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Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion

We investigate analytically and numerically a basic model of driven Brownian motion with a velocity-dependent friction coefficient in nonlinear viscoelastic media featured by a stress plateau at intermediate shear velocities and profound memory effects. For constant force driving, we show that nonli...

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Autor principal: Goychuk, Igor
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9860327/
https://www.ncbi.nlm.nih.gov/pubmed/36417440
http://dx.doi.org/10.1073/pnas.2205637119
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author Goychuk, Igor
author_facet Goychuk, Igor
author_sort Goychuk, Igor
collection PubMed
description We investigate analytically and numerically a basic model of driven Brownian motion with a velocity-dependent friction coefficient in nonlinear viscoelastic media featured by a stress plateau at intermediate shear velocities and profound memory effects. For constant force driving, we show that nonlinear oscillations of a microparticle velocity and position emerge by a Hopf bifurcation at a small critical force (first dynamical phase transition), where the friction’s nonlinearity seems to be wholly negligible. They also disappear by a second Hopf bifurcation at a much larger force value (second dynamical phase transition). The bifurcation diagram is found in an analytical form confirmed by numerics. Surprisingly, the particles’ inertial and the medium’s nonlinear properties remain crucial even in a parameter regime where they were earlier considered entirely negligible. Depending on the force and other parameters, the amplitude of oscillations can significantly exceed the size of the particles, and their period can span several time decades, primarily determined by the memory time of the medium. Such oscillations can also be thermally excited near the edges of dynamical phase transitions. The second dynamical phase transition combined with thermally induced stochastic limit cycle oscillations leads to a giant enhancement of diffusion over the limit of vast driving forces, where an effective linearization of stochastic dynamics occurs.
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spelling pubmed-98603272023-05-22 Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion Goychuk, Igor Proc Natl Acad Sci U S A Physical Sciences We investigate analytically and numerically a basic model of driven Brownian motion with a velocity-dependent friction coefficient in nonlinear viscoelastic media featured by a stress plateau at intermediate shear velocities and profound memory effects. For constant force driving, we show that nonlinear oscillations of a microparticle velocity and position emerge by a Hopf bifurcation at a small critical force (first dynamical phase transition), where the friction’s nonlinearity seems to be wholly negligible. They also disappear by a second Hopf bifurcation at a much larger force value (second dynamical phase transition). The bifurcation diagram is found in an analytical form confirmed by numerics. Surprisingly, the particles’ inertial and the medium’s nonlinear properties remain crucial even in a parameter regime where they were earlier considered entirely negligible. Depending on the force and other parameters, the amplitude of oscillations can significantly exceed the size of the particles, and their period can span several time decades, primarily determined by the memory time of the medium. Such oscillations can also be thermally excited near the edges of dynamical phase transitions. The second dynamical phase transition combined with thermally induced stochastic limit cycle oscillations leads to a giant enhancement of diffusion over the limit of vast driving forces, where an effective linearization of stochastic dynamics occurs. National Academy of Sciences 2022-11-22 2022-11-29 /pmc/articles/PMC9860327/ /pubmed/36417440 http://dx.doi.org/10.1073/pnas.2205637119 Text en Copyright © 2022 the Author(s). Published by PNAS. https://creativecommons.org/licenses/by-nc-nd/4.0/This article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND) (https://creativecommons.org/licenses/by-nc-nd/4.0/) .
spellingShingle Physical Sciences
Goychuk, Igor
Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
title Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
title_full Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
title_fullStr Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
title_full_unstemmed Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
title_short Memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
title_sort memory can induce oscillations of microparticles in nonlinear viscoelastic media and cause a giant enhancement of driven diffusion
topic Physical Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9860327/
https://www.ncbi.nlm.nih.gov/pubmed/36417440
http://dx.doi.org/10.1073/pnas.2205637119
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