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A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors

Electrochemical ultracapacitors derived from green and sustainable materials could demonstrate superior energy output and an ultra-long cycle life owing to large accessible surface area and obviously shortened ion diffusion pathways. Herein, we have established an efficient strategy to fabricate por...

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Detalles Bibliográficos
Autores principales: Liu, Han, Zhang, Fumin, Lin, Xinyu, Wu, Jinggao, Huang, Jing
Formato: Online Artículo Texto
Lenguaje:English
Publicado: RSC 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9890899/
https://www.ncbi.nlm.nih.gov/pubmed/36756496
http://dx.doi.org/10.1039/d2na00758d
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author Liu, Han
Zhang, Fumin
Lin, Xinyu
Wu, Jinggao
Huang, Jing
author_facet Liu, Han
Zhang, Fumin
Lin, Xinyu
Wu, Jinggao
Huang, Jing
author_sort Liu, Han
collection PubMed
description Electrochemical ultracapacitors derived from green and sustainable materials could demonstrate superior energy output and an ultra-long cycle life owing to large accessible surface area and obviously shortened ion diffusion pathways. Herein, we have established an efficient strategy to fabricate porous carbon (GLAC) from sustainable gingko leaf precursors by a facile hydrothermal activation of H(3)PO(4) and low-cost pyrolysis. In this way, GLAC with a hierarchically porous structure exhibits extraordinary adaptability toward a high energy/power supercapacitor (∼709 F g(−1) at 1 A g(−1)) in an aqueous electrolyte (1 M KOH). Notably, the GLAC-2-based supercapacitor displays an ultra-high stability of ∼98.24% even after 10 000 cycles (10 A g(−1)) and an impressive energy density as large as ∼71 W h kg(−1) at a power density of 1.2 kW kg(−1). The results provide new insights that the facile synthetic procedure coupled with the excellent performance contributes to great potential for future application in the electrochemical energy storage field.
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spelling pubmed-98908992023-02-07 A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors Liu, Han Zhang, Fumin Lin, Xinyu Wu, Jinggao Huang, Jing Nanoscale Adv Chemistry Electrochemical ultracapacitors derived from green and sustainable materials could demonstrate superior energy output and an ultra-long cycle life owing to large accessible surface area and obviously shortened ion diffusion pathways. Herein, we have established an efficient strategy to fabricate porous carbon (GLAC) from sustainable gingko leaf precursors by a facile hydrothermal activation of H(3)PO(4) and low-cost pyrolysis. In this way, GLAC with a hierarchically porous structure exhibits extraordinary adaptability toward a high energy/power supercapacitor (∼709 F g(−1) at 1 A g(−1)) in an aqueous electrolyte (1 M KOH). Notably, the GLAC-2-based supercapacitor displays an ultra-high stability of ∼98.24% even after 10 000 cycles (10 A g(−1)) and an impressive energy density as large as ∼71 W h kg(−1) at a power density of 1.2 kW kg(−1). The results provide new insights that the facile synthetic procedure coupled with the excellent performance contributes to great potential for future application in the electrochemical energy storage field. RSC 2023-01-10 /pmc/articles/PMC9890899/ /pubmed/36756496 http://dx.doi.org/10.1039/d2na00758d Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Liu, Han
Zhang, Fumin
Lin, Xinyu
Wu, Jinggao
Huang, Jing
A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors
title A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors
title_full A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors
title_fullStr A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors
title_full_unstemmed A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors
title_short A hierarchical integrated 3D carbon electrode derived from gingko leaves via hydrothermal carbonization of H(3)PO(4) for high-performance supercapacitors
title_sort hierarchical integrated 3d carbon electrode derived from gingko leaves via hydrothermal carbonization of h(3)po(4) for high-performance supercapacitors
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9890899/
https://www.ncbi.nlm.nih.gov/pubmed/36756496
http://dx.doi.org/10.1039/d2na00758d
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