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Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
The discovery of superconductivity in planar nickelates raises the question of how the electronic structure and correlations of Ni(1+) compounds compare to those of the Cu(2+) cuprate superconductors. Here, we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickela...
Autores principales: | , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9839319/ https://www.ncbi.nlm.nih.gov/pubmed/36638179 http://dx.doi.org/10.1126/sciadv.ade4418 |
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author | Li, Haoxiang Hao, Peipei Zhang, Junjie Gordon, Kyle Linn, A. Garrison Chen, Xinglong Zheng, Hong Zhou, Xiaoqing Mitchell, J. F. Dessau, D. S. |
author_facet | Li, Haoxiang Hao, Peipei Zhang, Junjie Gordon, Kyle Linn, A. Garrison Chen, Xinglong Zheng, Hong Zhou, Xiaoqing Mitchell, J. F. Dessau, D. S. |
author_sort | Li, Haoxiang |
collection | PubMed |
description | The discovery of superconductivity in planar nickelates raises the question of how the electronic structure and correlations of Ni(1+) compounds compare to those of the Cu(2+) cuprate superconductors. Here, we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickelate Pr(4)Ni(3)O(8), revealing a Fermi surface resembling that of the hole-doped cuprates but with critical differences. Specifically, the main portions of the Fermi surface are extremely similar to that of the bilayer cuprates, with an additional piece that can accommodate additional hole doping. We find that the electronic correlations are about twice as strong in the nickelates and are almost k-independent, indicating that they originate from a local effect, likely the Mott interaction, whereas cuprate interactions are somewhat less local. Nevertheless, the nickelates still demonstrate the strange-metal behavior in the electron scattering rates. Understanding the similarities and differences between these two families of strongly correlated superconductors is an important challenge. |
format | Online Article Text |
id | pubmed-9839319 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-98393192023-01-24 Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) Li, Haoxiang Hao, Peipei Zhang, Junjie Gordon, Kyle Linn, A. Garrison Chen, Xinglong Zheng, Hong Zhou, Xiaoqing Mitchell, J. F. Dessau, D. S. Sci Adv Physical and Materials Sciences The discovery of superconductivity in planar nickelates raises the question of how the electronic structure and correlations of Ni(1+) compounds compare to those of the Cu(2+) cuprate superconductors. Here, we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickelate Pr(4)Ni(3)O(8), revealing a Fermi surface resembling that of the hole-doped cuprates but with critical differences. Specifically, the main portions of the Fermi surface are extremely similar to that of the bilayer cuprates, with an additional piece that can accommodate additional hole doping. We find that the electronic correlations are about twice as strong in the nickelates and are almost k-independent, indicating that they originate from a local effect, likely the Mott interaction, whereas cuprate interactions are somewhat less local. Nevertheless, the nickelates still demonstrate the strange-metal behavior in the electron scattering rates. Understanding the similarities and differences between these two families of strongly correlated superconductors is an important challenge. American Association for the Advancement of Science 2023-01-13 /pmc/articles/PMC9839319/ /pubmed/36638179 http://dx.doi.org/10.1126/sciadv.ade4418 Text en Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution license (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences Li, Haoxiang Hao, Peipei Zhang, Junjie Gordon, Kyle Linn, A. Garrison Chen, Xinglong Zheng, Hong Zhou, Xiaoqing Mitchell, J. F. Dessau, D. S. Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) |
title | Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) |
title_full | Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) |
title_fullStr | Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) |
title_full_unstemmed | Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) |
title_short | Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) |
title_sort | electronic structure and correlations in planar trilayer nickelate pr(4)ni(3)o(8) |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9839319/ https://www.ncbi.nlm.nih.gov/pubmed/36638179 http://dx.doi.org/10.1126/sciadv.ade4418 |
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