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A Global‐Scale Mineral Dust Equation

A robust method to estimate mineral dust mass in ambient particulate matter (PM) is essential, as the dust fraction cannot be directly measured but is needed to understand dust impacts on the environment and human health. In this study, a global‐scale dust equation is developed that builds on the wi...

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Autores principales: Liu, Xuan, Turner, Jay R., Hand, Jenny L., Schichtel, Bret A., Martin, Randall V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9787586/
https://www.ncbi.nlm.nih.gov/pubmed/36591339
http://dx.doi.org/10.1029/2022JD036937
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author Liu, Xuan
Turner, Jay R.
Hand, Jenny L.
Schichtel, Bret A.
Martin, Randall V.
author_facet Liu, Xuan
Turner, Jay R.
Hand, Jenny L.
Schichtel, Bret A.
Martin, Randall V.
author_sort Liu, Xuan
collection PubMed
description A robust method to estimate mineral dust mass in ambient particulate matter (PM) is essential, as the dust fraction cannot be directly measured but is needed to understand dust impacts on the environment and human health. In this study, a global‐scale dust equation is developed that builds on the widely used Interagency Monitoring of Protected Visual Environments (IMPROVE) network's “soil” formula that is based on five measured elements (Al, Si, Ca, Fe, and Ti). We incorporate K, Mg, and Na into the equation using the mineral‐to‐aluminum (MAL) mass ratio of (K(2)O + MgO + Na(2)O)/Al(2)O(3) and apply a correction factor (CF) to account for other missing compounds. We obtain region‐specific MAL ratios and CFs by investigating the variation in dust composition across desert regions. To calculate reference dust mass for equation evaluation, we use total‐mineral‐mass (summing all oxides of crustal elements) and residual‐mass (subtracting non‐dust species from total PM) approaches. For desert dust in source regions, the normalized mean bias (NMB) of the global equation (within ±1%) is significantly smaller than the NMB of the IMPROVE equation (−6% to 10%). For PM(2.5) with high dust content measured by the IMPROVE network, the global equation estimates dust mass well (NMB within ±5%) at most sites. For desert dust transported to non‐source regions, the global equation still performs well (NMB within ±2%). The global equation can also represent paved road, unpaved road, and agricultural soil dust (NMB within ±5%). This global equation provides a promising approach for calculating dust mass based on elemental analysis of dust.
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spelling pubmed-97875862022-12-28 A Global‐Scale Mineral Dust Equation Liu, Xuan Turner, Jay R. Hand, Jenny L. Schichtel, Bret A. Martin, Randall V. J Geophys Res Atmos Research Article A robust method to estimate mineral dust mass in ambient particulate matter (PM) is essential, as the dust fraction cannot be directly measured but is needed to understand dust impacts on the environment and human health. In this study, a global‐scale dust equation is developed that builds on the widely used Interagency Monitoring of Protected Visual Environments (IMPROVE) network's “soil” formula that is based on five measured elements (Al, Si, Ca, Fe, and Ti). We incorporate K, Mg, and Na into the equation using the mineral‐to‐aluminum (MAL) mass ratio of (K(2)O + MgO + Na(2)O)/Al(2)O(3) and apply a correction factor (CF) to account for other missing compounds. We obtain region‐specific MAL ratios and CFs by investigating the variation in dust composition across desert regions. To calculate reference dust mass for equation evaluation, we use total‐mineral‐mass (summing all oxides of crustal elements) and residual‐mass (subtracting non‐dust species from total PM) approaches. For desert dust in source regions, the normalized mean bias (NMB) of the global equation (within ±1%) is significantly smaller than the NMB of the IMPROVE equation (−6% to 10%). For PM(2.5) with high dust content measured by the IMPROVE network, the global equation estimates dust mass well (NMB within ±5%) at most sites. For desert dust transported to non‐source regions, the global equation still performs well (NMB within ±2%). The global equation can also represent paved road, unpaved road, and agricultural soil dust (NMB within ±5%). This global equation provides a promising approach for calculating dust mass based on elemental analysis of dust. John Wiley and Sons Inc. 2022-09-26 2022-09-27 /pmc/articles/PMC9787586/ /pubmed/36591339 http://dx.doi.org/10.1029/2022JD036937 Text en © 2022 The Authors. This article has been contributed to by U.S. Government employees and their work is in the public domain in the USA. https://creativecommons.org/licenses/by-nc-nd/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc-nd/4.0/ (https://creativecommons.org/licenses/by-nc-nd/4.0/) License, which permits use and distribution in any medium, provided the original work is properly cited, the use is non‐commercial and no modifications or adaptations are made.
spellingShingle Research Article
Liu, Xuan
Turner, Jay R.
Hand, Jenny L.
Schichtel, Bret A.
Martin, Randall V.
A Global‐Scale Mineral Dust Equation
title A Global‐Scale Mineral Dust Equation
title_full A Global‐Scale Mineral Dust Equation
title_fullStr A Global‐Scale Mineral Dust Equation
title_full_unstemmed A Global‐Scale Mineral Dust Equation
title_short A Global‐Scale Mineral Dust Equation
title_sort global‐scale mineral dust equation
topic Research Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9787586/
https://www.ncbi.nlm.nih.gov/pubmed/36591339
http://dx.doi.org/10.1029/2022JD036937
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