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Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures

The study of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) heterostructures on a MgO substrate with Ba(0.8)Sr(0.2)TiO(3) ferroelectric films revealed the occurrence of a metallic character of the temperature behavior of the resistance at a temperature less than 175 K. This behavior is associate...

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Autores principales: Chibirev, Aleksei O., Leontyev, Andrei V., Kabanov, Viktor V., Mamin, Rinat F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9655687/
https://www.ncbi.nlm.nih.gov/pubmed/36364550
http://dx.doi.org/10.3390/nano12213774
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author Chibirev, Aleksei O.
Leontyev, Andrei V.
Kabanov, Viktor V.
Mamin, Rinat F.
author_facet Chibirev, Aleksei O.
Leontyev, Andrei V.
Kabanov, Viktor V.
Mamin, Rinat F.
author_sort Chibirev, Aleksei O.
collection PubMed
description The study of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) heterostructures on a MgO substrate with Ba(0.8)Sr(0.2)TiO(3) ferroelectric films revealed the occurrence of a metallic character of the temperature behavior of the resistance at a temperature less than 175 K. This behavior is associated with an increased charge concentration at the interface due to a discontinuity in the ferroelectric polarization at the interface between the films. At these temperatures, the effect of negative photoconductivity is observed under uniform illumination with the light of a selected spectral composition event on the surface of the ferroelectric film. The combined exposure to green and infrared light led to an addition of the effects. As a result, a cumulative effect was observed. The effect of metallic conductivity is due to the discontinuity of ferroelectric polarization. Therefore, we explain that the partial screening of the ferroelectric polarization by photogenerated charge carriers causes a reduction in the carrier concentration at the interface. Measurements in the Kelvin mode of atomic force microscopy showed that illumination influences the surface charge concentration in a similar way; this observation confirms our hypothesis.
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spelling pubmed-96556872022-11-15 Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures Chibirev, Aleksei O. Leontyev, Andrei V. Kabanov, Viktor V. Mamin, Rinat F. Nanomaterials (Basel) Article The study of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) heterostructures on a MgO substrate with Ba(0.8)Sr(0.2)TiO(3) ferroelectric films revealed the occurrence of a metallic character of the temperature behavior of the resistance at a temperature less than 175 K. This behavior is associated with an increased charge concentration at the interface due to a discontinuity in the ferroelectric polarization at the interface between the films. At these temperatures, the effect of negative photoconductivity is observed under uniform illumination with the light of a selected spectral composition event on the surface of the ferroelectric film. The combined exposure to green and infrared light led to an addition of the effects. As a result, a cumulative effect was observed. The effect of metallic conductivity is due to the discontinuity of ferroelectric polarization. Therefore, we explain that the partial screening of the ferroelectric polarization by photogenerated charge carriers causes a reduction in the carrier concentration at the interface. Measurements in the Kelvin mode of atomic force microscopy showed that illumination influences the surface charge concentration in a similar way; this observation confirms our hypothesis. MDPI 2022-10-26 /pmc/articles/PMC9655687/ /pubmed/36364550 http://dx.doi.org/10.3390/nano12213774 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Chibirev, Aleksei O.
Leontyev, Andrei V.
Kabanov, Viktor V.
Mamin, Rinat F.
Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures
title Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures
title_full Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures
title_fullStr Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures
title_full_unstemmed Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures
title_short Origin of Negative Photoconductivity at the Interface of Ba(0.8)Sr(0.2)TiO(3)/LaMnO(3)/Ba(0.8)Sr(0.2)TiO(3) Heterostructures
title_sort origin of negative photoconductivity at the interface of ba(0.8)sr(0.2)tio(3)/lamno(3)/ba(0.8)sr(0.2)tio(3) heterostructures
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9655687/
https://www.ncbi.nlm.nih.gov/pubmed/36364550
http://dx.doi.org/10.3390/nano12213774
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