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Optically trapped room temperature polariton condensate in an organic semiconductor

The strong nonlinearities of exciton-polariton condensates in lattices make them suitable candidates for neuromorphic computing and physical simulations of complex problems. So far, all room temperature polariton condensate lattices have been achieved by nanoimprinting microcavities, which by nature...

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Autores principales: Wei, Mengjie, Verstraelen, Wouter, Orfanakis, Konstantinos, Ruseckas, Arvydas, Liew, Timothy C. H., Samuel, Ifor D. W., Turnbull, Graham A., Ohadi, Hamid
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9691723/
https://www.ncbi.nlm.nih.gov/pubmed/36424397
http://dx.doi.org/10.1038/s41467-022-34440-0
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author Wei, Mengjie
Verstraelen, Wouter
Orfanakis, Konstantinos
Ruseckas, Arvydas
Liew, Timothy C. H.
Samuel, Ifor D. W.
Turnbull, Graham A.
Ohadi, Hamid
author_facet Wei, Mengjie
Verstraelen, Wouter
Orfanakis, Konstantinos
Ruseckas, Arvydas
Liew, Timothy C. H.
Samuel, Ifor D. W.
Turnbull, Graham A.
Ohadi, Hamid
author_sort Wei, Mengjie
collection PubMed
description The strong nonlinearities of exciton-polariton condensates in lattices make them suitable candidates for neuromorphic computing and physical simulations of complex problems. So far, all room temperature polariton condensate lattices have been achieved by nanoimprinting microcavities, which by nature lacks the crucial tunability required for realistic reconfigurable simulators. Here, we report the observation of a quantised oscillating nonlinear quantum fluid in 1D and 2D potentials in an organic microcavity at room temperature, achieved by an on-the-fly fully tuneable optical approach. Remarkably, the condensate is delocalised from the excitation region by macroscopic distances, leading both to longer coherence and a threshold one order of magnitude lower than that with a conventional Gaussian excitation profile. We observe different mode selection behaviour compared to inorganic materials, which highlights the anomalous scaling of blueshift with pump intensity and the presence of sizeable energy-relaxation mechanisms. Our work is a major step towards a fully tuneable polariton simulator at room temperature.
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spelling pubmed-96917232022-11-26 Optically trapped room temperature polariton condensate in an organic semiconductor Wei, Mengjie Verstraelen, Wouter Orfanakis, Konstantinos Ruseckas, Arvydas Liew, Timothy C. H. Samuel, Ifor D. W. Turnbull, Graham A. Ohadi, Hamid Nat Commun Article The strong nonlinearities of exciton-polariton condensates in lattices make them suitable candidates for neuromorphic computing and physical simulations of complex problems. So far, all room temperature polariton condensate lattices have been achieved by nanoimprinting microcavities, which by nature lacks the crucial tunability required for realistic reconfigurable simulators. Here, we report the observation of a quantised oscillating nonlinear quantum fluid in 1D and 2D potentials in an organic microcavity at room temperature, achieved by an on-the-fly fully tuneable optical approach. Remarkably, the condensate is delocalised from the excitation region by macroscopic distances, leading both to longer coherence and a threshold one order of magnitude lower than that with a conventional Gaussian excitation profile. We observe different mode selection behaviour compared to inorganic materials, which highlights the anomalous scaling of blueshift with pump intensity and the presence of sizeable energy-relaxation mechanisms. Our work is a major step towards a fully tuneable polariton simulator at room temperature. Nature Publishing Group UK 2022-11-23 /pmc/articles/PMC9691723/ /pubmed/36424397 http://dx.doi.org/10.1038/s41467-022-34440-0 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Wei, Mengjie
Verstraelen, Wouter
Orfanakis, Konstantinos
Ruseckas, Arvydas
Liew, Timothy C. H.
Samuel, Ifor D. W.
Turnbull, Graham A.
Ohadi, Hamid
Optically trapped room temperature polariton condensate in an organic semiconductor
title Optically trapped room temperature polariton condensate in an organic semiconductor
title_full Optically trapped room temperature polariton condensate in an organic semiconductor
title_fullStr Optically trapped room temperature polariton condensate in an organic semiconductor
title_full_unstemmed Optically trapped room temperature polariton condensate in an organic semiconductor
title_short Optically trapped room temperature polariton condensate in an organic semiconductor
title_sort optically trapped room temperature polariton condensate in an organic semiconductor
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9691723/
https://www.ncbi.nlm.nih.gov/pubmed/36424397
http://dx.doi.org/10.1038/s41467-022-34440-0
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