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Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators

[Image: see text] Optically active defects in 2D materials, such as hexagonal boron nitride (hBN) and transition-metal dichalcogenides (TMDs), are an attractive class of single-photon emitters with high brightness, operation up to room temperature, site-specific engineering of emitter arrays with st...

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Autores principales: Parto, K., Azzam, S. I., Lewis, N., Patel, S. D., Umezawa, S., Watanabe, K., Taniguchi, T., Moody, G.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9756340/
https://www.ncbi.nlm.nih.gov/pubmed/36318636
http://dx.doi.org/10.1021/acs.nanolett.2c03151
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author Parto, K.
Azzam, S. I.
Lewis, N.
Patel, S. D.
Umezawa, S.
Watanabe, K.
Taniguchi, T.
Moody, G.
author_facet Parto, K.
Azzam, S. I.
Lewis, N.
Patel, S. D.
Umezawa, S.
Watanabe, K.
Taniguchi, T.
Moody, G.
author_sort Parto, K.
collection PubMed
description [Image: see text] Optically active defects in 2D materials, such as hexagonal boron nitride (hBN) and transition-metal dichalcogenides (TMDs), are an attractive class of single-photon emitters with high brightness, operation up to room temperature, site-specific engineering of emitter arrays with strain and irradiation techniques, and tunability with external electric fields. In this work, we demonstrate a novel approach to precisely align and embed hBN and TMDs within background-free silicon nitride microring resonators. Through the Purcell effect, high-purity hBN emitters exhibit a cavity-enhanced spectral coupling efficiency of up to 46% at room temperature, exceeding the theoretical limit (up to 40%) for cavity-free waveguide-emitter coupling and demonstrating nearly a 1 order of magnitude improvement over previous work. The devices are fabricated with a CMOS-compatible process and exhibit no degradation of the 2D material optical properties, robustness to thermal annealing, and 100 nm positioning accuracy of quantum emitters within single-mode waveguides, opening a path for scalable quantum photonic chips with on-demand single-photon sources.
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spelling pubmed-97563402022-12-17 Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators Parto, K. Azzam, S. I. Lewis, N. Patel, S. D. Umezawa, S. Watanabe, K. Taniguchi, T. Moody, G. Nano Lett [Image: see text] Optically active defects in 2D materials, such as hexagonal boron nitride (hBN) and transition-metal dichalcogenides (TMDs), are an attractive class of single-photon emitters with high brightness, operation up to room temperature, site-specific engineering of emitter arrays with strain and irradiation techniques, and tunability with external electric fields. In this work, we demonstrate a novel approach to precisely align and embed hBN and TMDs within background-free silicon nitride microring resonators. Through the Purcell effect, high-purity hBN emitters exhibit a cavity-enhanced spectral coupling efficiency of up to 46% at room temperature, exceeding the theoretical limit (up to 40%) for cavity-free waveguide-emitter coupling and demonstrating nearly a 1 order of magnitude improvement over previous work. The devices are fabricated with a CMOS-compatible process and exhibit no degradation of the 2D material optical properties, robustness to thermal annealing, and 100 nm positioning accuracy of quantum emitters within single-mode waveguides, opening a path for scalable quantum photonic chips with on-demand single-photon sources. American Chemical Society 2022-11-01 2022-12-14 /pmc/articles/PMC9756340/ /pubmed/36318636 http://dx.doi.org/10.1021/acs.nanolett.2c03151 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Parto, K.
Azzam, S. I.
Lewis, N.
Patel, S. D.
Umezawa, S.
Watanabe, K.
Taniguchi, T.
Moody, G.
Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators
title Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators
title_full Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators
title_fullStr Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators
title_full_unstemmed Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators
title_short Cavity-Enhanced 2D Material Quantum Emitters Deterministically Integrated with Silicon Nitride Microresonators
title_sort cavity-enhanced 2d material quantum emitters deterministically integrated with silicon nitride microresonators
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9756340/
https://www.ncbi.nlm.nih.gov/pubmed/36318636
http://dx.doi.org/10.1021/acs.nanolett.2c03151
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