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Attosecond field emission

Field emission of electrons underlies great advances in science and technology, ranging from signal processing at ever higher frequencies(1) to imaging of the atomic-scale structure of matter(2) with picometre resolution. The advancing of electron microscopy techniques to enable the complete visuali...

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Autores principales: Kim, H. Y., Garg, M., Mandal, S., Seiffert, L., Fennel, T., Goulielmakis, E.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9876796/
https://www.ncbi.nlm.nih.gov/pubmed/36697865
http://dx.doi.org/10.1038/s41586-022-05577-1
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author Kim, H. Y.
Garg, M.
Mandal, S.
Seiffert, L.
Fennel, T.
Goulielmakis, E.
author_facet Kim, H. Y.
Garg, M.
Mandal, S.
Seiffert, L.
Fennel, T.
Goulielmakis, E.
author_sort Kim, H. Y.
collection PubMed
description Field emission of electrons underlies great advances in science and technology, ranging from signal processing at ever higher frequencies(1) to imaging of the atomic-scale structure of matter(2) with picometre resolution. The advancing of electron microscopy techniques to enable the complete visualization of matter on the native spatial (picometre) and temporal (attosecond) scales of electron dynamics calls for techniques that can confine and examine the field emission on sub-femtosecond time intervals. Intense laser pulses have paved the way to this end(3,4) by demonstrating femtosecond confinement(5,6) and sub-optical cycle control(7,8) of the optical field emission(9) from nanostructured metals. Yet the measurement of attosecond electron pulses has remained elusive. We used intense, sub-cycle light transients to induce optical field emission of electron pulses from tungsten nanotips and a weak replica of the same transient to directly investigate the emission dynamics in real time. Access to the temporal properties of the electron pulses rescattering off the tip surface, including the duration τ = (53 as ± 5 as) and chirp, and the direct exploration of nanoscale near fields open new prospects for research and applications at the interface of attosecond physics and nano-optics.
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spelling pubmed-98767962023-01-27 Attosecond field emission Kim, H. Y. Garg, M. Mandal, S. Seiffert, L. Fennel, T. Goulielmakis, E. Nature Article Field emission of electrons underlies great advances in science and technology, ranging from signal processing at ever higher frequencies(1) to imaging of the atomic-scale structure of matter(2) with picometre resolution. The advancing of electron microscopy techniques to enable the complete visualization of matter on the native spatial (picometre) and temporal (attosecond) scales of electron dynamics calls for techniques that can confine and examine the field emission on sub-femtosecond time intervals. Intense laser pulses have paved the way to this end(3,4) by demonstrating femtosecond confinement(5,6) and sub-optical cycle control(7,8) of the optical field emission(9) from nanostructured metals. Yet the measurement of attosecond electron pulses has remained elusive. We used intense, sub-cycle light transients to induce optical field emission of electron pulses from tungsten nanotips and a weak replica of the same transient to directly investigate the emission dynamics in real time. Access to the temporal properties of the electron pulses rescattering off the tip surface, including the duration τ = (53 as ± 5 as) and chirp, and the direct exploration of nanoscale near fields open new prospects for research and applications at the interface of attosecond physics and nano-optics. Nature Publishing Group UK 2023-01-25 2023 /pmc/articles/PMC9876796/ /pubmed/36697865 http://dx.doi.org/10.1038/s41586-022-05577-1 Text en © The Author(s) 2023 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Kim, H. Y.
Garg, M.
Mandal, S.
Seiffert, L.
Fennel, T.
Goulielmakis, E.
Attosecond field emission
title Attosecond field emission
title_full Attosecond field emission
title_fullStr Attosecond field emission
title_full_unstemmed Attosecond field emission
title_short Attosecond field emission
title_sort attosecond field emission
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9876796/
https://www.ncbi.nlm.nih.gov/pubmed/36697865
http://dx.doi.org/10.1038/s41586-022-05577-1
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