Cargando…
Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination
Functional aerogels composed of regenerated cellulose and tungsten oxide were fabricated by implanting tungsten-oxide nanodots into regenerated cellulose fiber. This superfast photochromic property benefitted from the small size and even distribution of tungsten oxide, which was caused by the confin...
Autores principales: | , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9858587/ https://www.ncbi.nlm.nih.gov/pubmed/36661778 http://dx.doi.org/10.3390/gels9010010 |
_version_ | 1784874139034583040 |
---|---|
author | Tang, Yanjin Lai, Yuhan Gao, Ruiqin Chen, Yuxuan Xiong, Kexin Ye, Juan Zheng, Qi Fang, Zhenxing Pang, Guangsheng Lee, Hoo-Jeong |
author_facet | Tang, Yanjin Lai, Yuhan Gao, Ruiqin Chen, Yuxuan Xiong, Kexin Ye, Juan Zheng, Qi Fang, Zhenxing Pang, Guangsheng Lee, Hoo-Jeong |
author_sort | Tang, Yanjin |
collection | PubMed |
description | Functional aerogels composed of regenerated cellulose and tungsten oxide were fabricated by implanting tungsten-oxide nanodots into regenerated cellulose fiber. This superfast photochromic property benefitted from the small size and even distribution of tungsten oxide, which was caused by the confinement effect of the regenerated cellulose fiber. The composite was characterized using XRD and TEM to illustrate the successful loading of tungsten oxide. The composite turned from pale white to bright blue under ambient solar irradiation in five seconds. The evidence of solar absorption and electron paramagnetic resonance (EPR) demonstrated the fast photochromic nature of the composite and its mechanism. Furthermore, carbon fiber filled with preferential growth tungsten-oxide nanorods was obtained by annealing the photochromic composite in a N(2) atmosphere. This annealed product exhibited good absorption across the whole solar spectrum and revealed an excellent photothermal conversion performance. The water evaporation rate reached 1.75 kg m(−2) h(−1) under one sun illumination, which is 4.4 times higher than that of pure water. The photothermal conversion efficiency was 85%, which shows its potential application prospects in seawater desalination. |
format | Online Article Text |
id | pubmed-9858587 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-98585872023-01-21 Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination Tang, Yanjin Lai, Yuhan Gao, Ruiqin Chen, Yuxuan Xiong, Kexin Ye, Juan Zheng, Qi Fang, Zhenxing Pang, Guangsheng Lee, Hoo-Jeong Gels Article Functional aerogels composed of regenerated cellulose and tungsten oxide were fabricated by implanting tungsten-oxide nanodots into regenerated cellulose fiber. This superfast photochromic property benefitted from the small size and even distribution of tungsten oxide, which was caused by the confinement effect of the regenerated cellulose fiber. The composite was characterized using XRD and TEM to illustrate the successful loading of tungsten oxide. The composite turned from pale white to bright blue under ambient solar irradiation in five seconds. The evidence of solar absorption and electron paramagnetic resonance (EPR) demonstrated the fast photochromic nature of the composite and its mechanism. Furthermore, carbon fiber filled with preferential growth tungsten-oxide nanorods was obtained by annealing the photochromic composite in a N(2) atmosphere. This annealed product exhibited good absorption across the whole solar spectrum and revealed an excellent photothermal conversion performance. The water evaporation rate reached 1.75 kg m(−2) h(−1) under one sun illumination, which is 4.4 times higher than that of pure water. The photothermal conversion efficiency was 85%, which shows its potential application prospects in seawater desalination. MDPI 2022-12-25 /pmc/articles/PMC9858587/ /pubmed/36661778 http://dx.doi.org/10.3390/gels9010010 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Tang, Yanjin Lai, Yuhan Gao, Ruiqin Chen, Yuxuan Xiong, Kexin Ye, Juan Zheng, Qi Fang, Zhenxing Pang, Guangsheng Lee, Hoo-Jeong Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination |
title | Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination |
title_full | Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination |
title_fullStr | Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination |
title_full_unstemmed | Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination |
title_short | Functional Aerogels Composed of Regenerated Cellulose and Tungsten Oxide for UV Detection and Seawater Desalination |
title_sort | functional aerogels composed of regenerated cellulose and tungsten oxide for uv detection and seawater desalination |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9858587/ https://www.ncbi.nlm.nih.gov/pubmed/36661778 http://dx.doi.org/10.3390/gels9010010 |
work_keys_str_mv | AT tangyanjin functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT laiyuhan functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT gaoruiqin functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT chenyuxuan functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT xiongkexin functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT yejuan functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT zhengqi functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT fangzhenxing functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT pangguangsheng functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination AT leehoojeong functionalaerogelscomposedofregeneratedcelluloseandtungstenoxideforuvdetectionandseawaterdesalination |