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Room-temperature polariton quantum fluids in halide perovskites

Quantum fluids exhibit quantum mechanical effects at the macroscopic level, which contrast strongly with classical fluids. Gain-dissipative solid-state exciton-polaritons systems are promising emulation platforms for complex quantum fluid studies at elevated temperatures. Recently, halide perovskite...

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Autores principales: Peng, Kai, Tao, Renjie, Haeberlé, Louis, Li, Quanwei, Jin, Dafei, Fleming, Graham R., Kéna-Cohen, Stéphane, Zhang, Xiang, Bao, Wei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9712507/
https://www.ncbi.nlm.nih.gov/pubmed/36450719
http://dx.doi.org/10.1038/s41467-022-34987-y
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author Peng, Kai
Tao, Renjie
Haeberlé, Louis
Li, Quanwei
Jin, Dafei
Fleming, Graham R.
Kéna-Cohen, Stéphane
Zhang, Xiang
Bao, Wei
author_facet Peng, Kai
Tao, Renjie
Haeberlé, Louis
Li, Quanwei
Jin, Dafei
Fleming, Graham R.
Kéna-Cohen, Stéphane
Zhang, Xiang
Bao, Wei
author_sort Peng, Kai
collection PubMed
description Quantum fluids exhibit quantum mechanical effects at the macroscopic level, which contrast strongly with classical fluids. Gain-dissipative solid-state exciton-polaritons systems are promising emulation platforms for complex quantum fluid studies at elevated temperatures. Recently, halide perovskite polariton systems have emerged as materials with distinctive advantages over other room-temperature systems for future studies of topological physics, non-Abelian gauge fields, and spin-orbit interactions. However, the demonstration of nonlinear quantum hydrodynamics, such as superfluidity and Čerenkov flow, which is a consequence of the renormalized elementary excitation spectrum, remains elusive in halide perovskites. Here, using homogenous halide perovskites single crystals, we report, in both one- and two-dimensional cases, the complete set of quantum fluid phase transitions from normal classical fluids to scatterless polariton superfluids and supersonic fluids—all at room temperature, clear consequences of the Landau criterion. Specifically, the supersonic Čerenkov wave pattern was observed at room temperature. The experimental results are also in quantitative agreement with theoretical predictions from the dissipative Gross-Pitaevskii equation. Our results set the stage for exploring the rich non-equilibrium quantum fluid many-body physics at room temperature and also pave the way for important polaritonic device applications.
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spelling pubmed-97125072022-12-02 Room-temperature polariton quantum fluids in halide perovskites Peng, Kai Tao, Renjie Haeberlé, Louis Li, Quanwei Jin, Dafei Fleming, Graham R. Kéna-Cohen, Stéphane Zhang, Xiang Bao, Wei Nat Commun Article Quantum fluids exhibit quantum mechanical effects at the macroscopic level, which contrast strongly with classical fluids. Gain-dissipative solid-state exciton-polaritons systems are promising emulation platforms for complex quantum fluid studies at elevated temperatures. Recently, halide perovskite polariton systems have emerged as materials with distinctive advantages over other room-temperature systems for future studies of topological physics, non-Abelian gauge fields, and spin-orbit interactions. However, the demonstration of nonlinear quantum hydrodynamics, such as superfluidity and Čerenkov flow, which is a consequence of the renormalized elementary excitation spectrum, remains elusive in halide perovskites. Here, using homogenous halide perovskites single crystals, we report, in both one- and two-dimensional cases, the complete set of quantum fluid phase transitions from normal classical fluids to scatterless polariton superfluids and supersonic fluids—all at room temperature, clear consequences of the Landau criterion. Specifically, the supersonic Čerenkov wave pattern was observed at room temperature. The experimental results are also in quantitative agreement with theoretical predictions from the dissipative Gross-Pitaevskii equation. Our results set the stage for exploring the rich non-equilibrium quantum fluid many-body physics at room temperature and also pave the way for important polaritonic device applications. Nature Publishing Group UK 2022-11-30 /pmc/articles/PMC9712507/ /pubmed/36450719 http://dx.doi.org/10.1038/s41467-022-34987-y Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Peng, Kai
Tao, Renjie
Haeberlé, Louis
Li, Quanwei
Jin, Dafei
Fleming, Graham R.
Kéna-Cohen, Stéphane
Zhang, Xiang
Bao, Wei
Room-temperature polariton quantum fluids in halide perovskites
title Room-temperature polariton quantum fluids in halide perovskites
title_full Room-temperature polariton quantum fluids in halide perovskites
title_fullStr Room-temperature polariton quantum fluids in halide perovskites
title_full_unstemmed Room-temperature polariton quantum fluids in halide perovskites
title_short Room-temperature polariton quantum fluids in halide perovskites
title_sort room-temperature polariton quantum fluids in halide perovskites
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9712507/
https://www.ncbi.nlm.nih.gov/pubmed/36450719
http://dx.doi.org/10.1038/s41467-022-34987-y
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