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Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs

This paper proposes a novel LED-assisted deposition of platinum nanoparticles on the titania surface. For the first time, this process was supported by a UV-LED solution. We used two light sources with different wavelengths (λ(max) = 365 and 395 nm), and power (P = 1, 5, and 10 W) because the photod...

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Autores principales: Kubiak, Adam, Varma, Naisargi, Sikorski, Marek
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9800554/
https://www.ncbi.nlm.nih.gov/pubmed/36581762
http://dx.doi.org/10.1038/s41598-022-27232-5
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author Kubiak, Adam
Varma, Naisargi
Sikorski, Marek
author_facet Kubiak, Adam
Varma, Naisargi
Sikorski, Marek
author_sort Kubiak, Adam
collection PubMed
description This paper proposes a novel LED-assisted deposition of platinum nanoparticles on the titania surface. For the first time, this process was supported by a UV-LED solution. We used two light sources with different wavelengths (λ(max) = 365 and 395 nm), and power (P = 1, 5, and 10 W) because the photodeposition process based on LEDs has not been defined. The TiO(2)–Pt material was discovered to be nano-crystalline anatase particles with nano-platinum particles deposited on the surface of titanium dioxide. Furthermore, the luminescence intensity decreased when Pt was added to TiO(2), indicating that charge carrier recombination was reduced. The spectra matching of the photocatalyst and LED reactor was performed for the first time in this work. We proposed a convenient LED reactor that focused light in the range of 350–450 nm, allowing us to effectively use photo-oxidative properties of TiO(2)–Pt materials in the process of removing 4-chlorophenol. In the presented work, the LED light source plays a dual role. They first induce the platinum photodeposition process, before becoming an important component of tailored photoreactors, which is an important innovative aspect of this research.
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spelling pubmed-98005542022-12-31 Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs Kubiak, Adam Varma, Naisargi Sikorski, Marek Sci Rep Article This paper proposes a novel LED-assisted deposition of platinum nanoparticles on the titania surface. For the first time, this process was supported by a UV-LED solution. We used two light sources with different wavelengths (λ(max) = 365 and 395 nm), and power (P = 1, 5, and 10 W) because the photodeposition process based on LEDs has not been defined. The TiO(2)–Pt material was discovered to be nano-crystalline anatase particles with nano-platinum particles deposited on the surface of titanium dioxide. Furthermore, the luminescence intensity decreased when Pt was added to TiO(2), indicating that charge carrier recombination was reduced. The spectra matching of the photocatalyst and LED reactor was performed for the first time in this work. We proposed a convenient LED reactor that focused light in the range of 350–450 nm, allowing us to effectively use photo-oxidative properties of TiO(2)–Pt materials in the process of removing 4-chlorophenol. In the presented work, the LED light source plays a dual role. They first induce the platinum photodeposition process, before becoming an important component of tailored photoreactors, which is an important innovative aspect of this research. Nature Publishing Group UK 2022-12-29 /pmc/articles/PMC9800554/ /pubmed/36581762 http://dx.doi.org/10.1038/s41598-022-27232-5 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Kubiak, Adam
Varma, Naisargi
Sikorski, Marek
Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs
title Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs
title_full Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs
title_fullStr Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs
title_full_unstemmed Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs
title_short Insight into the LED-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of LEDs
title_sort insight into the led-assisted deposition of platinum nanoparticles on the titania surface: understanding the effect of leds
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9800554/
https://www.ncbi.nlm.nih.gov/pubmed/36581762
http://dx.doi.org/10.1038/s41598-022-27232-5
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