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Dipolar-Coupled Entangled Molecular 4f Qubits

[Image: see text] We demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute Yb(III) ions in Yb(0.01)Lu(0.99)(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interact...

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Autores principales: Bode, Bela E., Fusco, Edoardo, Nixon, Rachel, Buch, Christian D., Weihe, Høgni, Piligkos, Stergios
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2023
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9912257/
https://www.ncbi.nlm.nih.gov/pubmed/36695706
http://dx.doi.org/10.1021/jacs.2c10902
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author Bode, Bela E.
Fusco, Edoardo
Nixon, Rachel
Buch, Christian D.
Weihe, Høgni
Piligkos, Stergios
author_facet Bode, Bela E.
Fusco, Edoardo
Nixon, Rachel
Buch, Christian D.
Weihe, Høgni
Piligkos, Stergios
author_sort Bode, Bela E.
collection PubMed
description [Image: see text] We demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute Yb(III) ions in Yb(0.01)Lu(0.99)(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interactions between neighboring Yb(III) centers. Furthermore, we show that the phase memory time and Rabi frequencies of these dipolar-interaction-coupled entangled two-qubit systems are comparable to the ones of the corresponding single qubits.
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spelling pubmed-99122572023-02-11 Dipolar-Coupled Entangled Molecular 4f Qubits Bode, Bela E. Fusco, Edoardo Nixon, Rachel Buch, Christian D. Weihe, Høgni Piligkos, Stergios J Am Chem Soc [Image: see text] We demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute Yb(III) ions in Yb(0.01)Lu(0.99)(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interactions between neighboring Yb(III) centers. Furthermore, we show that the phase memory time and Rabi frequencies of these dipolar-interaction-coupled entangled two-qubit systems are comparable to the ones of the corresponding single qubits. American Chemical Society 2023-01-25 /pmc/articles/PMC9912257/ /pubmed/36695706 http://dx.doi.org/10.1021/jacs.2c10902 Text en © 2023 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Bode, Bela E.
Fusco, Edoardo
Nixon, Rachel
Buch, Christian D.
Weihe, Høgni
Piligkos, Stergios
Dipolar-Coupled Entangled Molecular 4f Qubits
title Dipolar-Coupled Entangled Molecular 4f Qubits
title_full Dipolar-Coupled Entangled Molecular 4f Qubits
title_fullStr Dipolar-Coupled Entangled Molecular 4f Qubits
title_full_unstemmed Dipolar-Coupled Entangled Molecular 4f Qubits
title_short Dipolar-Coupled Entangled Molecular 4f Qubits
title_sort dipolar-coupled entangled molecular 4f qubits
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9912257/
https://www.ncbi.nlm.nih.gov/pubmed/36695706
http://dx.doi.org/10.1021/jacs.2c10902
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