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Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods

In this article, we investigate an active plasmonic element which will act as the key building block for future photonic devices. This element operates by modulating optical constants in a localised fashion, thereby providing an external control over the strength of the electromagnetic near field ab...

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Autores principales: Barron, Ciarán, Di Fazio, Giulia, Kenny, Samuel, O’Toole, Silas, O’Reilly, Robin, Zerulla, Dominic
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Beilstein-Institut 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9874232/
https://www.ncbi.nlm.nih.gov/pubmed/36743300
http://dx.doi.org/10.3762/bjnano.14.12
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author Barron, Ciarán
Di Fazio, Giulia
Kenny, Samuel
O’Toole, Silas
O’Reilly, Robin
Zerulla, Dominic
author_facet Barron, Ciarán
Di Fazio, Giulia
Kenny, Samuel
O’Toole, Silas
O’Reilly, Robin
Zerulla, Dominic
author_sort Barron, Ciarán
collection PubMed
description In this article, we investigate an active plasmonic element which will act as the key building block for future photonic devices. This element operates by modulating optical constants in a localised fashion, thereby providing an external control over the strength of the electromagnetic near field above the element as well as its far-field response. A dual experimental approach is employed in tandem with computational methods to characterise the response of this system. First, an enhanced surface plasmon resonance experiment in a classical Kretschmann configuration is used to measure the changes in the reflectivity induced by an alternating electric current. A lock-in amplifier is used to extract the dynamic changes in the far-field reflectivity resulting from Joule heating. A clear modulation of the materials’ optical constants can be inferred from the changed reflectivity, which is highly sensitive and dependent on the input current. The changed electrical permittivity of the active element is due to Joule heating. Second, the resulting expansion of the metallic element is measured using scanning Joule expansion microscopy. The localised temperature distribution, and hence information about the localisation of the modulation of the optical constants of the system, can be extracted using this technique. Both optical and thermal data are used to inform detailed finite element method simulations for verification and to predict system responses allowing for enhanced design choices to maximise modulation depth and localisation.
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spelling pubmed-98742322023-02-02 Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods Barron, Ciarán Di Fazio, Giulia Kenny, Samuel O’Toole, Silas O’Reilly, Robin Zerulla, Dominic Beilstein J Nanotechnol Full Research Paper In this article, we investigate an active plasmonic element which will act as the key building block for future photonic devices. This element operates by modulating optical constants in a localised fashion, thereby providing an external control over the strength of the electromagnetic near field above the element as well as its far-field response. A dual experimental approach is employed in tandem with computational methods to characterise the response of this system. First, an enhanced surface plasmon resonance experiment in a classical Kretschmann configuration is used to measure the changes in the reflectivity induced by an alternating electric current. A lock-in amplifier is used to extract the dynamic changes in the far-field reflectivity resulting from Joule heating. A clear modulation of the materials’ optical constants can be inferred from the changed reflectivity, which is highly sensitive and dependent on the input current. The changed electrical permittivity of the active element is due to Joule heating. Second, the resulting expansion of the metallic element is measured using scanning Joule expansion microscopy. The localised temperature distribution, and hence information about the localisation of the modulation of the optical constants of the system, can be extracted using this technique. Both optical and thermal data are used to inform detailed finite element method simulations for verification and to predict system responses allowing for enhanced design choices to maximise modulation depth and localisation. Beilstein-Institut 2023-01-16 /pmc/articles/PMC9874232/ /pubmed/36743300 http://dx.doi.org/10.3762/bjnano.14.12 Text en Copyright © 2023, Barron et al. https://creativecommons.org/licenses/by/4.0/This is an open access article licensed under the terms of the Beilstein-Institut Open Access License Agreement (https://www.beilstein-journals.org/bjnano/terms/terms), which is identical to the Creative Commons Attribution 4.0 International License (https://creativecommons.org/licenses/by/4.0 (https://creativecommons.org/licenses/by/4.0/) ). The reuse of material under this license requires that the author(s), source and license are credited. Third-party material in this article could be subject to other licenses (typically indicated in the credit line), and in this case, users are required to obtain permission from the license holder to reuse the material.
spellingShingle Full Research Paper
Barron, Ciarán
Di Fazio, Giulia
Kenny, Samuel
O’Toole, Silas
O’Reilly, Robin
Zerulla, Dominic
Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
title Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
title_full Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
title_fullStr Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
title_full_unstemmed Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
title_short Characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
title_sort characterisation of a micrometer-scale active plasmonic element by means of complementary computational and experimental methods
topic Full Research Paper
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9874232/
https://www.ncbi.nlm.nih.gov/pubmed/36743300
http://dx.doi.org/10.3762/bjnano.14.12
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