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Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction
The rapid depletion of fossil fuels and environmental pollution has motivated scientists to cultivate renewable and green energy sources. The hydrogen economy is an emerging replacement for fossil fuels, and photocatalytic water splitting is a suitable strategy to produce clean hydrogen fuel. Herein...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9864274/ https://www.ncbi.nlm.nih.gov/pubmed/36677631 http://dx.doi.org/10.3390/molecules28020572 |
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author | Altaf, Amna Sohail, Manzar Nafady, Ayman Siddique, Rashid G. Shah, Syed Shoaib Ahmad Najam, Tayyaba |
author_facet | Altaf, Amna Sohail, Manzar Nafady, Ayman Siddique, Rashid G. Shah, Syed Shoaib Ahmad Najam, Tayyaba |
author_sort | Altaf, Amna |
collection | PubMed |
description | The rapid depletion of fossil fuels and environmental pollution has motivated scientists to cultivate renewable and green energy sources. The hydrogen economy is an emerging replacement for fossil fuels, and photocatalytic water splitting is a suitable strategy to produce clean hydrogen fuel. Herein, the photocatalyst (PdO.TiO(2)) is introduced as an accelerated photoelectrochemical oxygen evolution reaction (OER). The catalyst showed significant improvement in the current density magnitude from 0.89 (dark) to 4.27 mA/cm(2) (light) during OER at 0.5 V applied potential. The as-synthesized material exhibits a Tafel slope of 170 mVdec(−1) and efficiency of 0.25% at 0.93 V. The overall outcomes associated with the photocatalytic activity of PdO.TiO(2) demonstrated that the catalyst is highly efficient, thereby encouraging researchers to explore more related catalysts for promoting facile OER. |
format | Online Article Text |
id | pubmed-9864274 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-98642742023-01-22 Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction Altaf, Amna Sohail, Manzar Nafady, Ayman Siddique, Rashid G. Shah, Syed Shoaib Ahmad Najam, Tayyaba Molecules Article The rapid depletion of fossil fuels and environmental pollution has motivated scientists to cultivate renewable and green energy sources. The hydrogen economy is an emerging replacement for fossil fuels, and photocatalytic water splitting is a suitable strategy to produce clean hydrogen fuel. Herein, the photocatalyst (PdO.TiO(2)) is introduced as an accelerated photoelectrochemical oxygen evolution reaction (OER). The catalyst showed significant improvement in the current density magnitude from 0.89 (dark) to 4.27 mA/cm(2) (light) during OER at 0.5 V applied potential. The as-synthesized material exhibits a Tafel slope of 170 mVdec(−1) and efficiency of 0.25% at 0.93 V. The overall outcomes associated with the photocatalytic activity of PdO.TiO(2) demonstrated that the catalyst is highly efficient, thereby encouraging researchers to explore more related catalysts for promoting facile OER. MDPI 2023-01-06 /pmc/articles/PMC9864274/ /pubmed/36677631 http://dx.doi.org/10.3390/molecules28020572 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Altaf, Amna Sohail, Manzar Nafady, Ayman Siddique, Rashid G. Shah, Syed Shoaib Ahmad Najam, Tayyaba Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction |
title | Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction |
title_full | Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction |
title_fullStr | Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction |
title_full_unstemmed | Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction |
title_short | Facile Synthesis of PdO.TiO(2) Nanocomposite for Photoelectrochemical Oxygen Evolution Reaction |
title_sort | facile synthesis of pdo.tio(2) nanocomposite for photoelectrochemical oxygen evolution reaction |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9864274/ https://www.ncbi.nlm.nih.gov/pubmed/36677631 http://dx.doi.org/10.3390/molecules28020572 |
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