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Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties

Polycrystalline PbTe:In films on a polyimide substrate were obtained and investigated. Their structural and transport properties in a wide range of temperatures (10–300 K) were studied. The unique feature of In impurity in PbTe is the stabilization of the Fermi level (pinning effect) that allowed fo...

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Autores principales: Kovalyuk, Vadim, Sheveleva, Evgeniia, Auslender, Mark, Goltsman, Gregory, Shneck, Roni, Dashevsky, Zinovi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9736097/
https://www.ncbi.nlm.nih.gov/pubmed/36499879
http://dx.doi.org/10.3390/ma15238383
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author Kovalyuk, Vadim
Sheveleva, Evgeniia
Auslender, Mark
Goltsman, Gregory
Shneck, Roni
Dashevsky, Zinovi
author_facet Kovalyuk, Vadim
Sheveleva, Evgeniia
Auslender, Mark
Goltsman, Gregory
Shneck, Roni
Dashevsky, Zinovi
author_sort Kovalyuk, Vadim
collection PubMed
description Polycrystalline PbTe:In films on a polyimide substrate were obtained and investigated. Their structural and transport properties in a wide range of temperatures (10–300 K) were studied. The unique feature of In impurity in PbTe is the stabilization of the Fermi level (pinning effect) that allowed for the preparation polycrystalline films with the same carrier concentration. We found that heat treatment in an argon atmosphere does not change the average grain size and carrier concentration for as-grown films but greatly increases the Hall mobility and the electron mean free path. By comparing the mobility in the bulk and in the film after heat treatment, we extracted the value of the mobility that arises due to scattering at the grain boundary barriers. The ultimate goal of the present study is the development of these films in designing portable uncooled photodetectors for the mid-IR range.
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spelling pubmed-97360972022-12-11 Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties Kovalyuk, Vadim Sheveleva, Evgeniia Auslender, Mark Goltsman, Gregory Shneck, Roni Dashevsky, Zinovi Materials (Basel) Article Polycrystalline PbTe:In films on a polyimide substrate were obtained and investigated. Their structural and transport properties in a wide range of temperatures (10–300 K) were studied. The unique feature of In impurity in PbTe is the stabilization of the Fermi level (pinning effect) that allowed for the preparation polycrystalline films with the same carrier concentration. We found that heat treatment in an argon atmosphere does not change the average grain size and carrier concentration for as-grown films but greatly increases the Hall mobility and the electron mean free path. By comparing the mobility in the bulk and in the film after heat treatment, we extracted the value of the mobility that arises due to scattering at the grain boundary barriers. The ultimate goal of the present study is the development of these films in designing portable uncooled photodetectors for the mid-IR range. MDPI 2022-11-25 /pmc/articles/PMC9736097/ /pubmed/36499879 http://dx.doi.org/10.3390/ma15238383 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Kovalyuk, Vadim
Sheveleva, Evgeniia
Auslender, Mark
Goltsman, Gregory
Shneck, Roni
Dashevsky, Zinovi
Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties
title Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties
title_full Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties
title_fullStr Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties
title_full_unstemmed Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties
title_short Polycrystalline PbTe:In Films on Amorphous Substrate: Structure and Physical Properties
title_sort polycrystalline pbte:in films on amorphous substrate: structure and physical properties
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9736097/
https://www.ncbi.nlm.nih.gov/pubmed/36499879
http://dx.doi.org/10.3390/ma15238383
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