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Destabilization of the Charge Density Wave and the Absence of Superconductivity in ScV(6)Sn(6) under High Pressures up to 11 GPa

RV(6)Sn(6) (R = Sc, Y, or rare earth) is a new family of kagome metals that have a similar vanadium structural motif as AV(3)Sb(5) (A = K, Rb, Cs) compounds. Unlike AV(3)Sb(5), ScV(6)Sn(6) is the only compound among the series of RV(6)Sn(6) that displays a charge density wave (CDW) order at ambient...

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Detalles Bibliográficos
Autores principales: Zhang, Xiaoxiao, Hou, Jun, Xia, Wei, Xu, Zhian, Yang, Pengtao, Wang, Anqi, Liu, Ziyi, Shen, Jie, Zhang, Hua, Dong, Xiaoli, Uwatoko, Yoshiya, Sun, Jianping, Wang, Bosen, Guo, Yanfeng, Cheng, Jinguang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9611248/
https://www.ncbi.nlm.nih.gov/pubmed/36295437
http://dx.doi.org/10.3390/ma15207372
Descripción
Sumario:RV(6)Sn(6) (R = Sc, Y, or rare earth) is a new family of kagome metals that have a similar vanadium structural motif as AV(3)Sb(5) (A = K, Rb, Cs) compounds. Unlike AV(3)Sb(5), ScV(6)Sn(6) is the only compound among the series of RV(6)Sn(6) that displays a charge density wave (CDW) order at ambient pressure, yet it shows no superconductivity (SC) at low temperatures. Here, we perform a high-pressure transport study on the ScV(6)Sn(6) single crystal to track the evolutions of the CDW transition and to explore possible SC. In contrast to AV(3)Sb(5) compounds, the CDW order of ScV(6)Sn(6) can be suppressed completely by a pressure of about 2.4 GPa, but no SC is detected down to 40 mK at 2.35 GPa and 1.5 K up to 11 GPa. Moreover, we observed that the resistivity anomaly around the CDW transition undergoes an obvious change at ~2.04 GPa before it vanishes completely. The present work highlights a distinct relationship between CDW and SC in ScV(6)Sn(6) in comparison with the well-studied AV(3)Sb(5).