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Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)

Environmental pollution, especially water pollution, is becoming increasingly serious. Organic dyes are one type of the harmful pollutants that pollute groundwater and destroy ecosystems. In this work, a series of graphitic carbon nitride (g-C(3)N(4))/ZnO photocatalysts were facilely synthesized thr...

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Detalles Bibliográficos
Autores principales: Wang, Yayang, Yang, Xiaojie, Lou, Jiahui, Huang, Yaqiong, Peng, Jian, Li, Yuesheng, Liu, Yi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9736064/
https://www.ncbi.nlm.nih.gov/pubmed/36500561
http://dx.doi.org/10.3390/molecules27238476
Descripción
Sumario:Environmental pollution, especially water pollution, is becoming increasingly serious. Organic dyes are one type of the harmful pollutants that pollute groundwater and destroy ecosystems. In this work, a series of graphitic carbon nitride (g-C(3)N(4))/ZnO photocatalysts were facilely synthesized through a grinding method using ZnO nanoparticles and g-C(3)N(4) as the starting materials. According to the results, the photocatalytic performance of 10 wt.% CN-200/Z-500 (CN-200, which g-C(3)N(4) was 200 kGy, referred to the irradiation metering. Z-500, which ZnO was 500 °C, referred to the calcination temperature) with the CN-200 exposed to electron beam radiation was better than those of either Z-500 or CN-200 alone. This material displayed a 98.9% degradation rate of MB (20 mg/L) in 120 min. The improvement of the photocatalytic performance of the 10 wt.% CN-200/Z-500 composite material was caused by the improvement of the separation efficiency of photoinduced electron–hole pairs, which was, in turn, due to the formation of heterojunctions between CN-200 and Z-500 interfaces. Thus, this study proposes the application of electron-beam irradiation technology for the modification of photocatalytic materials and the improvement of photocatalytic performance.