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Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes

Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substitut...

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Autores principales: Long, Tianyu, Zhu, Chen, Li, Ling, Shao, Liang, Zhu, Shengqing, Rueping, Magnus, Chu, Lingling
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9813127/
https://www.ncbi.nlm.nih.gov/pubmed/36599820
http://dx.doi.org/10.1038/s41467-022-35688-2
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author Long, Tianyu
Zhu, Chen
Li, Ling
Shao, Liang
Zhu, Shengqing
Rueping, Magnus
Chu, Lingling
author_facet Long, Tianyu
Zhu, Chen
Li, Ling
Shao, Liang
Zhu, Shengqing
Rueping, Magnus
Chu, Lingling
author_sort Long, Tianyu
collection PubMed
description Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substituted 1,3-dienes from common substrates remains underexploited. Here, we report a photoredox and nickel dual catalytic strategy for the stereodivergent sulfonylalkenylation of terminal alkynes with vinyl triflates and sodium sulfinates under mild conditions. With a judicious choice of simple nickel catalyst and ligand, this method enables efficient and divergent access to both Z- and E-sulfonyl-1,3-dienes from the same set of simple starting materials. This method features broad substrate scope, good functional compatibility, and excellent chemo-, regio-, and stereoselectivity. Experimental and DFT mechanistic studies offer insights into the observed divergent stereoselectivity controlled by ligands.
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spelling pubmed-98131272023-01-06 Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes Long, Tianyu Zhu, Chen Li, Ling Shao, Liang Zhu, Shengqing Rueping, Magnus Chu, Lingling Nat Commun Article Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substituted 1,3-dienes from common substrates remains underexploited. Here, we report a photoredox and nickel dual catalytic strategy for the stereodivergent sulfonylalkenylation of terminal alkynes with vinyl triflates and sodium sulfinates under mild conditions. With a judicious choice of simple nickel catalyst and ligand, this method enables efficient and divergent access to both Z- and E-sulfonyl-1,3-dienes from the same set of simple starting materials. This method features broad substrate scope, good functional compatibility, and excellent chemo-, regio-, and stereoselectivity. Experimental and DFT mechanistic studies offer insights into the observed divergent stereoselectivity controlled by ligands. Nature Publishing Group UK 2023-01-04 /pmc/articles/PMC9813127/ /pubmed/36599820 http://dx.doi.org/10.1038/s41467-022-35688-2 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Long, Tianyu
Zhu, Chen
Li, Ling
Shao, Liang
Zhu, Shengqing
Rueping, Magnus
Chu, Lingling
Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
title Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
title_full Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
title_fullStr Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
title_full_unstemmed Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
title_short Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
title_sort ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9813127/
https://www.ncbi.nlm.nih.gov/pubmed/36599820
http://dx.doi.org/10.1038/s41467-022-35688-2
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