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The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application

The integration of additive manufacturing (3D printing) in the biomedical sector required material to portray a holistic characteristic in terms of printability, biocompatibility, degradability, and mechanical properties. This research aims to evaluate the 3D printability and mechanical properties o...

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Autores principales: Abu Bakar, Ahmad Adnan, Zainuddin, Muhammad Zulhilmi, Abdullah, Shahino Mah, Tamchek, Nizam, Mohd Noor, Ikhwan Syafiq, Alauddin, Muhammad Syafiq, Alforidi, Ahmad, Mohd Ghazali, Mohd Ifwat
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9657082/
https://www.ncbi.nlm.nih.gov/pubmed/36365512
http://dx.doi.org/10.3390/polym14214518
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author Abu Bakar, Ahmad Adnan
Zainuddin, Muhammad Zulhilmi
Abdullah, Shahino Mah
Tamchek, Nizam
Mohd Noor, Ikhwan Syafiq
Alauddin, Muhammad Syafiq
Alforidi, Ahmad
Mohd Ghazali, Mohd Ifwat
author_facet Abu Bakar, Ahmad Adnan
Zainuddin, Muhammad Zulhilmi
Abdullah, Shahino Mah
Tamchek, Nizam
Mohd Noor, Ikhwan Syafiq
Alauddin, Muhammad Syafiq
Alforidi, Ahmad
Mohd Ghazali, Mohd Ifwat
author_sort Abu Bakar, Ahmad Adnan
collection PubMed
description The integration of additive manufacturing (3D printing) in the biomedical sector required material to portray a holistic characteristic in terms of printability, biocompatibility, degradability, and mechanical properties. This research aims to evaluate the 3D printability and mechanical properties of polyhydroxybutyrate (PHB) as additives in the urethane dimethacrylate (UDMA) based resin and its potential for medical applications. The printability of the PHB/UDMA resin blends was limited to 11 wt.% as it reached the maximum viscosity value at 2188 cP. Two-way analysis of variance (ANOVA) was also conducted to assess the significant effect of the varied PHB (wt.%) incorporation within UDMA resin, and the aging duration of 3D printed PHB/UDMA on mechanical properties in terms of tensile and impact properties. Meanwhile, the increasing crystallinity index (CI) of X-ray diffraction (XRD) in the 3D printed PHB/UDMA as the PHB loading increased, indicating that there is a strong correlation with the lower tensile and impact strength. FESEM images also proved that the agglomerations that occurred within the UDMA matrix had affected the mechanical performance of 3D printed PHB/UDMA. Nonetheless, the thermal stability of the 3D printed PHB/UDMA had only a slight deviation from the 3D printed UDMA since it had better thermal processability.
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spelling pubmed-96570822022-11-15 The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application Abu Bakar, Ahmad Adnan Zainuddin, Muhammad Zulhilmi Abdullah, Shahino Mah Tamchek, Nizam Mohd Noor, Ikhwan Syafiq Alauddin, Muhammad Syafiq Alforidi, Ahmad Mohd Ghazali, Mohd Ifwat Polymers (Basel) Article The integration of additive manufacturing (3D printing) in the biomedical sector required material to portray a holistic characteristic in terms of printability, biocompatibility, degradability, and mechanical properties. This research aims to evaluate the 3D printability and mechanical properties of polyhydroxybutyrate (PHB) as additives in the urethane dimethacrylate (UDMA) based resin and its potential for medical applications. The printability of the PHB/UDMA resin blends was limited to 11 wt.% as it reached the maximum viscosity value at 2188 cP. Two-way analysis of variance (ANOVA) was also conducted to assess the significant effect of the varied PHB (wt.%) incorporation within UDMA resin, and the aging duration of 3D printed PHB/UDMA on mechanical properties in terms of tensile and impact properties. Meanwhile, the increasing crystallinity index (CI) of X-ray diffraction (XRD) in the 3D printed PHB/UDMA as the PHB loading increased, indicating that there is a strong correlation with the lower tensile and impact strength. FESEM images also proved that the agglomerations that occurred within the UDMA matrix had affected the mechanical performance of 3D printed PHB/UDMA. Nonetheless, the thermal stability of the 3D printed PHB/UDMA had only a slight deviation from the 3D printed UDMA since it had better thermal processability. MDPI 2022-10-25 /pmc/articles/PMC9657082/ /pubmed/36365512 http://dx.doi.org/10.3390/polym14214518 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Abu Bakar, Ahmad Adnan
Zainuddin, Muhammad Zulhilmi
Abdullah, Shahino Mah
Tamchek, Nizam
Mohd Noor, Ikhwan Syafiq
Alauddin, Muhammad Syafiq
Alforidi, Ahmad
Mohd Ghazali, Mohd Ifwat
The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application
title The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application
title_full The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application
title_fullStr The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application
title_full_unstemmed The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application
title_short The 3D Printability and Mechanical Properties of Polyhydroxybutyrate (PHB) as Additives in Urethane Dimethacrylate (UDMA) Blends Polymer for Medical Application
title_sort 3d printability and mechanical properties of polyhydroxybutyrate (phb) as additives in urethane dimethacrylate (udma) blends polymer for medical application
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9657082/
https://www.ncbi.nlm.nih.gov/pubmed/36365512
http://dx.doi.org/10.3390/polym14214518
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