Kirigami‐Inspired Programmable Soft Magnetoresponsive Actuators with Versatile Morphing Modes

Untethered soft magnetoresponsive actuators (SMRAs), which can realize rapid shape transformation, have attracted widespread attention for their strategic applications in exploration, transportation, and minimally invasive medicine. It remains a challenge to fabricate SMRAs with complicated morphing modes (more than bending and folding), limiting their applications to simple shape‐morphing and locomotion. Herein, a method integrating the ancient kirigami art and an advanced mechanical assembly method is proposed, which realizes 2D‐to‐3D and 3D‐to‐3D complicated shape‐morphing and precise magnetization programming through cut‐guided deformation. The kirigami‐inspired SMRAs exhibit good robustness after actuating more than 10000 times. An integrated finite element analysis method is developed to quantitatively predict the shape transformation of SMRAs under magnetic actuation. By leveraging this method, a set of 3D curved responsive morphologies with programmed Gaussian curvature are fabricated (e.g., ellipsoid and saddle structures), specifically 3D multilayer structures and face‐like shapes with different expressions, which are difficult to realize using previous approaches. Furthermore, a bionic‐scaled soft crawling robot with significant obstacle surmounting ability is fabricated using the kirigami‐inspired method. The ability of the method to achieve programmable SMRAs with versatile morphing modes may broaden its applications in soft robotics, color‐switchable devices, and clinical treatments.