Cargando…

New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide

Transition metal dichalcogenide (TMD) semiconductors are two-dimensional materials with great potential for the future of nano-optics and nano-optoelectronics as well as the rich and exciting development of basic research. The influence of an external magnetic field on a TMD monolayer raises a new q...

Descripción completa

Detalles Bibliográficos
Autores principales: Trallero-Giner, Carlos, Santiago-Pérez, Darío G., Fomin, Vladimir M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9822968/
https://www.ncbi.nlm.nih.gov/pubmed/36609670
http://dx.doi.org/10.1038/s41598-023-27404-x
_version_ 1784866053715656704
author Trallero-Giner, Carlos
Santiago-Pérez, Darío G.
Fomin, Vladimir M.
author_facet Trallero-Giner, Carlos
Santiago-Pérez, Darío G.
Fomin, Vladimir M.
author_sort Trallero-Giner, Carlos
collection PubMed
description Transition metal dichalcogenide (TMD) semiconductors are two-dimensional materials with great potential for the future of nano-optics and nano-optoelectronics as well as the rich and exciting development of basic research. The influence of an external magnetic field on a TMD monolayer raises a new question: to unveil the behavior of the magneto-polaron resonances (MPRs) associated with the phonon symmetry inherent in the system. It is shown that the renormalized Landau energy levels are modified by the interplay of the long-range Pekar–Fröhlich (PF) and short-range deformation potential (DP) interactions. This leads to a new series of MPRs involving the optical phonons at the center of the Brillouin zone. The coupling of the two Landau levels with the LO and [Formula: see text] optical phonon modes provokes resonant splittings of double avoided-crossing levels giving rise to three excitation branches. This effect appears as bigger energy gaps at the anticrossing points in the renormalized Landau levels. To explore the interplay between the MPRs, the electron-phonon interactions (PF and DP) and the couplings between adjacent Landau levels, a full Green’s function treatment for the evaluation of the energy and its life-time broadening is developed. A generalization of the two-level approach is performed for the description of the new MPR branches. The obtained results are a guideline for the magneto-optical experiments in TMDs, where three MPR peaks should be observable.
format Online
Article
Text
id pubmed-9822968
institution National Center for Biotechnology Information
language English
publishDate 2023
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-98229682023-01-08 New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide Trallero-Giner, Carlos Santiago-Pérez, Darío G. Fomin, Vladimir M. Sci Rep Article Transition metal dichalcogenide (TMD) semiconductors are two-dimensional materials with great potential for the future of nano-optics and nano-optoelectronics as well as the rich and exciting development of basic research. The influence of an external magnetic field on a TMD monolayer raises a new question: to unveil the behavior of the magneto-polaron resonances (MPRs) associated with the phonon symmetry inherent in the system. It is shown that the renormalized Landau energy levels are modified by the interplay of the long-range Pekar–Fröhlich (PF) and short-range deformation potential (DP) interactions. This leads to a new series of MPRs involving the optical phonons at the center of the Brillouin zone. The coupling of the two Landau levels with the LO and [Formula: see text] optical phonon modes provokes resonant splittings of double avoided-crossing levels giving rise to three excitation branches. This effect appears as bigger energy gaps at the anticrossing points in the renormalized Landau levels. To explore the interplay between the MPRs, the electron-phonon interactions (PF and DP) and the couplings between adjacent Landau levels, a full Green’s function treatment for the evaluation of the energy and its life-time broadening is developed. A generalization of the two-level approach is performed for the description of the new MPR branches. The obtained results are a guideline for the magneto-optical experiments in TMDs, where three MPR peaks should be observable. Nature Publishing Group UK 2023-01-06 /pmc/articles/PMC9822968/ /pubmed/36609670 http://dx.doi.org/10.1038/s41598-023-27404-x Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Trallero-Giner, Carlos
Santiago-Pérez, Darío G.
Fomin, Vladimir M.
New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
title New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
title_full New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
title_fullStr New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
title_full_unstemmed New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
title_short New magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
title_sort new magneto-polaron resonances in a monolayer of a transition metal dichalcogenide
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9822968/
https://www.ncbi.nlm.nih.gov/pubmed/36609670
http://dx.doi.org/10.1038/s41598-023-27404-x
work_keys_str_mv AT tralleroginercarlos newmagnetopolaronresonancesinamonolayerofatransitionmetaldichalcogenide
AT santiagoperezdariog newmagnetopolaronresonancesinamonolayerofatransitionmetaldichalcogenide
AT fominvladimirm newmagnetopolaronresonancesinamonolayerofatransitionmetaldichalcogenide