Cargando…
Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China
This study investigated the effects of low molecular weight organic acids (citric acid and malic acid) on the migration properties of nickel in soil. A reclaimed soil sample was obtained from the Panyi Mine in Huainan City, China. The effects of adding different concentrations of Ni, citric acid (CA...
Autores principales: | , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9788445/ https://www.ncbi.nlm.nih.gov/pubmed/36548631 http://dx.doi.org/10.3390/toxics10120798 |
_version_ | 1784858756157276160 |
---|---|
author | Zheng, Yonghong Lu, Jiangwei Zhang, Zhiguo Li, Yating Tan, Yuning Cai, Weiqing Ma, Chengnan Chen, Fangling |
author_facet | Zheng, Yonghong Lu, Jiangwei Zhang, Zhiguo Li, Yating Tan, Yuning Cai, Weiqing Ma, Chengnan Chen, Fangling |
author_sort | Zheng, Yonghong |
collection | PubMed |
description | This study investigated the effects of low molecular weight organic acids (citric acid and malic acid) on the migration properties of nickel in soil. A reclaimed soil sample was obtained from the Panyi Mine in Huainan City, China. The effects of adding different concentrations of Ni, citric acid (CA) and malic acid (MA) were assessed on the migration and transformation of soil Ni forms. The results showed: (1) An increase in soil Ni activity with increasing Ni concentrations. (2) An increased proportion of exchangeable forms of Ni in soil with increased malic acid and citric acid concentrations, effectively promoting Ni mobility. In addition, the active Ni fraction in reclaimed soil increased significantly with increasing concentrations of citric and malic acid. The nickel activation effect of citric acid was found to be higher than that of malic acid. (3) The activation effect of organic acids on Ni weakened with aging, exhibiting a gradual transformation from the loosely bound form of Ni, to the strongly bound form. The results of this study provide a theoretical basis for improving the effectiveness and efficiency of the phytoremediation techniques used for the treatment of Ni-polluted soils. |
format | Online Article Text |
id | pubmed-9788445 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-97884452022-12-24 Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China Zheng, Yonghong Lu, Jiangwei Zhang, Zhiguo Li, Yating Tan, Yuning Cai, Weiqing Ma, Chengnan Chen, Fangling Toxics Article This study investigated the effects of low molecular weight organic acids (citric acid and malic acid) on the migration properties of nickel in soil. A reclaimed soil sample was obtained from the Panyi Mine in Huainan City, China. The effects of adding different concentrations of Ni, citric acid (CA) and malic acid (MA) were assessed on the migration and transformation of soil Ni forms. The results showed: (1) An increase in soil Ni activity with increasing Ni concentrations. (2) An increased proportion of exchangeable forms of Ni in soil with increased malic acid and citric acid concentrations, effectively promoting Ni mobility. In addition, the active Ni fraction in reclaimed soil increased significantly with increasing concentrations of citric and malic acid. The nickel activation effect of citric acid was found to be higher than that of malic acid. (3) The activation effect of organic acids on Ni weakened with aging, exhibiting a gradual transformation from the loosely bound form of Ni, to the strongly bound form. The results of this study provide a theoretical basis for improving the effectiveness and efficiency of the phytoremediation techniques used for the treatment of Ni-polluted soils. MDPI 2022-12-19 /pmc/articles/PMC9788445/ /pubmed/36548631 http://dx.doi.org/10.3390/toxics10120798 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Zheng, Yonghong Lu, Jiangwei Zhang, Zhiguo Li, Yating Tan, Yuning Cai, Weiqing Ma, Chengnan Chen, Fangling Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China |
title | Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China |
title_full | Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China |
title_fullStr | Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China |
title_full_unstemmed | Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China |
title_short | Effect of Low-Molecular Organic Acids on the Migration Characteristics of Nickel in Reclaimed Soil from The Panyi Mine Area in China |
title_sort | effect of low-molecular organic acids on the migration characteristics of nickel in reclaimed soil from the panyi mine area in china |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9788445/ https://www.ncbi.nlm.nih.gov/pubmed/36548631 http://dx.doi.org/10.3390/toxics10120798 |
work_keys_str_mv | AT zhengyonghong effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT lujiangwei effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT zhangzhiguo effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT liyating effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT tanyuning effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT caiweiqing effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT machengnan effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina AT chenfangling effectoflowmolecularorganicacidsonthemigrationcharacteristicsofnickelinreclaimedsoilfromthepanyimineareainchina |