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Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)

The discovery of superconductivity in planar nickelates raises the question of how the electronic structure and correlations of Ni(1+) compounds compare to those of the Cu(2+) cuprate superconductors. Here, we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickela...

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Autores principales: Li, Haoxiang, Hao, Peipei, Zhang, Junjie, Gordon, Kyle, Linn, A. Garrison, Chen, Xinglong, Zheng, Hong, Zhou, Xiaoqing, Mitchell, J. F., Dessau, D. S.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9839319/
https://www.ncbi.nlm.nih.gov/pubmed/36638179
http://dx.doi.org/10.1126/sciadv.ade4418
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author Li, Haoxiang
Hao, Peipei
Zhang, Junjie
Gordon, Kyle
Linn, A. Garrison
Chen, Xinglong
Zheng, Hong
Zhou, Xiaoqing
Mitchell, J. F.
Dessau, D. S.
author_facet Li, Haoxiang
Hao, Peipei
Zhang, Junjie
Gordon, Kyle
Linn, A. Garrison
Chen, Xinglong
Zheng, Hong
Zhou, Xiaoqing
Mitchell, J. F.
Dessau, D. S.
author_sort Li, Haoxiang
collection PubMed
description The discovery of superconductivity in planar nickelates raises the question of how the electronic structure and correlations of Ni(1+) compounds compare to those of the Cu(2+) cuprate superconductors. Here, we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickelate Pr(4)Ni(3)O(8), revealing a Fermi surface resembling that of the hole-doped cuprates but with critical differences. Specifically, the main portions of the Fermi surface are extremely similar to that of the bilayer cuprates, with an additional piece that can accommodate additional hole doping. We find that the electronic correlations are about twice as strong in the nickelates and are almost k-independent, indicating that they originate from a local effect, likely the Mott interaction, whereas cuprate interactions are somewhat less local. Nevertheless, the nickelates still demonstrate the strange-metal behavior in the electron scattering rates. Understanding the similarities and differences between these two families of strongly correlated superconductors is an important challenge.
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spelling pubmed-98393192023-01-24 Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8) Li, Haoxiang Hao, Peipei Zhang, Junjie Gordon, Kyle Linn, A. Garrison Chen, Xinglong Zheng, Hong Zhou, Xiaoqing Mitchell, J. F. Dessau, D. S. Sci Adv Physical and Materials Sciences The discovery of superconductivity in planar nickelates raises the question of how the electronic structure and correlations of Ni(1+) compounds compare to those of the Cu(2+) cuprate superconductors. Here, we present an angle-resolved photoemission spectroscopy (ARPES) study of the trilayer nickelate Pr(4)Ni(3)O(8), revealing a Fermi surface resembling that of the hole-doped cuprates but with critical differences. Specifically, the main portions of the Fermi surface are extremely similar to that of the bilayer cuprates, with an additional piece that can accommodate additional hole doping. We find that the electronic correlations are about twice as strong in the nickelates and are almost k-independent, indicating that they originate from a local effect, likely the Mott interaction, whereas cuprate interactions are somewhat less local. Nevertheless, the nickelates still demonstrate the strange-metal behavior in the electron scattering rates. Understanding the similarities and differences between these two families of strongly correlated superconductors is an important challenge. American Association for the Advancement of Science 2023-01-13 /pmc/articles/PMC9839319/ /pubmed/36638179 http://dx.doi.org/10.1126/sciadv.ade4418 Text en Copyright © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution license (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Li, Haoxiang
Hao, Peipei
Zhang, Junjie
Gordon, Kyle
Linn, A. Garrison
Chen, Xinglong
Zheng, Hong
Zhou, Xiaoqing
Mitchell, J. F.
Dessau, D. S.
Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
title Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
title_full Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
title_fullStr Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
title_full_unstemmed Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
title_short Electronic structure and correlations in planar trilayer nickelate Pr(4)Ni(3)O(8)
title_sort electronic structure and correlations in planar trilayer nickelate pr(4)ni(3)o(8)
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9839319/
https://www.ncbi.nlm.nih.gov/pubmed/36638179
http://dx.doi.org/10.1126/sciadv.ade4418
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