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Nanomechanical Spectroscopy of 2D Materials

[Image: see text] We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high Q silicon nitride nanomechanical resonator illuminated b...

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Autores principales: Kirchhof, Jan N., Yu, Yuefeng, Antheaume, Gabriel, Gordeev, Georgy, Yagodkin, Denis, Elliott, Peter, de Araújo, Daniel B., Sharma, Sangeeta, Reich, Stephanie, Bolotin, Kirill I.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9615986/
https://www.ncbi.nlm.nih.gov/pubmed/36252952
http://dx.doi.org/10.1021/acs.nanolett.2c01289
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author Kirchhof, Jan N.
Yu, Yuefeng
Antheaume, Gabriel
Gordeev, Georgy
Yagodkin, Denis
Elliott, Peter
de Araújo, Daniel B.
Sharma, Sangeeta
Reich, Stephanie
Bolotin, Kirill I.
author_facet Kirchhof, Jan N.
Yu, Yuefeng
Antheaume, Gabriel
Gordeev, Georgy
Yagodkin, Denis
Elliott, Peter
de Araújo, Daniel B.
Sharma, Sangeeta
Reich, Stephanie
Bolotin, Kirill I.
author_sort Kirchhof, Jan N.
collection PubMed
description [Image: see text] We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high Q silicon nitride nanomechanical resonator illuminated by a wavelength-tunable laser source. From the heating-related frequency shift of the resonator as well as its optical reflection measured as a function of photon energy, we obtain the real and imaginary parts of the dielectric function. Our measurements are unaffected by substrate-related screening and do not require any assumptions on the underling optical constants. This fast (τ(rise) ∼ 135 ns), sensitive (noise-equivalent power = [Image: see text]), and broadband (1.2–3.1 eV, extendable to UV–THz) method provides an attractive alternative to spectroscopic or ellipsometric characterization techniques.
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spelling pubmed-96159862023-10-17 Nanomechanical Spectroscopy of 2D Materials Kirchhof, Jan N. Yu, Yuefeng Antheaume, Gabriel Gordeev, Georgy Yagodkin, Denis Elliott, Peter de Araújo, Daniel B. Sharma, Sangeeta Reich, Stephanie Bolotin, Kirill I. Nano Lett [Image: see text] We introduce a nanomechanical platform for fast and sensitive measurements of the spectrally resolved optical dielectric function of 2D materials. At the heart of our approach is a suspended 2D material integrated into a high Q silicon nitride nanomechanical resonator illuminated by a wavelength-tunable laser source. From the heating-related frequency shift of the resonator as well as its optical reflection measured as a function of photon energy, we obtain the real and imaginary parts of the dielectric function. Our measurements are unaffected by substrate-related screening and do not require any assumptions on the underling optical constants. This fast (τ(rise) ∼ 135 ns), sensitive (noise-equivalent power = [Image: see text]), and broadband (1.2–3.1 eV, extendable to UV–THz) method provides an attractive alternative to spectroscopic or ellipsometric characterization techniques. American Chemical Society 2022-10-17 2022-10-26 /pmc/articles/PMC9615986/ /pubmed/36252952 http://dx.doi.org/10.1021/acs.nanolett.2c01289 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Kirchhof, Jan N.
Yu, Yuefeng
Antheaume, Gabriel
Gordeev, Georgy
Yagodkin, Denis
Elliott, Peter
de Araújo, Daniel B.
Sharma, Sangeeta
Reich, Stephanie
Bolotin, Kirill I.
Nanomechanical Spectroscopy of 2D Materials
title Nanomechanical Spectroscopy of 2D Materials
title_full Nanomechanical Spectroscopy of 2D Materials
title_fullStr Nanomechanical Spectroscopy of 2D Materials
title_full_unstemmed Nanomechanical Spectroscopy of 2D Materials
title_short Nanomechanical Spectroscopy of 2D Materials
title_sort nanomechanical spectroscopy of 2d materials
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9615986/
https://www.ncbi.nlm.nih.gov/pubmed/36252952
http://dx.doi.org/10.1021/acs.nanolett.2c01289
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