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Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction

The rapid depletion of fossil fuels and environmental pollution has motivated scientists to cultivate renewable and green energy sources. The hydrogen economy is an emerging replacement for fossil fuels, and photocatalytic water splitting is a suitable strategy to produce clean hydrogen fuel. Herein...

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Autores principales: Altaf, Amna, Sohail, Manzar, Nafady, Ayman, Siddique, Rashid G., Shah, Syed Shoaib Ahmad, Najam, Tayyaba
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9864274/
https://www.ncbi.nlm.nih.gov/pubmed/36677631
http://dx.doi.org/10.3390/molecules28020572
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author Altaf, Amna
Sohail, Manzar
Nafady, Ayman
Siddique, Rashid G.
Shah, Syed Shoaib Ahmad
Najam, Tayyaba
author_facet Altaf, Amna
Sohail, Manzar
Nafady, Ayman
Siddique, Rashid G.
Shah, Syed Shoaib Ahmad
Najam, Tayyaba
author_sort Altaf, Amna
collection PubMed
description The rapid depletion of fossil fuels and environmental pollution has motivated scientists to cultivate renewable and green energy sources. The hydrogen economy is an emerging replacement for fossil fuels, and photocatalytic water splitting is a suitable strategy to produce clean hydrogen fuel. Herein, the photocatalyst (PdO.TiO(2)) is introduced as an accelerated photoelectrochemical oxygen evolution reaction (OER). The catalyst showed significant improvement in the current density magnitude from 0.89 (dark) to 4.27 mA/cm(2) (light) during OER at 0.5 V applied potential. The as-synthesized material exhibits a Tafel slope of 170 mVdec(−1) and efficiency of 0.25% at 0.93 V. The overall outcomes associated with the photocatalytic activity of PdO.TiO(2) demonstrated that the catalyst is highly efficient, thereby encouraging researchers to explore more related catalysts for promoting facile OER.
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spelling pubmed-98642742023-01-22 Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction Altaf, Amna Sohail, Manzar Nafady, Ayman Siddique, Rashid G. Shah, Syed Shoaib Ahmad Najam, Tayyaba Molecules Article The rapid depletion of fossil fuels and environmental pollution has motivated scientists to cultivate renewable and green energy sources. The hydrogen economy is an emerging replacement for fossil fuels, and photocatalytic water splitting is a suitable strategy to produce clean hydrogen fuel. Herein, the photocatalyst (PdO.TiO(2)) is introduced as an accelerated photoelectrochemical oxygen evolution reaction (OER). The catalyst showed significant improvement in the current density magnitude from 0.89 (dark) to 4.27 mA/cm(2) (light) during OER at 0.5 V applied potential. The as-synthesized material exhibits a Tafel slope of 170 mVdec(−1) and efficiency of 0.25% at 0.93 V. The overall outcomes associated with the photocatalytic activity of PdO.TiO(2) demonstrated that the catalyst is highly efficient, thereby encouraging researchers to explore more related catalysts for promoting facile OER. MDPI 2023-01-06 /pmc/articles/PMC9864274/ /pubmed/36677631 http://dx.doi.org/10.3390/molecules28020572 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Altaf, Amna
Sohail, Manzar
Nafady, Ayman
Siddique, Rashid G.
Shah, Syed Shoaib Ahmad
Najam, Tayyaba
Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
title Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
title_full Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
title_fullStr Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
title_full_unstemmed Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
title_short Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
title_sort facile synthesis of pdo.tio(2) nanocomposite for photoelectrochemical oxygen evolution reaction
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9864274/
https://www.ncbi.nlm.nih.gov/pubmed/36677631
http://dx.doi.org/10.3390/molecules28020572
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