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Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants

In recent years, photocatalytic reactions have shown great potential in degrading organic pollutants because of their simple operation and no secondary pollution. Graphitic carbon nitride (g-C(3)N(4)) is one of the most frequently used photocatalyst materials in the field of photocatalysis because i...

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Autores principales: Gu, Yaohua, Li, Siao, Li, Mingming, Wang, Xinyu, Liu, Ying, Shi, Keren, Bai, Xiaoyan, Yao, Qing, Wu, Zhiqiang, Yao, Huiqin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9811494/
https://www.ncbi.nlm.nih.gov/pubmed/36686928
http://dx.doi.org/10.1039/d2ra06994f
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author Gu, Yaohua
Li, Siao
Li, Mingming
Wang, Xinyu
Liu, Ying
Shi, Keren
Bai, Xiaoyan
Yao, Qing
Wu, Zhiqiang
Yao, Huiqin
author_facet Gu, Yaohua
Li, Siao
Li, Mingming
Wang, Xinyu
Liu, Ying
Shi, Keren
Bai, Xiaoyan
Yao, Qing
Wu, Zhiqiang
Yao, Huiqin
author_sort Gu, Yaohua
collection PubMed
description In recent years, photocatalytic reactions have shown great potential in degrading organic pollutants because of their simple operation and no secondary pollution. Graphitic carbon nitride (g-C(3)N(4)) is one of the most frequently used photocatalyst materials in the field of photocatalysis because it is a form of photocatalytic material with facile synthesis, no metal, visible light response, and strong stability. Enzyme-catalyzed degradation has received extensive attention due to its broad selectivity, high efficiency, and environmental friendliness. Horseradish peroxidase (HRP), one of several oxidoreductases utilized for pollutant degradation, has a wide range of applications due to its mild reaction conditions and high stability. Exploring efficient platforms for immobilizing g-C(3)N(4) and HRP to develop photo-enzyme-coupled catalysis is an attractive practical topic. The coupling effect of g-C(3)N(4) and HRP improves the carrier separation efficiency and generates more active species, which finally realize the solar-driven non-selective destruction of organic pollutants. We describe the alteration of g-C(3)N(4) and the immobilization of HRP in detail in this study, and we outline recent developments in the photo-enzyme coupling of g-C(3)N(4) and HRP.
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spelling pubmed-98114942023-01-20 Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants Gu, Yaohua Li, Siao Li, Mingming Wang, Xinyu Liu, Ying Shi, Keren Bai, Xiaoyan Yao, Qing Wu, Zhiqiang Yao, Huiqin RSC Adv Chemistry In recent years, photocatalytic reactions have shown great potential in degrading organic pollutants because of their simple operation and no secondary pollution. Graphitic carbon nitride (g-C(3)N(4)) is one of the most frequently used photocatalyst materials in the field of photocatalysis because it is a form of photocatalytic material with facile synthesis, no metal, visible light response, and strong stability. Enzyme-catalyzed degradation has received extensive attention due to its broad selectivity, high efficiency, and environmental friendliness. Horseradish peroxidase (HRP), one of several oxidoreductases utilized for pollutant degradation, has a wide range of applications due to its mild reaction conditions and high stability. Exploring efficient platforms for immobilizing g-C(3)N(4) and HRP to develop photo-enzyme-coupled catalysis is an attractive practical topic. The coupling effect of g-C(3)N(4) and HRP improves the carrier separation efficiency and generates more active species, which finally realize the solar-driven non-selective destruction of organic pollutants. We describe the alteration of g-C(3)N(4) and the immobilization of HRP in detail in this study, and we outline recent developments in the photo-enzyme coupling of g-C(3)N(4) and HRP. The Royal Society of Chemistry 2023-01-04 /pmc/articles/PMC9811494/ /pubmed/36686928 http://dx.doi.org/10.1039/d2ra06994f Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Gu, Yaohua
Li, Siao
Li, Mingming
Wang, Xinyu
Liu, Ying
Shi, Keren
Bai, Xiaoyan
Yao, Qing
Wu, Zhiqiang
Yao, Huiqin
Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants
title Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants
title_full Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants
title_fullStr Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants
title_full_unstemmed Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants
title_short Recent advances in g-C(3)N(4)-based photo-enzyme catalysts for degrading organic pollutants
title_sort recent advances in g-c(3)n(4)-based photo-enzyme catalysts for degrading organic pollutants
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9811494/
https://www.ncbi.nlm.nih.gov/pubmed/36686928
http://dx.doi.org/10.1039/d2ra06994f
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