Cargando…

Shedding Light on the Enigmatic TcO(2) ⋅ xH(2)O Structure with Density Functional Theory and EXAFS Spectroscopy

The β‐emitting (99)Tc isotope is a high‐yield fission product in (235)U and (239)Pu nuclear reactors, raising special concern in nuclear waste management due to its long half‐life and the high mobility of pertechnetate (TcO(4) (−)). Under the conditions of deep nuclear waste repositories, Tc is reta...

Descripción completa

Detalles Bibliográficos
Autores principales:	Oliveira, Augusto F., Kuc, Agnieszka, Heine, Thomas, Abram, Ulrich, Scheinost, Andreas C.
Formato:	Online Artículo Texto
Lenguaje:	English
Publicado:	John Wiley and Sons Inc. 2022
Materias:	Research Articles
Acceso en línea:	https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9826482/ https://www.ncbi.nlm.nih.gov/pubmed/36053144 http://dx.doi.org/10.1002/chem.202202235

Ejemplares similares

trans-K(3)[TcO(2)(CN)(4)]
por: Chatterjee, Sayandev, et al.
Publicado: (2010)

(99)TcO(4)(−) remediation by a cationic polymeric network
por: Li, Jie, et al.
Publicado: (2018)

Anion-adaptive crystalline cationic material for (99)TcO(4)(−) trapping
por: Mei, Lei, et al.
Publicado: (2019)

Highly Efficient Uptake of TcO(4)(–) by Imidazolium-Functionalized Wood Sawdust
por: Dong, Fangfei, et al.
Publicado: (2021)

Hyperthyroidism secondary to disseminated differentiated thyroid cancer on (99m)TcO(4) scan
por: Hu, Yan, et al.
Publicado: (2019)

(99m)TcO(4)(-)/(99m)Tc-MIBI dual-tracer scintigraphy for preoperative localization of parathyroid adenomas
por: Huang, Zhongke, et al.
Publicado: (2018)

Reaction of Pertechnetate in Highly Alkaline Solution: Synthesis and Characterization of the Nitridotrioxotechnetate Ba[TcO(3)N]
por: Badea, D., et al.
Publicado: (2022)

(99m)TcO(4) (−)-, Auger-Mediated Thyroid Stunning: Dosimetric Requirements and Associated Molecular Events
por: Cambien, Béatrice, et al.
Publicado: (2014)

Optimizing Strategy for Enhancing the Stability and (99)TcO(4)(–) Sequestration of Poly(ionic liquids)@MOFs Composites
por: Li, Cheng-Peng, et al.
Publicado: (2020)

Highly Selective Adsorption of (99)TcO(4)(−)/ReO(4)(−) by a Novel Polyamide-Functionalized Polyacrylamide Polymer Material
por: Qin, Ben, et al.
Publicado: (2022)

An ionic vinylene-linked three-dimensional covalent organic framework for selective and efficient trapping of ReO(4)(−) or (99)TcO(4)(−)
por: Zhang, Cheng-Rong, et al.
Publicado: (2022)

(99)TcO(4)(−) removal from legacy defense nuclear waste by an alkaline-stable 2D cationic metal organic framework
por: Shen, Nannan, et al.
Publicado: (2020)

(99m)TcO(4)(−) scintigraphic detection of follicular thyroid cancer and multiple metastatic lesions: A case report
por: WANG, CHANG-YIN, et al.
Publicado: (2013)

Primary accessory thyroid carcinoma with negative (99m)TcO(4)(−) SPECT/CTimaging: a case report and literature review
por: Ma, Yibo, et al.
Publicado: (2019)

Functional Carbon Capsules Supporting Ruthenium Nanoclusters for Efficient Electrocatalytic (99)TcO(4) (−)/ReO(4) (−) Removal from Acidic and Alkaline Nuclear Wastes
por: Liu, Xiaolu, et al.
Publicado: (2023)

Quick-EXAFS implementation on the general purpose EXAFS beamline at ESRF
por: Prestipino, Carmelo, et al.
Publicado: (2011)

Chemistry of the Interaction and Retention of Tc(VII) and Tc(IV) Species at the Fe(3)O(4)(001) Surface
por: Bianchetti, Enrico, et al.
Publicado: (2023)

