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Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substitut...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9813127/ https://www.ncbi.nlm.nih.gov/pubmed/36599820 http://dx.doi.org/10.1038/s41467-022-35688-2 |
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author | Long, Tianyu Zhu, Chen Li, Ling Shao, Liang Zhu, Shengqing Rueping, Magnus Chu, Lingling |
author_facet | Long, Tianyu Zhu, Chen Li, Ling Shao, Liang Zhu, Shengqing Rueping, Magnus Chu, Lingling |
author_sort | Long, Tianyu |
collection | PubMed |
description | Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substituted 1,3-dienes from common substrates remains underexploited. Here, we report a photoredox and nickel dual catalytic strategy for the stereodivergent sulfonylalkenylation of terminal alkynes with vinyl triflates and sodium sulfinates under mild conditions. With a judicious choice of simple nickel catalyst and ligand, this method enables efficient and divergent access to both Z- and E-sulfonyl-1,3-dienes from the same set of simple starting materials. This method features broad substrate scope, good functional compatibility, and excellent chemo-, regio-, and stereoselectivity. Experimental and DFT mechanistic studies offer insights into the observed divergent stereoselectivity controlled by ligands. |
format | Online Article Text |
id | pubmed-9813127 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-98131272023-01-06 Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes Long, Tianyu Zhu, Chen Li, Ling Shao, Liang Zhu, Shengqing Rueping, Magnus Chu, Lingling Nat Commun Article Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substituted 1,3-dienes from common substrates remains underexploited. Here, we report a photoredox and nickel dual catalytic strategy for the stereodivergent sulfonylalkenylation of terminal alkynes with vinyl triflates and sodium sulfinates under mild conditions. With a judicious choice of simple nickel catalyst and ligand, this method enables efficient and divergent access to both Z- and E-sulfonyl-1,3-dienes from the same set of simple starting materials. This method features broad substrate scope, good functional compatibility, and excellent chemo-, regio-, and stereoselectivity. Experimental and DFT mechanistic studies offer insights into the observed divergent stereoselectivity controlled by ligands. Nature Publishing Group UK 2023-01-04 /pmc/articles/PMC9813127/ /pubmed/36599820 http://dx.doi.org/10.1038/s41467-022-35688-2 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Long, Tianyu Zhu, Chen Li, Ling Shao, Liang Zhu, Shengqing Rueping, Magnus Chu, Lingling Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
title | Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
title_full | Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
title_fullStr | Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
title_full_unstemmed | Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
title_short | Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
title_sort | ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9813127/ https://www.ncbi.nlm.nih.gov/pubmed/36599820 http://dx.doi.org/10.1038/s41467-022-35688-2 |
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