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Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)

Environmental pollution, especially water pollution, is becoming increasingly serious. Organic dyes are one type of the harmful pollutants that pollute groundwater and destroy ecosystems. In this work, a series of graphitic carbon nitride (g-C(3)N(4))/ZnO photocatalysts were facilely synthesized thr...

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Autores principales: Wang, Yayang, Yang, Xiaojie, Lou, Jiahui, Huang, Yaqiong, Peng, Jian, Li, Yuesheng, Liu, Yi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9736064/
https://www.ncbi.nlm.nih.gov/pubmed/36500561
http://dx.doi.org/10.3390/molecules27238476
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author Wang, Yayang
Yang, Xiaojie
Lou, Jiahui
Huang, Yaqiong
Peng, Jian
Li, Yuesheng
Liu, Yi
author_facet Wang, Yayang
Yang, Xiaojie
Lou, Jiahui
Huang, Yaqiong
Peng, Jian
Li, Yuesheng
Liu, Yi
author_sort Wang, Yayang
collection PubMed
description Environmental pollution, especially water pollution, is becoming increasingly serious. Organic dyes are one type of the harmful pollutants that pollute groundwater and destroy ecosystems. In this work, a series of graphitic carbon nitride (g-C(3)N(4))/ZnO photocatalysts were facilely synthesized through a grinding method using ZnO nanoparticles and g-C(3)N(4) as the starting materials. According to the results, the photocatalytic performance of 10 wt.% CN-200/Z-500 (CN-200, which g-C(3)N(4) was 200 kGy, referred to the irradiation metering. Z-500, which ZnO was 500 °C, referred to the calcination temperature) with the CN-200 exposed to electron beam radiation was better than those of either Z-500 or CN-200 alone. This material displayed a 98.9% degradation rate of MB (20 mg/L) in 120 min. The improvement of the photocatalytic performance of the 10 wt.% CN-200/Z-500 composite material was caused by the improvement of the separation efficiency of photoinduced electron–hole pairs, which was, in turn, due to the formation of heterojunctions between CN-200 and Z-500 interfaces. Thus, this study proposes the application of electron-beam irradiation technology for the modification of photocatalytic materials and the improvement of photocatalytic performance.
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spelling pubmed-97360642022-12-11 Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4) Wang, Yayang Yang, Xiaojie Lou, Jiahui Huang, Yaqiong Peng, Jian Li, Yuesheng Liu, Yi Molecules Article Environmental pollution, especially water pollution, is becoming increasingly serious. Organic dyes are one type of the harmful pollutants that pollute groundwater and destroy ecosystems. In this work, a series of graphitic carbon nitride (g-C(3)N(4))/ZnO photocatalysts were facilely synthesized through a grinding method using ZnO nanoparticles and g-C(3)N(4) as the starting materials. According to the results, the photocatalytic performance of 10 wt.% CN-200/Z-500 (CN-200, which g-C(3)N(4) was 200 kGy, referred to the irradiation metering. Z-500, which ZnO was 500 °C, referred to the calcination temperature) with the CN-200 exposed to electron beam radiation was better than those of either Z-500 or CN-200 alone. This material displayed a 98.9% degradation rate of MB (20 mg/L) in 120 min. The improvement of the photocatalytic performance of the 10 wt.% CN-200/Z-500 composite material was caused by the improvement of the separation efficiency of photoinduced electron–hole pairs, which was, in turn, due to the formation of heterojunctions between CN-200 and Z-500 interfaces. Thus, this study proposes the application of electron-beam irradiation technology for the modification of photocatalytic materials and the improvement of photocatalytic performance. MDPI 2022-12-02 /pmc/articles/PMC9736064/ /pubmed/36500561 http://dx.doi.org/10.3390/molecules27238476 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Wang, Yayang
Yang, Xiaojie
Lou, Jiahui
Huang, Yaqiong
Peng, Jian
Li, Yuesheng
Liu, Yi
Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)
title Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)
title_full Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)
title_fullStr Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)
title_full_unstemmed Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)
title_short Enhance ZnO Photocatalytic Performance via Radiation Modified g-C(3)N(4)
title_sort enhance zno photocatalytic performance via radiation modified g-c(3)n(4)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9736064/
https://www.ncbi.nlm.nih.gov/pubmed/36500561
http://dx.doi.org/10.3390/molecules27238476
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