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Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane

Semiconductor photoconductive switches are useful and versatile emitters of terahertz (THz) radiation with a broad range of applications in THz imaging and time-domain spectroscopy. One fundamental challenge for achieving efficient ultrafast switching, however, is the relatively long carrier lifetim...

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Autores principales: Zhang, Dehui, Xu, Zhen, Cheng, Gong, Liu, Zhe, Gutierrez, Audrey Rose, Zang, Wenzhe, Norris, Theodore B., Zhong, Zhaohui
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9613981/
https://www.ncbi.nlm.nih.gov/pubmed/36302852
http://dx.doi.org/10.1038/s41467-022-34170-3
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author Zhang, Dehui
Xu, Zhen
Cheng, Gong
Liu, Zhe
Gutierrez, Audrey Rose
Zang, Wenzhe
Norris, Theodore B.
Zhong, Zhaohui
author_facet Zhang, Dehui
Xu, Zhen
Cheng, Gong
Liu, Zhe
Gutierrez, Audrey Rose
Zang, Wenzhe
Norris, Theodore B.
Zhong, Zhaohui
author_sort Zhang, Dehui
collection PubMed
description Semiconductor photoconductive switches are useful and versatile emitters of terahertz (THz) radiation with a broad range of applications in THz imaging and time-domain spectroscopy. One fundamental challenge for achieving efficient ultrafast switching, however, is the relatively long carrier lifetime in most common semiconductors. To obtain picosecond ultrafast pulses, especially when coupled with waveguides/transmission lines, semiconductors are typically engineered with high defect density to reduce the carrier lifetimes, which in turn lowers the overall power output of the photoconductive switches. To overcome this fundamental trade-off, here we present a new hybrid photoconductive switch design by engineering a hot-carrier fast lane using graphene on silicon. While photoexcited carriers are generated in the silicon layer, similar to a conventional switch, the hot carriers are transferred to the graphene layer for efficient collection at the contacts. As a result, the graphene-silicon hybrid photoconductive switch emits THz fields with up to 80 times amplitude enhancement compared to its graphene-free counterpart. These results both further the understanding of ultrafast hot carrier transport in such hybrid systems and lay the groundwork toward intrinsically more powerful THz devices based on 2D-3D hybrid heterostructures.
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spelling pubmed-96139812022-10-29 Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane Zhang, Dehui Xu, Zhen Cheng, Gong Liu, Zhe Gutierrez, Audrey Rose Zang, Wenzhe Norris, Theodore B. Zhong, Zhaohui Nat Commun Article Semiconductor photoconductive switches are useful and versatile emitters of terahertz (THz) radiation with a broad range of applications in THz imaging and time-domain spectroscopy. One fundamental challenge for achieving efficient ultrafast switching, however, is the relatively long carrier lifetime in most common semiconductors. To obtain picosecond ultrafast pulses, especially when coupled with waveguides/transmission lines, semiconductors are typically engineered with high defect density to reduce the carrier lifetimes, which in turn lowers the overall power output of the photoconductive switches. To overcome this fundamental trade-off, here we present a new hybrid photoconductive switch design by engineering a hot-carrier fast lane using graphene on silicon. While photoexcited carriers are generated in the silicon layer, similar to a conventional switch, the hot carriers are transferred to the graphene layer for efficient collection at the contacts. As a result, the graphene-silicon hybrid photoconductive switch emits THz fields with up to 80 times amplitude enhancement compared to its graphene-free counterpart. These results both further the understanding of ultrafast hot carrier transport in such hybrid systems and lay the groundwork toward intrinsically more powerful THz devices based on 2D-3D hybrid heterostructures. Nature Publishing Group UK 2022-10-27 /pmc/articles/PMC9613981/ /pubmed/36302852 http://dx.doi.org/10.1038/s41467-022-34170-3 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Zhang, Dehui
Xu, Zhen
Cheng, Gong
Liu, Zhe
Gutierrez, Audrey Rose
Zang, Wenzhe
Norris, Theodore B.
Zhong, Zhaohui
Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane
title Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane
title_full Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane
title_fullStr Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane
title_full_unstemmed Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane
title_short Strongly enhanced THz generation enabled by a graphene hot-carrier fast lane
title_sort strongly enhanced thz generation enabled by a graphene hot-carrier fast lane
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9613981/
https://www.ncbi.nlm.nih.gov/pubmed/36302852
http://dx.doi.org/10.1038/s41467-022-34170-3
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