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Correlation driven near-flat band Stoner excitations in a Kagome magnet

Among condensed matter systems, Mott insulators exhibit diverse properties that emerge from electronic correlations. In itinerant metals, correlations are usually weak, but can also be enhanced via geometrical confinement of electrons, that manifest as ‘flat’ dispersionless electronic bands. In the...

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Autores principales: Nag, Abhishek, Peng, Yiran, Li, Jiemin, Agrestini, S., Robarts, H. C., García-Fernández, Mirian, Walters, A. C., Wang, Qi, Yin, Qiangwei, Lei, Hechang, Yin, Zhiping, Zhou, Ke-Jin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9705307/
https://www.ncbi.nlm.nih.gov/pubmed/36443343
http://dx.doi.org/10.1038/s41467-022-34933-y
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author Nag, Abhishek
Peng, Yiran
Li, Jiemin
Agrestini, S.
Robarts, H. C.
García-Fernández, Mirian
Walters, A. C.
Wang, Qi
Yin, Qiangwei
Lei, Hechang
Yin, Zhiping
Zhou, Ke-Jin
author_facet Nag, Abhishek
Peng, Yiran
Li, Jiemin
Agrestini, S.
Robarts, H. C.
García-Fernández, Mirian
Walters, A. C.
Wang, Qi
Yin, Qiangwei
Lei, Hechang
Yin, Zhiping
Zhou, Ke-Jin
author_sort Nag, Abhishek
collection PubMed
description Among condensed matter systems, Mott insulators exhibit diverse properties that emerge from electronic correlations. In itinerant metals, correlations are usually weak, but can also be enhanced via geometrical confinement of electrons, that manifest as ‘flat’ dispersionless electronic bands. In the fast developing field of topological materials, which includes Dirac and Weyl semimetals, flat bands are one of the important components that can result in unusual magnetic and transport behaviour. To date, characterisation of flat bands and their magnetism is scarce, hindering the design of novel materials. Here, we investigate the ferromagnetic Kagomé semimetal Co(3)Sn(2)S(2) using resonant inelastic X-ray scattering. Remarkably, nearly non-dispersive Stoner spin excitation peaks are observed, sharply contrasting with the featureless Stoner continuum expected in conventional ferromagnetic metals. Our band structure and dynamic spin susceptibility calculations, and thermal evolution of the excitations, confirm the nearly non-dispersive Stoner excitations as unique signatures of correlations and spin-polarized electronic flat bands in Co(3)Sn(2)S(2). These observations serve as a cornerstone for further exploration of band-induced symmetry-breaking orders in topological materials.
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spelling pubmed-97053072022-11-30 Correlation driven near-flat band Stoner excitations in a Kagome magnet Nag, Abhishek Peng, Yiran Li, Jiemin Agrestini, S. Robarts, H. C. García-Fernández, Mirian Walters, A. C. Wang, Qi Yin, Qiangwei Lei, Hechang Yin, Zhiping Zhou, Ke-Jin Nat Commun Article Among condensed matter systems, Mott insulators exhibit diverse properties that emerge from electronic correlations. In itinerant metals, correlations are usually weak, but can also be enhanced via geometrical confinement of electrons, that manifest as ‘flat’ dispersionless electronic bands. In the fast developing field of topological materials, which includes Dirac and Weyl semimetals, flat bands are one of the important components that can result in unusual magnetic and transport behaviour. To date, characterisation of flat bands and their magnetism is scarce, hindering the design of novel materials. Here, we investigate the ferromagnetic Kagomé semimetal Co(3)Sn(2)S(2) using resonant inelastic X-ray scattering. Remarkably, nearly non-dispersive Stoner spin excitation peaks are observed, sharply contrasting with the featureless Stoner continuum expected in conventional ferromagnetic metals. Our band structure and dynamic spin susceptibility calculations, and thermal evolution of the excitations, confirm the nearly non-dispersive Stoner excitations as unique signatures of correlations and spin-polarized electronic flat bands in Co(3)Sn(2)S(2). These observations serve as a cornerstone for further exploration of band-induced symmetry-breaking orders in topological materials. Nature Publishing Group UK 2022-11-28 /pmc/articles/PMC9705307/ /pubmed/36443343 http://dx.doi.org/10.1038/s41467-022-34933-y Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Nag, Abhishek
Peng, Yiran
Li, Jiemin
Agrestini, S.
Robarts, H. C.
García-Fernández, Mirian
Walters, A. C.
Wang, Qi
Yin, Qiangwei
Lei, Hechang
Yin, Zhiping
Zhou, Ke-Jin
Correlation driven near-flat band Stoner excitations in a Kagome magnet
title Correlation driven near-flat band Stoner excitations in a Kagome magnet
title_full Correlation driven near-flat band Stoner excitations in a Kagome magnet
title_fullStr Correlation driven near-flat band Stoner excitations in a Kagome magnet
title_full_unstemmed Correlation driven near-flat band Stoner excitations in a Kagome magnet
title_short Correlation driven near-flat band Stoner excitations in a Kagome magnet
title_sort correlation driven near-flat band stoner excitations in a kagome magnet
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9705307/
https://www.ncbi.nlm.nih.gov/pubmed/36443343
http://dx.doi.org/10.1038/s41467-022-34933-y
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