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Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes

Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodi...

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Autores principales: Kroychuk, Maria K., Shorokhov, Alexander S., Yagudin, Damir F., Rakhlin, Maxim V., Klimko, Grigorii V., Toropov, Alexey A., Shubina, Tatiana V., Fedyanin, Andrey A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2023
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9919544/
https://www.ncbi.nlm.nih.gov/pubmed/36770468
http://dx.doi.org/10.3390/nano13030507
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author Kroychuk, Maria K.
Shorokhov, Alexander S.
Yagudin, Damir F.
Rakhlin, Maxim V.
Klimko, Grigorii V.
Toropov, Alexey A.
Shubina, Tatiana V.
Fedyanin, Andrey A.
author_facet Kroychuk, Maria K.
Shorokhov, Alexander S.
Yagudin, Damir F.
Rakhlin, Maxim V.
Klimko, Grigorii V.
Toropov, Alexey A.
Shubina, Tatiana V.
Fedyanin, Andrey A.
author_sort Kroychuk, Maria K.
collection PubMed
description Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodic structures with many thin layers is difficult. On the other hand, the coupling of single-photon sources with resonant nanoclusters made of high-index dielectric materials is known as a promising way for emission control. Our experiments and calculations show that the excitation of magnetic Mie-type resonance by linearly polarized light in a GaAs nanopillar oligomer with embedded InAs quantum dots leads to quantum emitters absorption efficiency enhancement. Moreover, the nanoresonator at the wavelength of magnetic dipole resonance also acts as a nanoantenna for a generated signal, allowing control over its radiation spatial profile. We experimentally demonstrated an order of magnitude emission enhancement and numerically reached forty times gain in comparison with unstructured film. These findings highlight the potential of quantum dots coupling with Mie-resonant oligomers collective modes for nanoscale single-photon sources development.
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spelling pubmed-99195442023-02-12 Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes Kroychuk, Maria K. Shorokhov, Alexander S. Yagudin, Damir F. Rakhlin, Maxim V. Klimko, Grigorii V. Toropov, Alexey A. Shubina, Tatiana V. Fedyanin, Andrey A. Nanomaterials (Basel) Article Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodic structures with many thin layers is difficult. On the other hand, the coupling of single-photon sources with resonant nanoclusters made of high-index dielectric materials is known as a promising way for emission control. Our experiments and calculations show that the excitation of magnetic Mie-type resonance by linearly polarized light in a GaAs nanopillar oligomer with embedded InAs quantum dots leads to quantum emitters absorption efficiency enhancement. Moreover, the nanoresonator at the wavelength of magnetic dipole resonance also acts as a nanoantenna for a generated signal, allowing control over its radiation spatial profile. We experimentally demonstrated an order of magnitude emission enhancement and numerically reached forty times gain in comparison with unstructured film. These findings highlight the potential of quantum dots coupling with Mie-resonant oligomers collective modes for nanoscale single-photon sources development. MDPI 2023-01-27 /pmc/articles/PMC9919544/ /pubmed/36770468 http://dx.doi.org/10.3390/nano13030507 Text en © 2023 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Kroychuk, Maria K.
Shorokhov, Alexander S.
Yagudin, Damir F.
Rakhlin, Maxim V.
Klimko, Grigorii V.
Toropov, Alexey A.
Shubina, Tatiana V.
Fedyanin, Andrey A.
Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
title Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
title_full Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
title_fullStr Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
title_full_unstemmed Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
title_short Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes
title_sort quantum dot photoluminescence enhancement in gaas nanopillar oligomers driven by collective magnetic modes
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC9919544/
https://www.ncbi.nlm.nih.gov/pubmed/36770468
http://dx.doi.org/10.3390/nano13030507
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