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Nanomechanical Spectroscopy of 2D Materials

[Image: see text] We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high Q silicon nitride nanomechanical resonator illuminated b...

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Detalles Bibliográficos
Autores principales: Kirchhof, Jan N., Yu, Yuefeng, Antheaume, Gabriel, Gordeev, Georgy, Yagodkin, Denis, Elliott, Peter, de Araújo, Daniel B., Sharma, Sangeeta, Reich, Stephanie, Bolotin, Kirill I.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9615986/
https://www.ncbi.nlm.nih.gov/pubmed/36252952
http://dx.doi.org/10.1021/acs.nanolett.2c01289
Descripción
Sumario:[Image: see text] We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high Q silicon nitride nanomechanical resonator illuminated by a wavelength-tunable laser source. From the heating-related frequency shift of the resonator as well as its optical reflection measured as a function of photon energy, we obtain the real and imaginary parts of the dielectric function. Our measurements are unaffected by substrate-related screening and do not require any assumptions on the underling optical constants. This fast (τ(rise) ∼ 135 ns), sensitive (noise-equivalent power = [Image: see text]), and broadband (1.2–3.1 eV, extendable to UV–THz) method provides an attractive alternative to spectroscopic or ellipsometric characterization techniques.