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Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant

One of the main environmental impacts of amine-based carbon capture processes is the emission of the solvent into the atmosphere. To understand how these emissions are affected by the intermittent operation of a power plant, we performed stress tests on a plant operating with a mixture of two amines...

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Autores principales: Jablonka, Kevin Maik, Charalambous, Charithea, Sanchez Fernandez, Eva, Wiechers, Georg, Monteiro, Juliana, Moser, Peter, Smit, Berend, Garcia, Susana
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9812371/
https://www.ncbi.nlm.nih.gov/pubmed/36598993
http://dx.doi.org/10.1126/sciadv.adc9576
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author Jablonka, Kevin Maik
Charalambous, Charithea
Sanchez Fernandez, Eva
Wiechers, Georg
Monteiro, Juliana
Moser, Peter
Smit, Berend
Garcia, Susana
author_facet Jablonka, Kevin Maik
Charalambous, Charithea
Sanchez Fernandez, Eva
Wiechers, Georg
Monteiro, Juliana
Moser, Peter
Smit, Berend
Garcia, Susana
author_sort Jablonka, Kevin Maik
collection PubMed
description One of the main environmental impacts of amine-based carbon capture processes is the emission of the solvent into the atmosphere. To understand how these emissions are affected by the intermittent operation of a power plant, we performed stress tests on a plant operating with a mixture of two amines, 2-amino-2-methyl-1-propanol and piperazine (CESAR1). To forecast the emissions and model the impact of interventions, we developed a machine learning model. Our model showed that some interventions have opposite effects on the emissions of the components of the solvent. Thus, mitigation strategies required for capture plants operating on a single component solvent (e.g., monoethanolamine) need to be reconsidered if operated using a mixture of amines. Amine emissions from a solvent-based carbon capture plant are an example of a process that is too complex to be described by conventional process models. We, therefore, expect that our approach can be more generally applied.
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spelling pubmed-98123712023-01-10 Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant Jablonka, Kevin Maik Charalambous, Charithea Sanchez Fernandez, Eva Wiechers, Georg Monteiro, Juliana Moser, Peter Smit, Berend Garcia, Susana Sci Adv Physical and Materials Sciences One of the main environmental impacts of amine-based carbon capture processes is the emission of the solvent into the atmosphere. To understand how these emissions are affected by the intermittent operation of a power plant, we performed stress tests on a plant operating with a mixture of two amines, 2-amino-2-methyl-1-propanol and piperazine (CESAR1). To forecast the emissions and model the impact of interventions, we developed a machine learning model. Our model showed that some interventions have opposite effects on the emissions of the components of the solvent. Thus, mitigation strategies required for capture plants operating on a single component solvent (e.g., monoethanolamine) need to be reconsidered if operated using a mixture of amines. Amine emissions from a solvent-based carbon capture plant are an example of a process that is too complex to be described by conventional process models. We, therefore, expect that our approach can be more generally applied. American Association for the Advancement of Science 2023-01-04 /pmc/articles/PMC9812371/ /pubmed/36598993 http://dx.doi.org/10.1126/sciadv.adc9576 Text en Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Jablonka, Kevin Maik
Charalambous, Charithea
Sanchez Fernandez, Eva
Wiechers, Georg
Monteiro, Juliana
Moser, Peter
Smit, Berend
Garcia, Susana
Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant
title Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant
title_full Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant
title_fullStr Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant
title_full_unstemmed Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant
title_short Machine learning for industrial processes: Forecasting amine emissions from a carbon capture plant
title_sort machine learning for industrial processes: forecasting amine emissions from a carbon capture plant
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9812371/
https://www.ncbi.nlm.nih.gov/pubmed/36598993
http://dx.doi.org/10.1126/sciadv.adc9576
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