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Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodi...
Autores principales: | , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2023
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9919544/ https://www.ncbi.nlm.nih.gov/pubmed/36770468 http://dx.doi.org/10.3390/nano13030507 |
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author | Kroychuk, Maria K. Shorokhov, Alexander S. Yagudin, Damir F. Rakhlin, Maxim V. Klimko, Grigorii V. Toropov, Alexey A. Shubina, Tatiana V. Fedyanin, Andrey A. |
author_facet | Kroychuk, Maria K. Shorokhov, Alexander S. Yagudin, Damir F. Rakhlin, Maxim V. Klimko, Grigorii V. Toropov, Alexey A. Shubina, Tatiana V. Fedyanin, Andrey A. |
author_sort | Kroychuk, Maria K. |
collection | PubMed |
description | Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodic structures with many thin layers is difficult. On the other hand, the coupling of single-photon sources with resonant nanoclusters made of high-index dielectric materials is known as a promising way for emission control. Our experiments and calculations show that the excitation of magnetic Mie-type resonance by linearly polarized light in a GaAs nanopillar oligomer with embedded InAs quantum dots leads to quantum emitters absorption efficiency enhancement. Moreover, the nanoresonator at the wavelength of magnetic dipole resonance also acts as a nanoantenna for a generated signal, allowing control over its radiation spatial profile. We experimentally demonstrated an order of magnitude emission enhancement and numerically reached forty times gain in comparison with unstructured film. These findings highlight the potential of quantum dots coupling with Mie-resonant oligomers collective modes for nanoscale single-photon sources development. |
format | Online Article Text |
id | pubmed-9919544 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2023 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-99195442023-02-12 Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes Kroychuk, Maria K. Shorokhov, Alexander S. Yagudin, Damir F. Rakhlin, Maxim V. Klimko, Grigorii V. Toropov, Alexey A. Shubina, Tatiana V. Fedyanin, Andrey A. Nanomaterials (Basel) Article Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodic structures with many thin layers is difficult. On the other hand, the coupling of single-photon sources with resonant nanoclusters made of high-index dielectric materials is known as a promising way for emission control. Our experiments and calculations show that the excitation of magnetic Mie-type resonance by linearly polarized light in a GaAs nanopillar oligomer with embedded InAs quantum dots leads to quantum emitters absorption efficiency enhancement. Moreover, the nanoresonator at the wavelength of magnetic dipole resonance also acts as a nanoantenna for a generated signal, allowing control over its radiation spatial profile. We experimentally demonstrated an order of magnitude emission enhancement and numerically reached forty times gain in comparison with unstructured film. These findings highlight the potential of quantum dots coupling with Mie-resonant oligomers collective modes for nanoscale single-photon sources development. MDPI 2023-01-27 /pmc/articles/PMC9919544/ /pubmed/36770468 http://dx.doi.org/10.3390/nano13030507 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Kroychuk, Maria K. Shorokhov, Alexander S. Yagudin, Damir F. Rakhlin, Maxim V. Klimko, Grigorii V. Toropov, Alexey A. Shubina, Tatiana V. Fedyanin, Andrey A. Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes |
title | Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes |
title_full | Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes |
title_fullStr | Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes |
title_full_unstemmed | Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes |
title_short | Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes |
title_sort | quantum dot photoluminescence enhancement in gaas nanopillar oligomers driven by collective magnetic modes |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9919544/ https://www.ncbi.nlm.nih.gov/pubmed/36770468 http://dx.doi.org/10.3390/nano13030507 |
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