquid material keeps its thickness. In addition, we consider that the melt flows onto the two-phase layer slowly in the opposite direction to directional crystallization and solidifies there. A complete analytical solution to non-linear two-phase layer equations is constructed in a parametric form, where the solid phase fraction represents a decision variable. The temperature and solute concentration distributions, mushy layer permeability and average interdendritic spacing as well as solidification velocity and mushy layer thickness are analytically determined. We show that incoming melt flow plays a decisive role on mushy layer parameters and internal structures. The solid phase fraction within the two-phase layer and its thickness essentially grow while the mushy layer permeability and average interdendritic spacing decrease with increasing intensity of incoming melt flow.
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spelling pubmed-95964622022-10-27 The role of incoming flow on crystallization of undercooled liquids with a two-phase layer Alexandrov, Dmitri V. Toropova, Liubov V. Sci Rep Article Motivated by important applications of crystallization phenomena, we consider a directional solidification process for a binary melt with a two-phase (mushy) layer in the presence of weak melt flow. We consider the steady-state solidification scenario, so that the two-phase layer filled with solid and liquid material keeps its thickness. In addition, we consider that the melt flows onto the two-phase layer slowly in the opposite direction to directional crystallization and solidifies there. A complete analytical solution to non-linear two-phase layer equations is constructed in a parametric form, where the solid phase fraction represents a decision variable. The temperature and solute concentration distributions, mushy layer permeability and average interdendritic spacing as well as solidification velocity and mushy layer thickness are analytically determined. We show that incoming melt flow plays a decisive role on mushy layer parameters and internal structures. The solid phase fraction within the two-phase layer and its thickness essentially grow while the mushy layer permeability and average interdendritic spacing decrease with increasing intensity of incoming melt flow. Nature Publishing Group UK 2022-10-25 /pmc/articles/PMC9596462/ /pubmed/36284156 http://dx.doi.org/10.1038/s41598-022-22786-w Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Alexandrov, Dmitri V.
Toropova, Liubov V.
The role of incoming flow on crystallization of undercooled liquids with a two-phase layer
title The role of incoming flow on crystallization of undercooled liquids with a two-phase layer
title_full The role of incoming flow on crystallization of undercooled liquids with a two-phase layer
title_fullStr The role of incoming flow on crystallization of undercooled liquids with a two-phase layer
title_full_unstemmed The role of incoming flow on crystallization of undercooled liquids with a two-phase layer
title_short The role of incoming flow on crystallization of undercooled liquids with a two-phase layer
title_sort role of incoming flow on crystallization of undercooled liquids with a two-phase layer
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9596462/
https://www.ncbi.nlm.nih.gov/pubmed/36284156
http://dx.doi.org/10.1038/s41598-022-22786-w
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