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Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage

[Image: see text] The cost-effective biomass-derived carbon with high electrochemical performance is highly desirable for the sustainable development of advanced energy storage devices. In this manuscript, Typha angustifolia with a large output and loose porous characteristics was selected as the ra...

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Autores principales: Wang, Shuya, Mei, Yidong, Shao, Zishuo, Wang, Jingru, Tan, Zhenzhen, Qiu, Zurui, Wang, Minghao, Zheng, Hong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9835543/
https://www.ncbi.nlm.nih.gov/pubmed/36643506
http://dx.doi.org/10.1021/acsomega.2c06782
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author Wang, Shuya
Mei, Yidong
Shao, Zishuo
Wang, Jingru
Tan, Zhenzhen
Qiu, Zurui
Wang, Minghao
Zheng, Hong
author_facet Wang, Shuya
Mei, Yidong
Shao, Zishuo
Wang, Jingru
Tan, Zhenzhen
Qiu, Zurui
Wang, Minghao
Zheng, Hong
author_sort Wang, Shuya
collection PubMed
description [Image: see text] The cost-effective biomass-derived carbon with high electrochemical performance is highly desirable for the sustainable development of advanced energy storage devices. In this manuscript, Typha angustifolia with a large output and loose porous characteristics was selected as the raw material of biomass. In the synthesis process, KHCO(3), which is more environmentally friendly, is used as a pore-forming agent, and the low-cost, easy-to-clean fluxing agent NaCl is used to assist the pore-forming process. Based on the analysis of thermogravimetric-infrared test results, the calcination procedure of porous carbon was designed reasonably, so that the functions of the pore-forming agent and fluxing agent could be fully exerted. Its high electrochemical performance is attributed to combined contributions from high surface area and hierarchical porous structures. The as-prepared carbon also showed an outstanding capacitance of 317.2 F/g at a current density of 1 A g(–1) and a high capacitance retention of over 97.83% after 5000 cycles at a current density of 4 A g(–1). This work provides an outstanding renewable candidate and a feasible route design strategy for the fabrication of high-performance electrodes.
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spelling pubmed-98355432023-01-13 Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage Wang, Shuya Mei, Yidong Shao, Zishuo Wang, Jingru Tan, Zhenzhen Qiu, Zurui Wang, Minghao Zheng, Hong ACS Omega [Image: see text] The cost-effective biomass-derived carbon with high electrochemical performance is highly desirable for the sustainable development of advanced energy storage devices. In this manuscript, Typha angustifolia with a large output and loose porous characteristics was selected as the raw material of biomass. In the synthesis process, KHCO(3), which is more environmentally friendly, is used as a pore-forming agent, and the low-cost, easy-to-clean fluxing agent NaCl is used to assist the pore-forming process. Based on the analysis of thermogravimetric-infrared test results, the calcination procedure of porous carbon was designed reasonably, so that the functions of the pore-forming agent and fluxing agent could be fully exerted. Its high electrochemical performance is attributed to combined contributions from high surface area and hierarchical porous structures. The as-prepared carbon also showed an outstanding capacitance of 317.2 F/g at a current density of 1 A g(–1) and a high capacitance retention of over 97.83% after 5000 cycles at a current density of 4 A g(–1). This work provides an outstanding renewable candidate and a feasible route design strategy for the fabrication of high-performance electrodes. American Chemical Society 2022-12-23 /pmc/articles/PMC9835543/ /pubmed/36643506 http://dx.doi.org/10.1021/acsomega.2c06782 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Wang, Shuya
Mei, Yidong
Shao, Zishuo
Wang, Jingru
Tan, Zhenzhen
Qiu, Zurui
Wang, Minghao
Zheng, Hong
Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage
title Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage
title_full Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage
title_fullStr Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage
title_full_unstemmed Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage
title_short Biomass Hierarchical Porous Carbonized Typha angustifolia Prepared by Green Pore-Making Technology for Energy Storage
title_sort biomass hierarchical porous carbonized typha angustifolia prepared by green pore-making technology for energy storage
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9835543/
https://www.ncbi.nlm.nih.gov/pubmed/36643506
http://dx.doi.org/10.1021/acsomega.2c06782
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