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Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
In this article, we investigate an active plasmonic element which will act as the key building block for future photonic devices. This element operates by modulating optical constants in a localised fashion, thereby providing an external control over the strength of the electromagnetic near field ab...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Beilstein-Institut
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9874232/ https://www.ncbi.nlm.nih.gov/pubmed/36743300 http://dx.doi.org/10.3762/bjnano.14.12 |
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author | Barron, Ciarán Di Fazio, Giulia Kenny, Samuel O’Toole, Silas O’Reilly, Robin Zerulla, Dominic |
author_facet | Barron, Ciarán Di Fazio, Giulia Kenny, Samuel O’Toole, Silas O’Reilly, Robin Zerulla, Dominic |
author_sort | Barron, Ciarán |
collection | PubMed |
description | In this article, we investigate an active plasmonic element which will act as the key building block for future photonic devices. This element operates by modulating optical constants in a localised fashion, thereby providing an external control over the strength of the electromagnetic near field above the element as well as its far-field response. A dual experimental approach is employed in tandem with computational methods to characterise the response of this system. First, an enhanced surface plasmon resonance experiment in a classical Kretschmann configuration is used to measure the changes in the reflectivity induced by an alternating electric current. A lock-in amplifier is used to extract the dynamic changes in the far-field reflectivity resulting from Joule heating. A clear modulation of the materials’ optical constants can be inferred from the changed reflectivity, which is highly sensitive and dependent on the input current. The changed electrical permittivity of the active element is due to Joule heating. Second, the resulting expansion of the metallic element is measured using scanning Joule expansion microscopy. The localised temperature distribution, and hence information about the localisation of the modulation of the optical constants of the system, can be extracted using this technique. Both optical and thermal data are used to inform detailed finite element method simulations for verification and to predict system responses allowing for enhanced design choices to maximise modulation depth and localisation. |
format | Online Article Text |
id | pubmed-9874232 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | Beilstein-Institut |
record_format | MEDLINE/PubMed |
spelling | pubmed-98742322023-02-02 Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods Barron, Ciarán Di Fazio, Giulia Kenny, Samuel O’Toole, Silas O’Reilly, Robin Zerulla, Dominic Beilstein J Nanotechnol Full Research Paper In this article, we investigate an active plasmonic element which will act as the key building block for future photonic devices. This element operates by modulating optical constants in a localised fashion, thereby providing an external control over the strength of the electromagnetic near field above the element as well as its far-field response. A dual experimental approach is employed in tandem with computational methods to characterise the response of this system. First, an enhanced surface plasmon resonance experiment in a classical Kretschmann configuration is used to measure the changes in the reflectivity induced by an alternating electric current. A lock-in amplifier is used to extract the dynamic changes in the far-field reflectivity resulting from Joule heating. A clear modulation of the materials’ optical constants can be inferred from the changed reflectivity, which is highly sensitive and dependent on the input current. The changed electrical permittivity of the active element is due to Joule heating. Second, the resulting expansion of the metallic element is measured using scanning Joule expansion microscopy. The localised temperature distribution, and hence information about the localisation of the modulation of the optical constants of the system, can be extracted using this technique. Both optical and thermal data are used to inform detailed finite element method simulations for verification and to predict system responses allowing for enhanced design choices to maximise modulation depth and localisation. Beilstein-Institut 2023-01-16 /pmc/articles/PMC9874232/ /pubmed/36743300 http://dx.doi.org/10.3762/bjnano.14.12 Text en Copyright © 2023, Barron et al. https://creativecommons.org/licenses/by/4.0/This is an open access article licensed under the terms of the Beilstein-Institut Open Access License Agreement (https://www.beilstein-journals.org/bjnano/terms/terms), which is identical to the Creative Commons Attribution 4.0 International License (https://creativecommons.org/licenses/by/4.0 (https://creativecommons.org/licenses/by/4.0/) ). The reuse of material under this license requires that the author(s), source and license are credited. Third-party material in this article could be subject to other licenses (typically indicated in the credit line), and in this case, users are required to obtain permission from the license holder to reuse the material. |
spellingShingle | Full Research Paper Barron, Ciarán Di Fazio, Giulia Kenny, Samuel O’Toole, Silas O’Reilly, Robin Zerulla, Dominic Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
title | Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
title_full | Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
title_fullStr | Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
title_full_unstemmed | Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
title_short | Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
title_sort | characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods |
topic | Full Research Paper |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9874232/ https://www.ncbi.nlm.nih.gov/pubmed/36743300 http://dx.doi.org/10.3762/bjnano.14.12 |
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