Assembly of flexible CoMoO(4)@NiMoO(4)·xH(2)O and Fe(2)O(3) electrodes for solid-state asymmetric supercapacitors
por: Wang, Jing, et al.
Publicado: (2017)

Task-Specific Tailored Cationic Polymeric Network with High Base-Resistance for Unprecedented (99)TcO(4)(–) Cleanup from Alkaline Nuclear Waste
por: Li, Jie, et al.
Publicado: (2021)

Octahedral Tilting in Homologous Perovskite Series CaMoO3-SrMoO3-BaMoO3 Probed by Temperature-Dependent EXAFS Spectroscopy
por: Bakradze, Georgijs, et al.
Publicado: (2022)

A Coupled EXAFS–Molecular Dynamics Study on PuO(2)(+) and NpO(2)(+) Hydration: The Importance of Electron Correlation in Force-Field Building
por: Raposo-Hernández, Gema, et al.
Publicado: (2022)

Scalable Synthesis of Esp and Rhodium(II) Carboxylates from Acetylacetone and RhCl(3)·xH(2)O
por: Martínez-Castro, Elisa, et al.
Publicado: (2020)

Synthesis and detection the oxidization of Co cores of Co@SiO(2) core-shell nanoparticles by in situ XRD and EXAFS
por: Zhang, Kunhao, et al.
Publicado: (2015)

A new detector for sub-millisecond EXAFS spectroscopy at the European Synchrotron Radiation Facility
por: Kantor, Innokenty, et al.
Publicado: (2014)

3rd International EXAFS Conference
por: Hodgson, Keith, et al.
Publicado: (1984)

EXAFS and XANES analysis of oxides at the nanoscale
por: Kuzmin, Alexei, et al.
Publicado: (2014)

Dual XH–π Interaction of Hexafluoroisopropanol with Arenes
por: Lu, Le, et al.
Publicado: (2021)

Mechanism unravelling for highly efficient and selective (99)TcO(4)(−) sequestration utilising crown ether based solvent system from nuclear liquid waste: experimental and computational investigations
por: Patra, Kankan, et al.
Publicado: (2022)

NLRP1 activation by UVB: Shedding light on an enigmatic inflammasome
por: Sandstrom, Andrew
Publicado: (2022)

Mechanism unravelling for ultrafast and selective (99)TcO(4)(–) uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study
por: He, Linwei, et al.
Publicado: (2019)

Potential Applications of (68)Ga-PSMA-11 PET/CT in the Evaluation of Salivary Gland Uptake Function: Preliminary Observations and Comparison with (99m)TcO(4)(−) Salivary Gland Scintigraphy
por: Zhao, Yanhong, et al.
Publicado: (2020)

Correction: Mechanism unravelling for highly efficient and selective (99)TcO(4)(−) sequestration utilising crown ether based solvent system from nuclear liquid waste: experimental and computational investigations
por: Patra, Kankan, et al.
Publicado: (2022)

Novel Supercapacitor Electrode Derived from One Dimensional Cerium Hydrogen Phosphate (1D-Ce(HPO(4))(2).xH(2)O)
por: Yoon, Jong Hee, et al.
Publicado: (2022)

Correction: Mechanism unravelling for ultrafast and selective (99)TcO(4)(–) uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study
por: He, Linwei, et al.
Publicado: (2019)

An Enigmatic Stramenopile Sheds Light on Early Evolution in Ochrophyta Plastid Organellogenesis
por: Azuma, Tomonori, et al.
Publicado: (2022)

Aggregation tendency of guest Fe in NaCo(1−x)Fe(x)O(2) (x < 0.1) as investigated by systematic EXAFS analysis
por: Moriya, Toshiaki, et al.
Publicado: (2020)

O-acetylation of Gd3: An Enigmatic Modification Regulating Apoptosis?
por: Chen, Helen Y., et al.
Publicado: (2002)

Complete Genome Sequence of Streptococcus gallolyticus Strain XH2168
por: Yang, Siyuan, et al.
Publicado: (2023)

Proceedings of the International Conference on EXAFS and Near Edge Structure
por: Bianconi, Antonio, et al.
Publicado: (1983)

Ferric Chloride Complexes in Aqueous Solution: An EXAFS Study
por: Persson, Ingmar
Publicado: (2018)

Cannot write session to /tmp/vufind_sessions/sess_gjl4v9cjugocmqu87e376tek7m